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DK2738191T3 - Amfifilt makromolekyle og anvendelse - Google Patents

Amfifilt makromolekyle og anvendelse Download PDF

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DK2738191T3
DK2738191T3 DK11870106.9T DK11870106T DK2738191T3 DK 2738191 T3 DK2738191 T3 DK 2738191T3 DK 11870106 T DK11870106 T DK 11870106T DK 2738191 T3 DK2738191 T3 DK 2738191T3
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amphiphilic macromolecule
amphiphilic
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Jinben Wang
Xuefeng Shi
Xiaohui Xu
Hui Yang
Yilin Wang
Haike Yan
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Beijing Junlun Runzhong Science&Technology Co Ltd
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    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F232/00Copolymers of cyclic compounds containing no unsaturated aliphatic radicals in a side chain, and having one or more carbon-to-carbon double bonds in a carbocyclic ring system
    • C08F232/02Copolymers of cyclic compounds containing no unsaturated aliphatic radicals in a side chain, and having one or more carbon-to-carbon double bonds in a carbocyclic ring system having no condensed rings
    • C08F232/04Copolymers of cyclic compounds containing no unsaturated aliphatic radicals in a side chain, and having one or more carbon-to-carbon double bonds in a carbocyclic ring system having no condensed rings having one carbon-to-carbon double bond
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    • C04B24/24Macromolecular compounds
    • C04B24/26Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
    • C04B24/2652Nitrogen containing polymers, e.g. polyacrylamides, polyacrylonitriles
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    • C09K8/00Compositions for drilling of boreholes or wells; Compositions for treating boreholes or wells, e.g. for completion or for remedial operations
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    • C09K8/00Compositions for drilling of boreholes or wells; Compositions for treating boreholes or wells, e.g. for completion or for remedial operations
    • C09K8/42Compositions for cementing, e.g. for cementing casings into boreholes; Compositions for plugging, e.g. for killing wells
    • C09K8/46Compositions for cementing, e.g. for cementing casings into boreholes; Compositions for plugging, e.g. for killing wells containing inorganic binders, e.g. Portland cement
    • C09K8/467Compositions for cementing, e.g. for cementing casings into boreholes; Compositions for plugging, e.g. for killing wells containing inorganic binders, e.g. Portland cement containing additives for specific purposes
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    • C09K8/00Compositions for drilling of boreholes or wells; Compositions for treating boreholes or wells, e.g. for completion or for remedial operations
    • C09K8/58Compositions for enhanced recovery methods for obtaining hydrocarbons, i.e. for improving the mobility of the oil, e.g. displacing fluids
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    • C08F220/02Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
    • C08F220/52Amides or imides
    • C08F220/54Amides, e.g. N,N-dimethylacrylamide or N-isopropylacrylamide
    • C08F220/58Amides, e.g. N,N-dimethylacrylamide or N-isopropylacrylamide containing oxygen in addition to the carbonamido oxygen, e.g. N-methylolacrylamide, N-(meth)acryloylmorpholine
    • C08F220/585Amides, e.g. N,N-dimethylacrylamide or N-isopropylacrylamide containing oxygen in addition to the carbonamido oxygen, e.g. N-methylolacrylamide, N-(meth)acryloylmorpholine and containing other heteroatoms, e.g. 2-acrylamido-2-methylpropane sulfonic acid [AMPS]

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Claims (14)

1. Amfifilt makromolekyle, der har, som gentagelsesenheder, en strukturenhed A til justering af molekylvægt, molekylvægtfordeling og ladningskarakteristika, en højt sterisk hindret strukturenhed B og en amfifil strukturenhed C, kendetegnet ved, at den højt sterisk hindrede strukturenhed B indeholder mindst en struktur G, hvor strukturen G er en cyklisk carbonhydridstruktur dannet på basis af to naboliggende carbonatomer i hovedkæden, eller er udvalgt fra en struktur med formel (3), og den højt sterisk hindrede strukturenhed B eventuelt indeholder en struktur med formel (4):
Formel (3) Formel (4) hvor i formel (3), R5 er H eller en methylgruppe; R6 er et radikal udvalgt fra gruppen bestående strukturerne med formel (5) og formel (6),
Formel (5) * Formel (G) hvor i formel (5), a er et helt tal fra 1 til 11, hvor i formel (4), R7 er H eller en methylgruppe; R8 er udvalgt fra gruppen bestående af -NHPhOH, -OCH2Ph, -OPhOH, -OPhCOOH og salte deraf, -NHC(CH3)2CH2S03H og salte deraf, -OC(CH3)2(CH2)bCH3, -NHC(CH3)2(CH2)cCH3, -OC(CH3)2CH2C(CH3)2(CH2)dCH3, -NHC(CH3)2CH2C(CH3)2(CH2)eCH3, -0(CH2)fN+(CH3)2CH2PhX",
hvor b og c er hele tal fra 0 til 21, respektivt; d og e er hele tal fra 0 til 17 respektivt; f er et helt tal fra 2 til 8; og X' er Cl' eller Br\
2. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at strukturenheden A til justering af molekylvægt, molekylvægtfordeling og ladningskarakteristika omfatter en (meth)acrylamid-monomerenhed Ai og/eller en (meth)acrylmono-merenhed A2.
3. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at, den amfifile strukturenhed C har en struktur med formel (8):
Formel (8) hvor i formel (8), R9 er H eller en methylgruppe; Ri0 er -O- eller -NH-; Ru er et radikal indeholdende en ligekædet hydrocarbyl, en forgrenet hydrocarbyl, en polyoxyethylen (PEO), en polyoxypropylen (PPO), en EO-PO-blok, et mo-no-kvaternært ammoniumsalt, et fler-kvaternært ammoniumsalt eller en sul-fonsyre og salte deraf.
4. Amfifilt makromolekyle ifølge krav 2, kendetegnet ved, at, baseret på 100 mol-% af alle gentagelsesenhederne af det amfifile makromolekyle, molprocentdelen af (meth)acrylamidmonomer-enheden A-ι er 70-99 mol-%; og molprocentdelen af (meth)acrylmonomer-enheden A2 er 1-30 mol-%.
5. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at, baseret på 100 mol-% af alle gentagelsesenhederne af det amfifile makromolekyle, molpro centdelen af strukturen G er 0,02-2 mol-%; og molprocentdelen af strukturen med formel (4) er 0,05-5 mol-%.
6. Amfifilt makromolekyle ifølge krav 3, kendetegnet ved, at, baseret på 100 mol-% af alle gentagelsesenhederne af det amfifile makromolekyle, molprocentdelen af strukturen med formel (8) er 0,05-10 mol-%.
7. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at strukturenheden A til justering af molekylvægt, molekylvægtfordeling og ladningskarakteristika har en struktur med formel (2);
Formel (2) hvor, i formel (2), R-ι er H eller en methylgruppe; R2 og R3 uafhængigt er valgt fra gruppen bestående af H og en CrC3-alkylgruppe; R4 er valgt fra gruppen bestående af H og en methylgruppe; Gr er -OH eller -0-Na+; m og n betegner molprocentdelene af strukturenhederne i hele det amfifile makromolekyle, og m er fra 70 til 99 mol-%; n er fra 1 til 30 mol-%.
8. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at den cykliske carbonhydridstruktur, der er dannet på basis af to naboliggende carbonato-mer i hovedkæden, er udvalgt fra gruppen bestående af:
9. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at den højt sterisk hindrede strukturenhed B har en struktur med formel (7):
Formel 17) hvor, i formel (7), definitionen på G er som beskrevet i krav 3; definitionerne på R7 og R8 er beskrevet i formel (4); henholdsvis x og y betegner molprocentdelene af strukturenhederne i hele det amfifile makromolekyle, og x er fra 0,02 til 2 mol-%, y er fra 0,05 til 5 mol-%.
10. Amfifilt makromolekyle ifølge krav 3, kendetegnet ved, at strukturen bestående af R-io og Ru kan være udvalgt fra gruppen bestående af -0(CH2)gN+(CH3)2(CH2)hCH3X\ -NH(CH2)iN+(CH3)2(CH2)jCH3X-, -0(CH2)kN+((CH2)pCH3)3X', -0(CH2)qN+(CH3)2(CH2)aCH(S03H)CH2(E0)3(P0)Y(CH2)5CH3X', -NH(CH2)qN+(CH3)2(CH2)aCH(S03H)CH2(E0)p(P0)Y(CH2)5CH3X·, -0(CH2)qN+(CH3)2(CH2)aCH(C00H)CH2(E0)p(P0)Y(CH2)5CH3X', -NH(CH2)qN+(CH3)2(CH2)aCH(COOH)CH2(EO)p(PO)Y(CH2)5CH3X', -0(CH2)2N+(CH3)2(CH2)ES03\ -(OCH(CH2N+(CH3)2(CH2^CH3Cr)CH2)nO(CH2)eCH3, -(0CH(CH2N+((CH2)ACH3)3Cr)CH2)T0(CH2)KCH3, -OCH(CH2N+(CH3)2(CH2)rCH3X'))2, -OCH(CH2N+((CH2)sCH3)3X'))2; hvor g, i, k og q respektivt er hele tal fra 1 til 6; h og j respektivt er hele tal fra 3 til 21; p er et helt tal fra 3 til 9; α er et helt tal fra 1 til 12; β og γ respektivt er hele tal fra 0 til 40; δ er et helt tal fra 0 til 21; ε er et helt tal fra 4 til 18; ζ er et helt tal fra 1 til 21; η og τ respektivt er hele tal fra 1 til 30; Θ og κ respektivt er hele tal fra 3 til 21; λ er et helt tal fra 0 til 9; r er et helt tal fra 3 til 21; s er et helt tal fra 3 til 9; og X' er Cl' eller Br\
11. Amfifilt makromolekyle ifølge krav 1, kendetegnet ved, at det amfifile makromolekyle har en struktur med formel (9):
Formel (9) hvor, i formel (9), FU er valgt fra gruppen bestående af H og en methylgrup-pe; m og n betegner molprocentdelene af strukturenhederne i hele det amfifi-le makromolekyle, og m er fra 70 til 99 mol-%; n er fra 1 til 30 mol-%; definitionerne på G, R7, R8j x og y er som beskrevet i formel (7); R9 er H eller en methylgruppe, R-|0 er -O- eller -NH-; R11 er et radikal, der indeholder et lige-kædet hydrocarbyl, et forgrenet hydrocarbyl, en polyoxyethylen (PEO), en polyoxypropylen (PPO), en EO-PO-blok, et mono-kvaternært ammoniumsalt, et fler-kvaternært ammoniumsalt eller en sulfonsyre og salte deraf; z betegner molprocentdelen af strukturenheden i hele det amfifile makromolekyle, og z er fra 0,05 til 10 mol-%.
12. Amfifilt makromolekyle ifølge krav 1, som er en forbindelse med formlerne (l)-(X):
(i) (IV) (VII)
(X)
13. Amfifilt makromolekyle ifølge et af kravene 1 til 12, kendetegnet ved, at det har en molekylvægt på mellem 1000000-20000000.
14. Anvendelse af det amfifile makromolekyle ifølge et af kravene 1 til 13 ved oliefeltboring, brønd-cementering, frakturering, opsamling og transport af råolie, spildevandsbehandling, slambehandling og papirfremstilling som forstærket olieproduktionsmiddel og oliefortrængningsmiddel, middel til reduktion af viskositeten af tung olie, fraktureringsfluid, lerstabilisator, spildevands-behandlingsmiddel, fastholdelseshjælpemiddel og afvandingshjælpemiddel og forstærkningsmiddel til papirfremstilling.
DK11870106.9T 2011-07-26 2011-09-16 Amfifilt makromolekyle og anvendelse DK2738191T3 (da)

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CN111363073A (zh) * 2019-11-14 2020-07-03 中国科学院化学研究所 一种兼具防膨和絮凝作用的两亲聚合物及其制备方法与应用
CN114426832A (zh) * 2020-10-15 2022-05-03 中国石油化工股份有限公司 一种边底水稠油油藏控水降粘剂的控水降粘方法
CN114456793B (zh) * 2020-10-21 2023-06-20 中国石油化工股份有限公司 一种针对低渗透稠油油藏的自降粘压裂液及其制备方法
CN114478906B (zh) 2020-10-26 2023-05-02 中国石油化工股份有限公司 一种聚丙烯酰胺基对称支化聚合物型表面活性剂及其制备方法和应用

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MY179433A (en) 2020-11-06
ES2641320T3 (es) 2017-11-08
EP2738191A1 (en) 2014-06-04
EA026294B1 (ru) 2017-03-31
WO2013013355A1 (zh) 2013-01-31
EP2738191A4 (en) 2015-08-12
NO2738191T3 (da) 2018-01-06
US20140350204A1 (en) 2014-11-27

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