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WO2011112042A3 - 유기고분자-규소 복합체 입자 및 그 제조방법과 이를 포함하는 음극 및 리튬 이차전지 - Google Patents

유기고분자-규소 복합체 입자 및 그 제조방법과 이를 포함하는 음극 및 리튬 이차전지 Download PDF

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Publication number
WO2011112042A3
WO2011112042A3 PCT/KR2011/001725 KR2011001725W WO2011112042A3 WO 2011112042 A3 WO2011112042 A3 WO 2011112042A3 KR 2011001725 W KR2011001725 W KR 2011001725W WO 2011112042 A3 WO2011112042 A3 WO 2011112042A3
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WIPO (PCT)
Prior art keywords
silicon
preparation
same
cathode
secondary battery
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Ceased
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PCT/KR2011/001725
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English (en)
French (fr)
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WO2011112042A2 (ko
Inventor
황선정
신동석
권윤경
정근창
최정석
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LG Chem Ltd
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LG Chem Ltd
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Publication date
Application filed by LG Chem Ltd filed Critical LG Chem Ltd
Priority to EP11753647.4A priority Critical patent/EP2546908B1/en
Priority to CN201180013510.7A priority patent/CN102792498B/zh
Priority to JP2012556989A priority patent/JP5712439B2/ja
Priority to US13/180,007 priority patent/US9142859B2/en
Publication of WO2011112042A2 publication Critical patent/WO2011112042A2/ko
Publication of WO2011112042A3 publication Critical patent/WO2011112042A3/ko
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

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    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01B—CABLES; CONDUCTORS; INSULATORS; SELECTION OF MATERIALS FOR THEIR CONDUCTIVE, INSULATING OR DIELECTRIC PROPERTIES
    • H01B1/00—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors
    • H01B1/20—Conductive material dispersed in non-conductive organic material
    • H01B1/24—Conductive material dispersed in non-conductive organic material the conductive material comprising carbon-silicon compounds, carbon or silicon
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H01M10/0525—Rocking-chair batteries, i.e. batteries with lithium insertion or intercalation in both electrodes; Lithium-ion batteries
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/60—Selection of substances as active materials, active masses, active liquids of organic compounds
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00—Secondary cells; Manufacture thereof
    • H01M10/05—Accumulators with non-aqueous electrolyte
    • H01M10/052—Li-accumulators
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/134—Electrodes based on metals, Si or alloys
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/13—Electrodes for accumulators with non-aqueous electrolyte, e.g. for lithium-accumulators; Processes of manufacture thereof
    • H01M4/139—Processes of manufacture
    • H01M4/1395—Processes of manufacture of electrodes based on metals, Si or alloys
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/362—Composites
    • H01M4/366—Composites as layered products
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/38—Selection of substances as active materials, active masses, active liquids of elements or alloys
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/36—Selection of substances as active materials, active masses, active liquids
    • H01M4/38—Selection of substances as active materials, active masses, active liquids of elements or alloys
    • H01M4/386—Silicon or alloys based on silicon
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/624—Electric conductive fillers
    • H01M4/625—Carbon or graphite
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/628—Inhibitors, e.g. gassing inhibitors, corrosion inhibitors
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/02—Electrodes composed of, or comprising, active material
    • H01M4/62—Selection of inactive substances as ingredients for active masses, e.g. binders, fillers
    • H01M4/624—Electric conductive fillers
    • H01M4/626—Metals
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10—Energy storage using batteries
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Composite Materials (AREA)
  • Manufacturing & Machinery (AREA)
  • Physics & Mathematics (AREA)
  • Dispersion Chemistry (AREA)
  • Spectroscopy & Molecular Physics (AREA)
  • Battery Electrode And Active Subsutance (AREA)

Abstract

본 발명은 고에너지 밀도를 나타내는 규소를 이용한 유기고분자-규소 복합체 입자 및 이를 제조하는 방법과 이를 포함하는 음극 및 리튬 이차전지에 대한 것으로, 고에너지 밀도의 규소를 음극 활물질 재료로 이용하여 용량이 높은 리튬 이차 전지를 제공하고 전기 전도성이 상대적으로 낮다는 문제점을 해결하는 방안으로 표면에 금속이 소정량 도금되어 있는 구조의 규소-고분자 복합체 입자 및 그의 제조방법을 제시하여 전기 전도도가 개선된 전극을 제공한다. 또한, 입자 표면에 무전해 도금 방법에 의해 금속을 소정량 피복시킨 규소-고분자 복합체 입자를 제조하고 이를 이용하여 전극을 구성함을 통해, 규소 활물질의 현저한 부피 변화로 인한 열화 문제 및 규소 입자를 전극 활물질로 사용할 때의 낮은 전기 전도도 문제를 해결한다.
PCT/KR2011/001725 2010-03-11 2011-03-11 유기고분자-규소 복합체 입자 및 그 제조방법과 이를 포함하는 음극 및 리튬 이차전지 Ceased WO2011112042A2 (ko)

Priority Applications (4)

Application Number Priority Date Filing Date Title
EP11753647.4A EP2546908B1 (en) 2010-03-11 2011-03-11 Organic polymer-silicon composite particle, preparation method for same, and cathode and lithium secondary battery including same
CN201180013510.7A CN102792498B (zh) 2010-03-11 2011-03-11 聚合物-硅复合粒子、其制备方法以及包含所述聚合物-硅复合粒子的负极和锂二次电池
JP2012556989A JP5712439B2 (ja) 2010-03-11 2011-03-11 有機高分子−ケイ素複合体粒子及びその製造方法とそれを含む負極及びリチウム二次電池
US13/180,007 US9142859B2 (en) 2010-03-11 2011-07-11 Polymer-silicon composite particles, method of making the same, and anode and lithium secondary battery including the same

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
KR10-2010-0021762 2010-03-11
KR20100021762 2010-03-11

Related Child Applications (1)

Application Number Title Priority Date Filing Date
US13/180,007 Continuation US9142859B2 (en) 2010-03-11 2011-07-11 Polymer-silicon composite particles, method of making the same, and anode and lithium secondary battery including the same

Publications (2)

Publication Number Publication Date
WO2011112042A2 WO2011112042A2 (ko) 2011-09-15
WO2011112042A3 true WO2011112042A3 (ko) 2012-03-01

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PCT/KR2011/001725 Ceased WO2011112042A2 (ko) 2010-03-11 2011-03-11 유기고분자-규소 복합체 입자 및 그 제조방법과 이를 포함하는 음극 및 리튬 이차전지

Country Status (6)

Country Link
US (1) US9142859B2 (ko)
EP (1) EP2546908B1 (ko)
JP (1) JP5712439B2 (ko)
KR (1) KR101252932B1 (ko)
CN (1) CN102792498B (ko)
WO (1) WO2011112042A2 (ko)

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EP2546908B1 (en) 2016-06-15
US20120007028A1 (en) 2012-01-12
WO2011112042A2 (ko) 2011-09-15
KR20110102844A (ko) 2011-09-19
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