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WO2008070931A1 - Appareil de combustion - Google Patents

Appareil de combustion Download PDF

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Publication number
WO2008070931A1
WO2008070931A1 PCT/AU2007/001938 AU2007001938W WO2008070931A1 WO 2008070931 A1 WO2008070931 A1 WO 2008070931A1 AU 2007001938 W AU2007001938 W AU 2007001938W WO 2008070931 A1 WO2008070931 A1 WO 2008070931A1
Authority
WO
WIPO (PCT)
Prior art keywords
combustion
gas
media
coal
kiln
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/AU2007/001938
Other languages
English (en)
Inventor
Patrick Joseph Glynn
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Eestech Inc Australia
Original Assignee
Eestech Inc Australia
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Priority claimed from AU2006907028A external-priority patent/AU2006907028A0/en
Application filed by Eestech Inc Australia filed Critical Eestech Inc Australia
Priority to US12/528,361 priority Critical patent/US20110059410A1/en
Priority to CN200780051161.1A priority patent/CN101631845B/zh
Priority to AU2007332089A priority patent/AU2007332089B2/en
Priority to EA200900840A priority patent/EA200900840A1/ru
Publication of WO2008070931A1 publication Critical patent/WO2008070931A1/fr
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

Links

Classifications

    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F02—COMBUSTION ENGINES; HOT-GAS OR COMBUSTION-PRODUCT ENGINE PLANTS
    • F02C—GAS-TURBINE PLANTS; AIR INTAKES FOR JET-PROPULSION PLANTS; CONTROLLING FUEL SUPPLY IN AIR-BREATHING JET-PROPULSION PLANTS
    • F02C3/00—Gas-turbine plants characterised by the use of combustion products as the working fluid
    • F02C3/20—Gas-turbine plants characterised by the use of combustion products as the working fluid using a special fuel, oxidant, or dilution fluid to generate the combustion products
    • F02C3/22—Gas-turbine plants characterised by the use of combustion products as the working fluid using a special fuel, oxidant, or dilution fluid to generate the combustion products the fuel or oxidant being gaseous at standard temperature and pressure
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F02—COMBUSTION ENGINES; HOT-GAS OR COMBUSTION-PRODUCT ENGINE PLANTS
    • F02C—GAS-TURBINE PLANTS; AIR INTAKES FOR JET-PROPULSION PLANTS; CONTROLLING FUEL SUPPLY IN AIR-BREATHING JET-PROPULSION PLANTS
    • F02C3/00—Gas-turbine plants characterised by the use of combustion products as the working fluid
    • F02C3/20—Gas-turbine plants characterised by the use of combustion products as the working fluid using a special fuel, oxidant, or dilution fluid to generate the combustion products
    • F02C3/26—Gas-turbine plants characterised by the use of combustion products as the working fluid using a special fuel, oxidant, or dilution fluid to generate the combustion products the fuel or oxidant being solid or pulverulent, e.g. in slurry or suspension
    • F02C3/28—Gas-turbine plants characterised by the use of combustion products as the working fluid using a special fuel, oxidant, or dilution fluid to generate the combustion products the fuel or oxidant being solid or pulverulent, e.g. in slurry or suspension using a separate gas producer for gasifying the fuel before combustion
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F02—COMBUSTION ENGINES; HOT-GAS OR COMBUSTION-PRODUCT ENGINE PLANTS
    • F02C—GAS-TURBINE PLANTS; AIR INTAKES FOR JET-PROPULSION PLANTS; CONTROLLING FUEL SUPPLY IN AIR-BREATHING JET-PROPULSION PLANTS
    • F02C6/00—Plural gas-turbine plants; Combinations of gas-turbine plants with other apparatus; Adaptations of gas-turbine plants for special use
    • F02C6/18—Plural gas-turbine plants; Combinations of gas-turbine plants with other apparatus; Adaptations of gas-turbine plants for special use using the waste heat of gas-turbine plants outside the plants themselves, e.g. gas-turbine power heat plants
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F23—COMBUSTION APPARATUS; COMBUSTION PROCESSES
    • F23G—CREMATION FURNACES; CONSUMING WASTE PRODUCTS BY COMBUSTION
    • F23G5/00—Incineration of waste; Incinerator constructions; Details, accessories or control therefor
    • F23G5/20—Incineration of waste; Incinerator constructions; Details, accessories or control therefor having rotating or oscillating drums
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F23—COMBUSTION APPARATUS; COMBUSTION PROCESSES
    • F23G—CREMATION FURNACES; CONSUMING WASTE PRODUCTS BY COMBUSTION
    • F23G5/00—Incineration of waste; Incinerator constructions; Details, accessories or control therefor
    • F23G5/44—Details; Accessories
    • F23G5/46—Recuperation of heat
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F23—COMBUSTION APPARATUS; COMBUSTION PROCESSES
    • F23G—CREMATION FURNACES; CONSUMING WASTE PRODUCTS BY COMBUSTION
    • F23G7/00—Incinerators or other apparatus for consuming industrial waste, e.g. chemicals
    • F23G7/06—Incinerators or other apparatus for consuming industrial waste, e.g. chemicals of waste gases or noxious gases, e.g. exhaust gases
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02T—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO TRANSPORTATION
    • Y02T50/00—Aeronautics or air transport
    • Y02T50/60—Efficient propulsion technologies, e.g. for aircraft

Definitions

  • THIS INVENTION relates to a combustion apparatus for combusting fuel media and in particular but not limited thereto a thermodynamic system having a combustion apparatus for combusting one or more relatively low grade fuel media, and a thermodynamic apparatus adapted to receive heat energy from the combustion apparatus.
  • thermodynamic apparatus general have a turbine with a built in combustion chamber.
  • the combustion chamber is configured to burn a relative high grade fuel such as high yielding coal. Consequently there is abundance of relatively lowgrade resources such as lowgrade coal, biomass, municipal waste and the like, which are unused and considered waste materials. These waste materials are normally left in the open and generally looked upon as environmental scars.
  • Coal mine vVentilation air methane contributes approximately 64% of coalmine CH 4 emissions, and is difficult to use as an energy source, as the air volume is large and the methane resource is dilute and variable in concentration and flow rate.
  • the low concentration of methane in mine ventilation air is a major problem, and mitigation requires either treatment in its dilute state, or concentrating up to levels that can be used in conventional methane fueled engines.
  • Effective technology for increasing the concentration of methane is not available but it is being developed, and most work has focussed on the oxidation of very low concentration methane. These processes are complex and not cost effective.
  • Methane is a homogonous gas that requires large amounts of heat energy to oxidise at low concentrations ⁇ 1 % in air. This is normally accomplished by exposing low concentration to very high temperatures >1000 0 C for .3 of a second.
  • the combustion mechanism of methane may be overall represented by the following equation:
  • Figure 1 shows a possible mechanism for methane catalytic oxidation proposed in the article entitled Methane oxidation over noble metal catalysts as related to controlling natural gas vehicle emissions, In: Silver JE and Summers (Eds), Catalytic control of air pollution: mobile and stationary sources, 202 nd National Meeting of the American Chemical Society, 25-30 August 1991 , ACS Series, Vol. 495, pp12-25.
  • "a” indicates an adsorbed phase and "g” a gas phase.
  • catalytic combustion is a multi-step process involving diffusion to the catalyst surface, adsorption onto the catalyst, reaction, and desorption of the product species from the catalyst surface and diffusion back into the bulk.
  • Most kinetic investigations have been performed in conditions where methane is present in excess of the stoichiometric ratio. The result of this is that the reaction has generally been found to be independent of the oxygen concentration.
  • the reaction order with respect to methane is generally found to be between 0.5 and 1.
  • the activation energies are quite variable, being dependent on the catalyst and operating temperature. Platinum and palladium are generally accepted as the most active catalysts for low temperature total oxidation. Other catalysts have been tested but are less active.
  • An object of the present invention is to provide a combustion apparatus which will at least reduce one or more of the above prior art disadvantages.
  • a further object of the present invention is to provide an indirect fired thermodynamic system which may be adapted to use relatively low grade fuel resources.
  • the present invention resides in a combustion apparatus for combusting one or more combustible media.
  • the apparatus comprises a combustion unit having a fuel inlet adapted to receive said one or more combustible media for combustion therein, and a gas outlet adapted for combustion gas formed during combustion to flow out of said combustion unit to provide heat energy to a down stream apparatus.
  • the combustion unit is arranged to provide a volatile release reaction, a char combustion reaction and a gas phase reaction.
  • the fuel inlet is configured to receive gaseous and solid combustible media
  • the apparatus includes a preheating arrangement adapted to preheat the gaseous medium or any of said gaseous media.
  • the heating arrangement is arranged to receive the combustion gas before or subsequent to reaching said down stream apparatus.
  • the apparatus may have a mixing unit arranged upstream of said combustion unit.
  • the mixing unit is adapted to mix the gaseous fuel media and solid waste fuel media from said combustion unit, and the mixed media are then conveyed to the combustion unit.
  • said one or more fuel media include a low grade fuel in the form of low grade coal, biomass or municipal waste.
  • said combustion unit is a kiln.
  • said combustion unit is a rotary kiln.
  • Said down stream apparatus may be a thermodynamic apparatus comprising a compressor, an expander and heat exchange means connecting the compressor and the expander in an open or closed cycle, and a compressible working medium arranged to flow in the open or closed cycle.
  • said combustion gas is arranged to heat said working medium at the heat exchange means.
  • the expander may release exhaust gas and the exhaust gas is conveyed to the combustion unit or the mixing unit for heating media therein.
  • said solid fuel medial is a low grade coal and the kiln is adapted to convert said coal into flue gas and ash which can be formed as a byproduct such as closed or open cell spherical nodules for lightweight building materials.
  • Limestone may be added to convert any sulphur dioxide to calcium sulphate. This should at least reduce the amount of low grade coal which poses environmental problems.
  • said gaseous fuel media is methane gas. This is specially advantageous as very low concentration methane from an underground mine can be put into good use while at the same time removing it from the mine.
  • the heat exchange means includes a first heat exchanger arranged for receiving said combustion gas from said combustion unit.
  • the combustion apparatus thus not only mitigates mine methane and utilises waste coal, but also to recover waste energy for power generation.
  • the waste coal could be combusted with mine methane from both drainage gas and ventilation air inside a rotating kiln, in particular, drainage gas flame could play a role in stabilising combustion process inside the kiln.
  • the rotary kiln has an "open structure" which earmarks it for mass burn applications involving bulky and "gooey" fuels and wastes.
  • Figure l is a schematic diagram of known reaction processes in methane catalytic oxidation
  • FIG. 2 is a schematic diagram of an embodiment of the thermodynamic system according to the present invention
  • Figure 3 is a schematic diagram of another embodiment of the thermodynamic system according to the present invention
  • Figure 4 is a specific form of the apparatus shown in Figure 3 being adapted to use low grade coal and waste methane as fuel sources;
  • Figure 5 is a graph showing variations in gas temperatures with flow ratios
  • Figure 6 is a graph showing percentage variations in energy versus flow ratios
  • Figure 7 a graph showing variations in efficiency versus flow ratios
  • Figure 8 is a graph showing variations in the ratios waste coal to ventilation air versus flow ratios.
  • thermodynamic system 10 according to an embodiment of the present invention.
  • the system 10 has a combustion apparatus 12 and a closed cycle thermodynamic apparatus 14.
  • the apparatus 14 is for powering a turbine engine.
  • the apparatus 14 has a compressor 16 for compressing a working medium which in this case is air.
  • the compressed air from the compressor 16 is preheated in a recuperator 20 with exhaust air from a turbine 18.
  • the preheated compressed air is then conveyed to a high temperature heat exchanger 22 from which it returns to the turbine 18 where it expands to provide energy (power output) to perform work at the turbine 18.
  • the turbine in this case turns a generator (not shown) to generate electricity.
  • the combustion apparatus 12 has a combustion unit in the form of a rotary kiln 24 having an inlet 26 with a port for feed gas and another port 27 for feed coal.
  • Combustion gas in the combustion unit 24 travels from the outlet 28 to provide heat energy to the high temperature heat exchanger 22 for heating the compressed gas.
  • the combustion gas then travels further to a low temperature heat exchanger for preheating ventilation air or drain air from a coal mine or any location in which methane is generated, before being put to flue.
  • the preheated ventilation air is mixed with solid wastes from the kiln 24 at a mixing unit 32 and the mixed materials are then subject to further heating at a recuperator 34 prior to feeding into the combustion unit 24.
  • the combustion unit 24 represents the reactions occurring between feed coal and pre-heated feed gas, including volatile release, char combustion and gas phase reaction.
  • Char burnout is estimated using an empirical correlation dependent on the temperature of reaction, as given in the equation below. This is for an arbitrary kiln and should be modified to correlate with experimental results for a specific kiln, operating conditions and feed coal.
  • the product gas from the kiln is taken to be at equilibrium at the kiln exit.
  • An estimate of heat loss from the kiln is determined from experimental data. Two products exit the kiln, one is a hot combustion gas and the other solid wastes comprising of char and ash. These are used to pre-heat the feed gas by mixing and re-separating the solids and gas;
  • the net power output of the system 10 is calculated by subtracting the power requirements for the compressor and fan from the power generated by the turbine.
  • the efficiency is determined by dividing the net power output by the sum of the calorific values of the feed coal and ventilation air. In the system shown the calculated efficiency is 26.1 %, with the coal being 50% ash content (heating value 10.1 MJ/kg) and the ventilation air containing 0.37% methane
  • the second embodiment of the thermodynamic apparatus 10 as shown is substantially similar to that shown in Figure 2 and the same numeral references are used for the same components.
  • Some of the components shown on the schematic diagram are symbolic only and are used to break the process up into sub-processes that can be more readily shown. For example, there are 8 units on the left of the Figure that are used in the model to replicate distinct processes that occur in the real kiln. A description of how the model describes the kiln through these separate unit operations is given below.
  • MIX-100' is a mixer that combines all the feeds to the kiln, namely air streams, coal and liquefied petroleum gas (LPG);
  • 'Volatile combust' is a reactor that transfers the volatile component of the coal into the gas phase and allows reaction of the volatiles with the other gases. Volatile release is typically the first stage of coal combustion and is the only stage likely to compete with the LPG in the consumption of oxygen;
  • 'Char burn' is a reactor that estimates the proportion of the coal char that will react with the remaining oxygen given the reaction temperature, where the temperature and proportion of char burnt are calculated iteratively.
  • a quadratic expression is used to estimate the percentage of the char burnt based on the peak temperature reached during reaction, as given below where X G is the percent of char combusted and T is the resultant temperature in Kelvin.
  • the equation is entirely empirical and was designed on the basis that the conversion will be low at low temperatures (-0% at 300K) and approach 100% at 2000K. It is for an arbitrary kiln and should be modified to correlate with experimental results for a specific kiln, operating conditions and feed coal;
  • • 'Gas equil' is a reactor that allows the gases to react so that an equilibrium composition and temperature at the exit of the kiln is calculated. This will only be a significant operation when the feeds to the kiln are close to stoichiometric ratios, so carbon monoxide and hydrogen may be produced in small quantities. Under typical combustion conditions, the gases will be fully oxidised to carbon dioxide and water vapour; • 'MIX-107' is a mixer that recombines solid and gas phases;
  • ⁇ -113' is a heat exchanger that transfers some heat from the kiln to preheat air that is being blown through the outer jacket of the kiln to be used as extra combustion air in the kiln;
  • • 'Kiln HL' is a fictional heat exchanger that represents the heat loss from the kiln and associated pipework to the atmosphere. This can be used to adjust the exit temperature of the kiln to match experimentally acquired values;
  • the indirectly fired turbine system constitutes the right half of the process diagram. This is comprised of two heat exchangers that transfer heat from the kiln product gas to compressed air, a topping combustor to heat the air to the required temperature and a turbine-compressor set (shown as a separate turbine and compressor units).
  • the diagram also includes a number of fictional heat exchangers that are used to represent heat losses from pipework and unit items of equipment.
  • the topping combustor burns methane in the compressed air to maintain the turbine inlet temperature at the target temperature.
  • the net power output of the system is calculated by subtracting the power requirements for the compressor and fan from the power generated by the turbine.
  • it can tune the model to identify the heat losses for the major components, the performance of the rotating plant and the unknown flow rates using the model.
  • the model can then be used as a tool for predicting the performance of the experimental plant under different operating conditions and developing designs for improved configurations.
  • the combustion unit 24 of the apparatus 12 is in the form of a rotary kiln adapted to receive low grade coal which has been ground to a size about 6 -
  • the rotary kiln 24 is also designed so that the low grade coal has a relatively long residence time therein and a relatively large surface area of high temperatures, for ensuring combustion of very low concentration mine methane.
  • the apparatus 24 shown in Figure 2 and 3 can therefore be utilised to burn reject coal (low grade coal) and waste mine methane.
  • the ash from the burnt coal can be processed so that it is converted into a useful by-product such as closed or open cell spherical nodules ideal for manufacture of lightweight building materials and gravel substitutes. In this manner, little or no fly ash or slag is produced from combustion of low grade coal with extremely high ash contents.
  • Limestone can be added to convert any sulphur compound to calcium sulphate. Greenhouse benefits can be maximised by sizing the plant to use all the mine ventilation air and rejects. This utilises carbonaceous waste that may eventually become carbon dioxide emissions by spontaneous combustion if stockpiled on the surface. Having separate flow paths provides the system with the flexibility to vary the proportion of ventilation air to gas turbine flow rate. This is managed by setting the temperature at which the gas is exhausted from the high temperature heat exchanger.
  • Figure 4 shows the ratio of ventilation air to gas turbine flow rate as a function of the primary heat exchanger exit temperature. This value has a practical range for 0.5 to 2.5, with the minimum value set by the energy value of the waste coal.
  • Figure 5 Changing the kiln/turbine flow ratio alters the proportion of energy derived from ventilation air compared to the waste coal and this is illustrated by Figure 5 for a number of different methane concentrations.
  • Figure 5 also demonstrates how the system flexibility allows it to be used from a range of 0% to 100% ventilation air. This allows the system performance to be matched to the mine's requirements.
  • variation in methane concentration occurs in a plane parallel to the vertical axis of the plot. Variability in methane concentration is compensated for by an increase in coal flow rate and not by a change to the turbine/kiln flow ratio.
  • the flow rate of coal can also be maximised by changing the kiln/turbine ratio.
  • Figure 7 shows the mass ratio of coal to ventilation air with changes to the kiln/turbine flow ratio. It demonstrates that the facility can also be operated in a coal only manner for applications where no ventilation air is available or the operation of the mine has ceased. This system is a candidate for remediation of waste coal stockpiles from older mines.

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  • Engineering & Computer Science (AREA)
  • Mechanical Engineering (AREA)
  • General Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Combustion & Propulsion (AREA)
  • Environmental & Geological Engineering (AREA)
  • Air Supply (AREA)
  • Incineration Of Waste (AREA)

Abstract

L'invention concerne un appareil de combustion (10) pour brûler un ou plusieurs combustibles, tels que du méthane de mine et des déchets de charbon. L'appareil est doté d'une unité de combustion (24) avec une entrée de combustible (26, 27), à travers laquelle les combustibles entrent dans l'unité de combustion pour une combustion dans celle-ci, et une sortie de gaz (28) afin que les gaz formés pendant la combustion s'écoulent hors de l'unité de combustion de manière à fournir une énergie calorifique à un appareil en aval, tel qu'un moteur à turbine (14). L'unité de combustion est agencée pour fournir une réaction de libération des matières volatiles, une réaction de combustion de charbon et une réaction en phase gazeuse.
PCT/AU2007/001938 2006-12-15 2007-12-13 Appareil de combustion Ceased WO2008070931A1 (fr)

Priority Applications (4)

Application Number Priority Date Filing Date Title
US12/528,361 US20110059410A1 (en) 2006-12-15 2007-12-13 combustion apparatus
CN200780051161.1A CN101631845B (zh) 2006-12-15 2007-12-13 燃烧设备
AU2007332089A AU2007332089B2 (en) 2006-12-15 2007-12-13 A combustion apparatus
EA200900840A EA200900840A1 (ru) 2006-12-15 2007-12-13 Устройство для сжигания

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
AU2006907028A AU2006907028A0 (en) 2006-12-15 A combustion apparatus
AU2006907028 2006-12-15

Publications (1)

Publication Number Publication Date
WO2008070931A1 true WO2008070931A1 (fr) 2008-06-19

Family

ID=39511167

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/AU2007/001938 Ceased WO2008070931A1 (fr) 2006-12-15 2007-12-13 Appareil de combustion

Country Status (5)

Country Link
US (1) US20110059410A1 (fr)
CN (1) CN101631845B (fr)
AU (1) AU2007332089B2 (fr)
EA (1) EA200900840A1 (fr)
WO (1) WO2008070931A1 (fr)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US9677398B2 (en) 2011-04-15 2017-06-13 Solvay Chemicals, Inc. Use of ventilation air methane exhausted during mining of non-combustible ore in a surface appliance

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CN101435338B (zh) * 2008-12-17 2011-12-07 胜利油田胜利动力机械集团有限公司 煤矿低浓度瓦斯甲烷销毁方法及装置
AU2009338680B2 (en) * 2009-01-29 2015-12-17 Commonwealth Scientific And Industrial Research Organisation System and method for mitigating at least one component from a fluid stream
EP2760790B1 (fr) 2011-09-30 2018-01-10 Newcastle Innovation Limited Élimination par cyclage chimique de méthane d'un air de ventilation
JP5456073B2 (ja) 2012-01-06 2014-03-26 三菱重工業株式会社 石炭不活性化処理装置
JP5971652B2 (ja) 2012-10-09 2016-08-17 三菱重工業株式会社 石炭不活性化処理装置
JP5536247B1 (ja) * 2013-03-04 2014-07-02 三菱重工業株式会社 石炭不活性化処理装置
PL2784388T3 (pl) * 2013-03-28 2015-07-31 Linde Ag Sposób spalania paliwa niskogatunkowego
CN111648745A (zh) * 2020-05-21 2020-09-11 河南理工大学 二氧化碳突出矿井抽采气体提升二氧化碳浓度的系统

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Publication number Priority date Publication date Assignee Title
US9677398B2 (en) 2011-04-15 2017-06-13 Solvay Chemicals, Inc. Use of ventilation air methane exhausted during mining of non-combustible ore in a surface appliance

Also Published As

Publication number Publication date
CN101631845A (zh) 2010-01-20
AU2007332089B2 (en) 2012-05-17
EA200900840A1 (ru) 2009-12-30
CN101631845B (zh) 2014-03-12
AU2007332089A1 (en) 2008-06-19
US20110059410A1 (en) 2011-03-10

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