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ES2369837T3 - Compuestos triheterocíclicos como antagonistas de receptor cfr. - Google Patents

Compuestos triheterocíclicos como antagonistas de receptor cfr. Download PDF

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ES2369837T3
ES2369837T3 ES07111569T ES07111569T ES2369837T3 ES 2369837 T3 ES2369837 T3 ES 2369837T3 ES 07111569 T ES07111569 T ES 07111569T ES 07111569 T ES07111569 T ES 07111569T ES 2369837 T3 ES2369837 T3 ES 2369837T3
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substituted
mono
alkyl
ring
oxygen
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Hisaoono Nakai
Yoshifumiono Kagamiishi
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Ono Pharmaceutical Co Ltd
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Ono Pharmaceutical Co Ltd
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Abstract

Compuesto de fórmulas (I-i), (I-ii) o (I-x) en las que R2 es (i) hidrógeno, (ii) alquilo C1-8, (iii) alquenilo C2-8, (iv) alquinilo C2-8, (v) átomo de halógeno, (vi) CF3, (vii) ciano, (viii) nitro, (ix) NR9R10 en el que R9 y R10 son cada uno independientemente, (i) hidrógeno, (ii) alquilo C1-4, (iii) anillo mono o bicarbocíclico C3-10, (iv) anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) o (v) alquilo C1-4 sustituido con anillo mono o bicarbocíclico C3-10 o anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s), (x) OR11 en el que R11 es (i) hidrógeno, (ii) alquilo C1-4, (iii) anillo carbocíclico C5-6, (iv) anillo heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre o (v) alquilo C1-4 sustituido con anillo carbocíclico C5-6 o anillo heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre, (xi) SH, (xii) S(O)nR12 en el que n es 0, 1 ó 2, R12 es (i) alquilo C1-4, (ii) anillo carbocíclico C5-6, (iii) anillo heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre o (iv) alquilo C1-4 sustituido con anillo carbocíclico C5-6 o anillo 5 heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre, (xiii) COR11, (xiv) COOR11, (xv) CONR9R10, (xvi) anillo mono o bicarbocíclico C3-10, (xvii) anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) o (xviii) alquilo C1-4 sustituido con 1-2 sustituyentes seleccionados de átomo de halógeno, CF3, OCF3, ciano, nitro, NR9R10, OR11, =N-OR11, SH, S(O)nR12, COR11, COOR11, CONR9R10, anillo mono o bicarbocíclico C3- 10 y anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s), en los que G es O, S o NH; Rx es alquilo C1-4, alcoxilo C1-4, átomo de halógeno o CF3; m es 0-3, R1 es (i) alquilo C1-8 que no está sustituido o está sustituido con 1-5 R14, (ii) alquenilo C2-8 que no está sustituido o está sustituido con 1-5 R14, (iii) alquinilo C2-8 que no está sustituido o está sustituido con 1-5 R14, (iv) NR4R5 en el que R4 y R5 son cada uno independientemente, (i) hidrógeno, (ii) alquilo C1-15 que no está sustituido o está sustituido con 1-5 R17, (iii) alquenilo C2-15 que no está sustituido o está sustituido con 1-5 R17, (iv) alquinilo C2-15 que no está sustituido o está sustituido con 1-5 R17, (v) anillo mono o bicarbocíclico C3-15 que no está sustituido o está sustituido con 1-5 R18, (vi) anillo mono o biheterocíclico de 3-15 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18, (v) OR6 en el que R6 es (i) hidrógeno, (ii) alquilo C1-10, (iii) alquenilo C2-10, (iv) alquinilo C2-10, (v) anillo mono o bicarbocíclico C3-15 que no está sustituido o está sustituido con 1-5 R18, (vi) anillo mono o biheterocíclico de 3-15 miembros que contiene 1-4 nitrógeno(s), 1-2 10 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18, (vii) alquilo C1-4 sustituido con 1-2 sustituyentes seleccionados de átomo de halógeno, CF3, OCF3, ciano, nitro, NR9R10, OR11, =N-OR11, SH, S(O)nR12, COR11, COOR11, CONR9R10, anillo mono o bicarbocíclico C3-10 que no está sustituido o está sustituido con 1-5 R18, y anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18, (vi) SH, (vii) S(O)nR7 en el que n es tal como se definió anteriormente en el presente documento, R7 es (i) alquilo C1-8, (ii) anillo mono o bicarbocíclico C3-10 que no está sustituido o está sustituido con 1-5 R18, (iii) anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18, (iv) alquilo C1-4 sustituido con anillo mono o bicarbocíclico C3-10, que no está sustituido o está sustituido con 1-5 R18 o anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1- 5 R18, (viii) COR6, (ix) COOR6, (x) CONR4R5, (xi) NR8COR6a en el que R6a es (i) hidrógeno, (ii) alquilo C1-10, (iii) alquenilo C2-10, (iv) alquinilo C2-10 o (v) alquilo C1-4 sustituido con 1-2 sustituyentes seleccionados de átomo de halógeno, CF3, OCF3, ciano, nitro, NR9R10, OR11a, =N-OR11, SH, S(O)nR12, COR11, COOR11 y CONR9R10, (xii) NR8COOR6 en el que R6 es tal como se definió anteriormente en el presente documento, R8 es (i) hidrógeno, (ii) alquilo C1-8, (iii) alquenilo C2-8, (iv) alquinilo C2-8, (v) anillo mono o bicarbocíclico C3-10 que no está sustituido o está sustituido con 1-5 R18, (vi) anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18 o (vii) alquilo C1-4 sustituido con 1-2 sustituyentes seleccionados de átomo de halógeno, CF3, OCF3, ciano, nitro, NR9R10, OR11, =N-OR11, SH, S(O)nR12, COR11, COOR11, CONR9R10, anillo mono o bicarbocíclico C3-10 que no está sustituido 5 o está sustituido con 1-5 R18 y anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18, (xiii) NR8CONR4R5, (xiv) anillo mono o bicarbocíclico C3-15 que no está sustituido o está sustituido con 1-5 R15 o (xv) anillo mono o biheterocíclico de 3-15 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R15, R11a es (i) hidrógeno, (ii) alquilo C1-4 o (iii) alquilo C1-4 sustituido con anillo carbocíclico C5-6 o anillo heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre, R14 es (a) átomo de halógeno, (b) CF3, (c) OCF3, (d) ciano, (e) nitro, (f) NR4R5, (g) OR6, (h) =N-OR6, (j) SH, (k) S(O)nR7, (l) COR6, (m) COOR6, (n) CONR4R5, (o) NR8COR6, (p) NR8COOR6, (q) NR8CONR4R5, (r) anillo mono o bicarbocíclico C3-15 que no está sustituido o está sustituido con 1-5 R15 o (s) anillo mono o biheterocíclico de 3-15 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R15, R15 es (a) alquilo C1-8, (b) alquenilo C2-8, (c) alquinilo C2-8, (d) alcoxi C1-4-alquilo (C1-4), (e) átomo de halógeno, (f) CF3, (g) OCF3, (h) ciano, (j) nitro, (k) NR4R5, (l) OR6, (m) SH, (n) S(O)nR7, (o) COR6, (p) COOR6, (q) CONR4R5, (r) NR8COR6, (s) NR8COOR6, (t) NR8CONR4R5, (u) anillo mono o bicarbocíclico C3- que no está sustituido o está sustituido con 1-5 R20, (v) anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R20 o (w) alquilo C1-4 sustituido con 1-2 sustituyentes seleccionados de átomo de halógeno, CF3, OCF3, ciano, nitro, NR4R5, OR6, =N-OR6, SH, S(O)nR7, COR6, COOR6, CONR4R5, NR8COR6, NR8COOR6, NR8CONR4R5, anillo mono o bicarbocíclico C3-10 que no está sustituido o está sustituido con 1-5 R20, y anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R20, R17 es (a) átomo de halógeno, (b) CF3, (c) OCF3, (d) ciano, (e) nitro, (f) NR9R10, (g) OR11a, (h) =N-OR11, (j) SH, (k) S(O)nR12, (l) COR11, (m) COOR11, (n) CONR9R10, (o) NR8COR11, (p) NR8COOR11, (q) NR8CONR9R10, (r) anillo mono o bicarbocíclico C3-15 que no está sustituido o está sustituido con 1-5 R18a o (s) anillo mono o biheterocíclico de 3-15 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) que no está sustituido o está sustituido con 1-5 R18a, R18 es (a) alquilo C1-4, (b) alquenilo C2-4, (c) alquinilo C2-4, (d) átomo de halógeno, (e) CF3, (f) OCF3, (g) ciano, (h) nitro, (j) SH, (k) S(O)nR12, (l) NR9R10, (m) OR11, (n) COR11, (o) COOR11, (p) CONR9R10, (q) anillo carbocíclico C5-6, (r) anillo heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre o (s) alquilo C1-4 sustituido con anillo carbocíclico C5-6 o anillo heterocíclico de 5 ó 6 miembros que contiene 1-2 nitrógeno(s), 1 oxígeno y/o 1 azufre, R18a es (a) alquilo C1-4, (b) alquenilo C2-4, (c) alquinilo C2-4, (d) átomo de halógeno, (e) CF3, (f) OCF3, (g) ciano, (h) nitro, (j) SH, (k) S(O)nR12, (l) NR9R10, (m) OR11a, (n) COR11, (o) COOR11 o (p) CONR9R10, R20 es alquilo C1-4, alcoxilo C1-4, átomo de halógeno, CF3, OCF3, ciano, nitro, amino, NH(alquilo C1-4) o N(alquilo C1-4)2, R3 es (i) anillo mono o bicarbocíclico C5-10 sustituido con 1-5 R16 o (ii) anillo mono o biheterocíclico C5-10 que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) sustituido con 1-5 R16, R16 es (a) alquilo C1-8, (b) alquenilo C2-8, (c) alquinilo C2-8, (d) átomo de halógeno, (e) CF3, (f) OCF3, (g) ciano, (h) nitro, (j) NR9R10, (k) OR11, (l) SH, (m) S(O)nR12, con la excepción de feniltio, (n) COR11, (o) COOR11, (p) CONR9R10, (q) NR8COR11, (r) NR8COOR11, (s) NR8CONR9R10, (t) anillo mono o bicarbocíclico C3-10, (u) anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s) (v) alquilo C1-4 sustituido con 1-2 sustituyentes seleccionados de átomo de halógeno, CF3, OCF3, ciano, nitro, NR9R10, OR11, =N-OR11, SH, S(O)nR12, COR11, COOR11, CONR9R10, NR8COR11, NR8COOR11, NR8CONR9R10, anillo mono o bicarbocíclico C3-10, y anillo mono o biheterocíclico de 3-10 miembros que contiene 1-4 nitrógeno(s), 1-2 oxígeno(s) y/o 1-2 azufre(s), con la condición de que cuando R1 en la fórmula (I-i) es OR6, entonces R3 no es fenilo sustituido con 1 átomo de halógeno, fenilo sustituido con 1 trifluorometilo y fenilo sustituido con trifluorometilo y nitro, una sal farmacéuticamente aceptable del mismo o un hidrato del mismo, con la condición de que el compuesto 8-
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BR0116609A (pt) 2005-02-15
IL156609A0 (en) 2004-01-04
NO20032956D0 (no) 2003-06-26
US7034153B2 (en) 2006-04-25
HUP0303653A2 (hu) 2004-03-01

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