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CN111455337A - Single-side conductive copper-plated PI film and preparation method thereof - Google Patents

Single-side conductive copper-plated PI film and preparation method thereof Download PDF

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Publication number
CN111455337A
CN111455337A CN202010363610.3A CN202010363610A CN111455337A CN 111455337 A CN111455337 A CN 111455337A CN 202010363610 A CN202010363610 A CN 202010363610A CN 111455337 A CN111455337 A CN 111455337A
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film
plated
copper alloy
copper
conductive copper
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刘稳
王荣福
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Shenzhen Hanyu New Material Technology Co ltd
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Shenzhen Hanyu New Material Technology Co ltd
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    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C14/00Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material
    • C23C14/22Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material characterised by the process of coating
    • C23C14/34Sputtering
    • C23C14/35Sputtering by application of a magnetic field, e.g. magnetron sputtering
    • CCHEMISTRY; METALLURGY
    • C22METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
    • C22CALLOYS
    • C22C9/00Alloys based on copper
    • C22C9/01Alloys based on copper with aluminium as the next major constituent
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C14/00Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material
    • C23C14/06Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material characterised by the coating material
    • C23C14/14Metallic material, boron or silicon
    • C23C14/16Metallic material, boron or silicon on metallic substrates or on substrates of boron or silicon
    • C23C14/165Metallic material, boron or silicon on metallic substrates or on substrates of boron or silicon by cathodic sputtering
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C14/00Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material
    • C23C14/06Coating by vacuum evaporation, by sputtering or by ion implantation of the coating forming material characterised by the coating material
    • C23C14/14Metallic material, boron or silicon
    • C23C14/20Metallic material, boron or silicon on organic substrates
    • C23C14/205Metallic material, boron or silicon on organic substrates by cathodic sputtering

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Shielding Devices Or Components To Electric Or Magnetic Fields (AREA)
  • Physical Vapour Deposition (AREA)

Abstract

The invention belongs to the technical field of electromagnetic shielding materials, and particularly relates to a single-side conductive copper-plated PI film and a preparation method thereof, wherein the preparation method comprises the following steps: step 1, plating chromium metal on a PI film by a magnetron sputtering method; step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method; and 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain the single-side conductive copper-plated PI film. The invention has the beneficial effects that: the single-side conductive copper-plated PI film obtained by the invention has stronger corrosion resistance and good mechanical property. Under the condition of 50MHZ-1.5GHZ, the shielding effectiveness reaches 80-130 dB. The single-side conductive copper-plated PI film is thin and low in density, does not obviously increase the overall weight of an electronic product, and reduces occupied space.

Description

Single-side conductive copper-plated PI film and preparation method thereof
Technical Field
The invention belongs to the technical field of electromagnetic shielding materials, and particularly relates to a single-side conductive copper-plated PI film and a preparation method thereof.
Background
With the development of technology, electronic products are required to be lighter in the market, so that the integration level of various integrated chips is higher. When a large number of various chips are operated, a certain amount of electromagnetic radiation is generated outwards. The electromagnetic radiation can generate interference to external electromagnetic signals and influence the use of other products for transmitting signals or receiving signals,
the following methods are generally known in the art: 1. for example, in the power adapter of the notebook computer, the inside of the power adapter is firstly wrapped by an insulating sheet and then wrapped by an aluminum foil, and the aluminum foil plays a role in shielding. The insulating sheet and the aluminum foil are manually or mechanically arranged, so that the process is complicated, and the insulating property is unreliable. 2. The chip or the whole circuit board is covered by the metal shielding cover, and when electromagnetic waves encounter conductive metal, the electromagnetic waves can be reflected back, so that the electromagnetic wave shielding effect is achieved. The method has the following defects: a. the metal shielding case has higher density, so that the weight of the electronic product is obviously increased; b. the metal shield is conductive and the shield needs to be spaced a distance from the chip so that the shield occupies a large space.
Disclosure of Invention
The technical problem to be solved by the invention is as follows: the single-side conductive copper-plated PI film is insulating, light in weight and good in electromagnetic shielding effect, and the preparation method thereof.
In order to solve the technical problems, the invention adopts the technical scheme that: the preparation method of the single-side conductive copper-plated PI film comprises the following steps:
step 1, plating chromium metal on a PI film by a magnetron sputtering method to obtain a first PI film with a chromium support layer;
step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method to obtain a second PI film with a copper alloy shielding layer;
the copper alloy target comprises the following components in percentage by weight: 0.2-0.6% of Cr, 1-3% of Al, 0.5-1% of Mn and the balance of Cu;
and 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain the single-side conductive copper-plated PI film.
The other technical scheme of the invention is as follows: the single-side conductive copper-plated PI film prepared by the preparation method is provided.
The invention has the beneficial effects that: the single-sided conductive copper-plated PI film can be used for a power adapter of a notebook computer, the PI film layer is insulated and can replace an insulating sheet to achieve an insulating effect, one side of the PI film in the single-sided conductive copper-plated PI film can be attached to a short distance or a close chip, occupied space is reduced, a plurality of metal shielding layers on the PI film can replace aluminum foil to achieve a better electromagnetic shielding effect, and the shielding efficiency can reach 80-115dB under the condition of 50MHZ-1.5 GHZ. The single-side conductive copper-plated PI film is thin and low in density, and the weight of the whole electronic product such as a notebook computer power adapter is not obviously increased (the thickness of the metal shielding layer is generally more than 100 mu m). At the same time. The metal shielding layer shielding shell replaces a copper foil coil, so that the metal shielding layer shielding shell has strong corrosion resistance and protection capability, cannot deform or break, and has good reliability.
Detailed Description
In order to explain the technical content, the objects and the effects of the present invention in detail, the following description will be given with reference to the embodiments.
The invention provides a preparation method of a single-side conductive copper-plated PI film, which comprises the following steps:
step 1, plating chromium metal on a PI film by a magnetron sputtering method to obtain a first PI film with a chromium support layer;
step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method to obtain a second PI film with a copper alloy shielding layer;
the copper alloy target comprises the following components in percentage by weight: 0.2-0.6% of Cr, 1-3% of Al, 0.5-1% of Mn and the balance of Cu;
and 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain the single-side conductive copper-plated PI film.
In the single-sided conductive copper-plated PI film and the preparation method thereof, three plating layers with different functions are arranged on the single-sided conductive copper-plated PI film and sequentially comprise a chromium supporting layer, a copper alloy shielding layer and a nickel metal layer. It has the following functions: 1. chromium is doped in the copper alloy shielding layer to improve the strength and conductivity of the copper alloy, Mn is doped to improve the oxidation resistance, and aluminum is also doped in the copper alloy shielding layer to ensure that the copper alloy shielding layer is stable, uniform and free from coagulation when being sputtered to the chromium supporting layer by magnetron sputtering. 2. The nickel metal layer has good corrosion resistance and protects the copper alloy shielding layer from being oxidized and damaged. 3. The chromium support layer provides sufficient bonding strength and hardness support for the copper alloy shielding layer, so that the bonding force between the copper alloy shielding layer and the PI film is increased. The electromagnetic shielding capability of the chromium supporting layer is also stronger than that of the copper alloy shielding layer, so that the electromagnetic shielding capability of the single-side conductive copper-plated PI film is further improved.
Preferably, in the above method for preparing a single-sided conductive copper-plated PI film, the thickness of the PI film is 25 to 75 μm, the thickness of the chromium support layer is 0.1 to 1 μm, the thickness of the copper alloy shielding layer is 2 to 8 μm, and the thickness of the nickel plated second PI film is 0.2 to 0.6 μm.
Preferably, in the above method for preparing a single-sided conductive copper-plated PI film, the method for preparing the copper alloy target material is:
the raw materials of Cr, Al, Mn and Cu are smelted and alloyed by an induction smelting method in a vacuum atmosphere at the temperature of 1100-1200 ℃, and then the alloyed molten liquid is cast into a casting mould to obtain the copper alloy target.
Preferably, in the above method for preparing a single-sided conductive copper-plated PI film, the thickness of the PI film is 30 μm, the thickness of the chromium support layer is 0.5 μm, the thickness of the copper alloy shielding layer is 5 μm, and the thickness of the nickel plated layer to the second PI film is 0.3 μm.
Preferably, in the above method for preparing a single-sided conductive copper-plated PI film, the copper alloy target material comprises, by weight: 0.3% of Cr, 1.5% of Al, 0.7% of Mn and the balance of Cu.
Preferably, in the above method for preparing a single-sided conductive copper-plated PI film, a circulating water cooling device is provided on the copper alloy target.
Example one
A preparation method of a single-side conductive copper-plated PI film comprises the following steps:
step 1, plating chromium metal on a PI film by a magnetron sputtering method to obtain a first PI film with a chromium support layer;
step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method to obtain a second PI film with a copper alloy shielding layer;
the preparation method of the copper alloy target comprises the following steps: preparing Cr, Al, Mn and Cu raw materials, then smelting and alloying at the temperature of 1100-1200 ℃ in a vacuum atmosphere by using an induction smelting method, and then casting the alloyed molten liquid into a casting mold to obtain the copper alloy target.
The copper alloy target comprises the following components in percentage by weight: 0.2% of Cr, 1% of Al, 0.5% of Mn and the balance of Cu;
and 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain the single-side conductive copper-plated PI film.
The thickness of the PI film is 25-75 μm, the thickness of the chromium supporting layer is 0.1-1 μm, the thickness of the copper alloy shielding layer is 2-8 μm, and the thickness of the nickel plated to the second PI film is 0.2-0.6 μm.
Example two
A preparation method of a single-side conductive copper-plated PI film comprises the following steps:
step 1, plating chromium metal on a PI film by a magnetron sputtering method to obtain a first PI film with a chromium support layer;
step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method to obtain a second PI film with a copper alloy shielding layer;
the preparation method of the copper alloy target comprises the following steps: preparing Cr, Al, Mn and Cu raw materials, then smelting and alloying at the temperature of 1100-1200 ℃ in a vacuum atmosphere by using an induction smelting method, and then casting the alloyed molten liquid into a casting mold to obtain the copper alloy target.
The copper alloy target comprises the following components in percentage by weight: 0.6% of Cr, 3% of Al, 1% of Mn and the balance of Cu;
step 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain a single-side conductive copper-plated PI film;
the thickness of the PI film is 25-75 μm, the thickness of the chromium supporting layer is 0.1-1 μm, the thickness of the copper alloy shielding layer is 2-8 μm, and the thickness of the nickel plated to the second PI film is 0.2-0.6 μm.
EXAMPLE III
A preparation method of a single-side conductive copper-plated PI film comprises the following steps:
step 1, plating chromium metal on a PI film by a magnetron sputtering method to obtain a first PI film with a chromium support layer;
step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method to obtain a second PI film with a copper alloy shielding layer;
the preparation method of the copper alloy target comprises the following steps: preparing Cr, Al, Mn and Cu raw materials, then smelting and alloying at the temperature of 1100-1200 ℃ in a vacuum atmosphere by using an induction smelting method, and then casting the alloyed molten liquid into a casting mold to obtain the copper alloy target.
The copper alloy target comprises the following components in percentage by weight: 0.3% of Cr, 1.5% of Al, 0.7% of Mn and the balance of Cu;
and 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain the single-side conductive copper-plated PI film.
The thickness of the PI film is 25-75 μm, the thickness of the chromium supporting layer is 0.1-1 μm, the thickness of the copper alloy shielding layer is 2-8 μm, and the thickness of the nickel plated to the second PI film is 0.2-0.6 μm.
The magnetron sputtering of chromium metal, copper alloy and nickel metal of the above examples was carried out under vacuum at a degree of vacuum of 10- 3From MPa to 10-5MPa. And unwinding and winding the PI film in a vacuum chamber. And sputtering and coating while rolling. The speed is 2-10 m/min. Each magnetron sputtering is implemented by installing 2-50 magnetron sputtering of each metal, heating the target materials in an ion beam mode, and adding a cooling device (circulating water cooling) behind each target material, so that the temperature of the whole coating environment is low, and the device is protected and can be produced in batches in a coiling manner.
The technological parameters are as follows: the power of the target power supply is set to be 30-40kw, argon is used as the working gas, the flow rate of the argon is 200-.
The single-sided conductive copper-plated PI film prepared by the preparation method of the single-sided conductive copper-plated PI film is subjected to mechanical property test on an electronic universal tester, and the tensile strength of the single-sided conductive copper-plated PI film is 110-160N/mm2(ii) a Yield strength of 120-150N/mm2Excellent impact resistance and reliability; the bonding strength reaches 3.5N/cm2In the above way, the plated metal film layer can obtain excellent shielding effect under a lower thickness; and compared with other copper plating methods, the method reduces pollution and is more environment-friendly. The electromagnetic shielding resistance of the single-sided conductive copper-plated PI film is 70-115dB (the working frequency is 50MHz-1 GHz). It has strong corrosion resistance and good mechanical property. The electromagnetic shielding and protection device can be used for electromagnetic shielding and protection of the notebook computer power adapter.
Test examples
Under the condition of the same other parameters, samples 1 to 4 were prepared according to the method for preparing the single-sided conductive copper-plated PI film described in the third example, and the product performance test results are shown in table 1.
TABLE 1
Figure BDA0002475831250000061
From the above description, in the preparation method of the single-sided conductive copper-plated PI film, when the thickness of the PI film is 30 μm, the thickness of the chromium supporting layer is 0.5 μm, the thickness of the copper alloy shielding layer is 5 μm, and the thickness of the nickel plated on the second PI film is 0.3 μm, the electromagnetic shielding performance of the single-sided conductive copper-plated PI film reaches 120dB, and the tensile strength is 550N/mm2At the moment, the single-side conductive copper-plated PI film is thin in thickness, low in cost and highest in cost performance. The electromagnetic shielding and protection device is most suitable for electromagnetic shielding and protection of the notebook computer power adapter.
The above description is only an embodiment of the present invention, and not intended to limit the scope of the present invention, and all equivalent modifications made by the present invention in the specification or directly or indirectly applied to the related technical field are included in the scope of the present invention.

Claims (7)

1. A preparation method of a single-side conductive copper-plated PI film is characterized by comprising the following steps:
step 1, plating chromium metal on a PI film by a magnetron sputtering method to obtain a first PI film with a chromium support layer;
step 2, plating the copper alloy on the copper alloy target material on a chromium supporting layer of the first PI film by a magnetron sputtering method to obtain a second PI film with a copper alloy shielding layer;
the copper alloy target comprises the following components in percentage by weight: 0.2-0.6% of Cr, 1-3% of Al, 0.5-1% of Mn and the balance of Cu;
and 3, plating nickel metal on the copper alloy shielding layer of the second PI film by a magnetron sputtering method to obtain the single-side conductive copper-plated PI film.
2. The method for preparing the single-sided conductive copper-plated PI film according to claim 1, wherein the thickness of the PI film is 25-75 μm, the thickness of the chromium support layer is 0.1-1 μm, the thickness of the copper alloy shielding layer is 2-8 μm, and the thickness of the nickel plated second PI film is 0.2-0.6 μm.
3. The method for preparing the single-sided conductive copper-plated PI film according to claim 1, wherein the method for preparing the copper alloy target comprises the following steps:
the raw materials of Cr, Al, Mn and Cu are smelted and alloyed by an induction smelting method in a vacuum atmosphere at the temperature of 1100-1200 ℃, and then the alloyed molten liquid is cast into a casting mould to obtain the copper alloy target.
4. The method for preparing the single-sided conductive copper-plated PI film according to claim 1, wherein the PI film has a thickness of 30 μm, the chromium support layer has a thickness of 0.5 μm, the copper alloy shielding layer has a thickness of 5 μm, and the nickel plating to the second PI film has a thickness of 0.3 μm.
5. The method for preparing the single-sided conductive copper-plated PI film according to claim 1, wherein the copper alloy target comprises the following components in percentage by weight: 0.3% of Cr, 1.5% of Al, 0.7% of Mn and the balance of Cu.
6. The method for preparing the single-sided conductive copper-plated PI film according to claim 1, wherein a circulating water cooling device is arranged on the copper alloy target.
7. The single-sided conductive copper-plated PI film prepared by the preparation method of the single-sided conductive copper-plated PI film as claimed in any one of claims 1 to 6.
CN202010363610.3A 2020-04-30 2020-04-30 Single-side conductive copper-plated PI film and preparation method thereof Pending CN111455337A (en)

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Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN114075655A (en) * 2020-08-22 2022-02-22 昆山鑫美源电子科技有限公司 Conductive film, preparation method of conductive film, current collection and transmission material and energy storage device
CN116024535A (en) * 2023-03-28 2023-04-28 苏州浪潮智能科技有限公司 Method and equipment for preparing radiation film, radiation film and optical device

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KR20020075643A (en) * 2001-03-27 2002-10-05 임조섭 Method for forming of the EMI protecting layer on a plastic substrate and an EMI protecting layer thereof
CN1818130A (en) * 2006-03-20 2006-08-16 浙江大学 Production of dual electromagnetic shielding screen by sputtering method
CN107109633A (en) * 2015-05-21 2017-08-29 捷客斯金属株式会社 Copper alloy sputtering target and its manufacture method
CN109306459A (en) * 2017-07-28 2019-02-05 苏州思锐达新材料有限公司 Two-sided conductive electromagnetic shielding material of a kind of high temperature resistant and the preparation method and application thereof
CN109306487A (en) * 2017-07-28 2019-02-05 苏州思锐达新材料有限公司 Electromagnetic shielding material and the preparation method and application thereof based on Kapton

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Publication number Priority date Publication date Assignee Title
KR20020075643A (en) * 2001-03-27 2002-10-05 임조섭 Method for forming of the EMI protecting layer on a plastic substrate and an EMI protecting layer thereof
CN1818130A (en) * 2006-03-20 2006-08-16 浙江大学 Production of dual electromagnetic shielding screen by sputtering method
CN107109633A (en) * 2015-05-21 2017-08-29 捷客斯金属株式会社 Copper alloy sputtering target and its manufacture method
CN109306459A (en) * 2017-07-28 2019-02-05 苏州思锐达新材料有限公司 Two-sided conductive electromagnetic shielding material of a kind of high temperature resistant and the preparation method and application thereof
CN109306487A (en) * 2017-07-28 2019-02-05 苏州思锐达新材料有限公司 Electromagnetic shielding material and the preparation method and application thereof based on Kapton

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN114075655A (en) * 2020-08-22 2022-02-22 昆山鑫美源电子科技有限公司 Conductive film, preparation method of conductive film, current collection and transmission material and energy storage device
CN114075655B (en) * 2020-08-22 2024-01-12 昆山鑫美源电子科技有限公司 Conductive film, method for producing conductive film, current collecting and transmitting material, and energy storage device
CN116024535A (en) * 2023-03-28 2023-04-28 苏州浪潮智能科技有限公司 Method and equipment for preparing radiation film, radiation film and optical device

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