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WO2003004942A1 - Reacteur permettant d'exploiter la chaleur du rayonnement solaire - Google Patents

Reacteur permettant d'exploiter la chaleur du rayonnement solaire Download PDF

Info

Publication number
WO2003004942A1
WO2003004942A1 PCT/CH2002/000361 CH0200361W WO03004942A1 WO 2003004942 A1 WO2003004942 A1 WO 2003004942A1 CH 0200361 W CH0200361 W CH 0200361W WO 03004942 A1 WO03004942 A1 WO 03004942A1
Authority
WO
WIPO (PCT)
Prior art keywords
absorber
reactor according
reactor
heat
solar radiation
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/CH2002/000361
Other languages
German (de)
English (en)
Other versions
WO2003004942A8 (fr
Inventor
Wolfgang Hoffelner
Aldo Steinfeld
Daniel Wuillemin
Anton Meier
Beatrice Schaffner
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Scherrer Paul Institut
Original Assignee
Scherrer Paul Institut
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Scherrer Paul Institut filed Critical Scherrer Paul Institut
Priority to AU2002315618A priority Critical patent/AU2002315618A1/en
Publication of WO2003004942A1 publication Critical patent/WO2003004942A1/fr
Publication of WO2003004942A8 publication Critical patent/WO2003004942A8/fr
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

Links

Classifications

    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F28—HEAT EXCHANGE IN GENERAL
    • F28F—DETAILS OF HEAT-EXCHANGE AND HEAT-TRANSFER APPARATUS, OF GENERAL APPLICATION
    • F28F13/00—Arrangements for modifying heat-transfer, e.g. increasing, decreasing
    • F28F13/14—Arrangements for modifying heat-transfer, e.g. increasing, decreasing by endowing the walls of conduits with zones of different degrees of conduction of heat
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J19/0053—Details of the reactor
    • B01J19/0073—Sealings
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J19/02—Apparatus characterised by being constructed of material selected for its chemically-resistant properties
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J19/08—Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor
    • B01J19/12—Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor employing electromagnetic waves
    • B01J19/122—Incoherent waves
    • B01J19/127—Sunlight; Visible light
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J19/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J19/18—Stationary reactors having moving elements inside
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F24—HEATING; RANGES; VENTILATING
    • F24S—SOLAR HEAT COLLECTORS; SOLAR HEAT SYSTEMS
    • F24S20/00—Solar heat collectors specially adapted for particular uses or environments
    • F24S20/20—Solar heat collectors for receiving concentrated solar energy, e.g. receivers for solar power plants
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F24—HEATING; RANGES; VENTILATING
    • F24S—SOLAR HEAT COLLECTORS; SOLAR HEAT SYSTEMS
    • F24S70/00—Details of absorbing elements
    • F24S70/10—Details of absorbing elements characterised by the absorbing material
    • F24S70/16—Details of absorbing elements characterised by the absorbing material made of ceramic; made of concrete; made of natural stone
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F24—HEATING; RANGES; VENTILATING
    • F24S—SOLAR HEAT COLLECTORS; SOLAR HEAT SYSTEMS
    • F24S70/00—Details of absorbing elements
    • F24S70/60—Details of absorbing elements characterised by the structure or construction
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J2219/00049—Controlling or regulating processes
    • B01J2219/00051—Controlling the temperature
    • B01J2219/00139—Controlling the temperature using electromagnetic heating
    • B01J2219/00144—Sunlight; Visible light
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2219/00—Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J2219/02—Apparatus characterised by their chemically-resistant properties
    • B01J2219/0204—Apparatus characterised by their chemically-resistant properties comprising coatings on the surfaces in direct contact with the reactive components
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02B—CLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO BUILDINGS, e.g. HOUSING, HOUSE APPLIANCES OR RELATED END-USER APPLICATIONS
    • Y02B10/00—Integration of renewable energy sources in buildings
    • Y02B10/20—Solar thermal
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E10/00—Energy generation through renewable energy sources
    • Y02E10/40—Solar thermal energy, e.g. solar towers

Definitions

  • the invention has for its object to provide a reactor of the type mentioned, which is even better suited for the use of solar radiant heat for thermal and thermochemical processes of different substances and in particular for a flat treatment of such substances.
  • the absorber is a volumetric black-body absorber which is arranged in a stove and which brings heat into the stove with a rear side.
  • the blackbody absorber is heated by solar energy and the heat is radiated into the hearth via a rear side.
  • the heat can be dissipated indirectly onto the material to be treated over a much larger area than before.
  • the reactor according to the invention is particularly suitable for the treatment of various types of dusts. Volatile elements, such as zinc or lead, can also be evaporated particularly effectively.
  • FIG. 1 shows schematically a section through an inventive reactor
  • the material C to be treated is introduced into the space 117 via a loading device 16.
  • the absorber 102 and the carrier 104 connected to it are continuously rotated about the axis A by the drive 7. If necessary, the cooker 109 can also rotate at the same time.
  • the material C introduced into the space 117 from above is conveyed downward by the transport screw 105 and comes into the area of a rear side 126 of the absorber 102 and is thus exposed to the radiant heat of the absorber 102. Above this area, the material C is exposed to the radiant heat of the carrier 104, which is, however, significantly lower than that in the lower area mentioned above.
  • pyrolysis is carried out at 500-600 ° C.
  • material C is melted, for example. Molten material C reaches the retraction table 113, which is slowly withdrawn downwards in accordance with the accumulation of molten material.

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Physics & Mathematics (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Mechanical Engineering (AREA)
  • Organic Chemistry (AREA)
  • General Engineering & Computer Science (AREA)
  • Thermal Sciences (AREA)
  • Sustainable Energy (AREA)
  • Combustion & Propulsion (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • Ceramic Engineering (AREA)
  • Toxicology (AREA)
  • Health & Medical Sciences (AREA)
  • Electromagnetism (AREA)
  • General Health & Medical Sciences (AREA)
  • Analytical Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Physical Or Chemical Processes And Apparatus (AREA)
  • Processing Of Solid Wastes (AREA)
  • Manufacture And Refinement Of Metals (AREA)

Abstract

La présente invention concerne un réacteur permettant d'exploiter la chaleur du rayonnement solaire pour des processus thermiques ou thermochimiques. Ce réacteur présente un logement de réacteur (1, 101), qui comprend une ouverture (2a, 125) permettant l'entrée du rayonnement solaire dans le logement de réacteur (1, 101), un espace réactionnel (13, 117) et un absorbeur volumétrique (2, 102), qui est chauffé sur la face frontale (2b, 102b) par le rayonnement solaire et qui libère de la chaleur dans l'espace réactionnel (13, 117). Cet absorbeur (2, 102) est un absorbeur à corps noir qui est monté dans un creuset (4, 109) et qui introduit avec une face arrière (2c, 126) de la chaleur dans le creuset (4, 109). L'avantage du réacteur selon cette invention est que la chaleur peut être libérée indirectement sur le produit à traiter, sur une surface sensiblement plus grande que jusqu'à présent.
PCT/CH2002/000361 2001-07-05 2002-07-03 Reacteur permettant d'exploiter la chaleur du rayonnement solaire Ceased WO2003004942A1 (fr)

Priority Applications (1)

Application Number Priority Date Filing Date Title
AU2002315618A AU2002315618A1 (en) 2001-07-05 2002-07-03 Reactor for using solar radiant heat

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH1240/01 2001-07-05
CH12402001 2001-07-05

Publications (2)

Publication Number Publication Date
WO2003004942A1 true WO2003004942A1 (fr) 2003-01-16
WO2003004942A8 WO2003004942A8 (fr) 2003-10-02

Family

ID=4564608

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/CH2002/000361 Ceased WO2003004942A1 (fr) 2001-07-05 2002-07-03 Reacteur permettant d'exploiter la chaleur du rayonnement solaire

Country Status (2)

Country Link
AU (1) AU2002315618A1 (fr)
WO (1) WO2003004942A1 (fr)

Cited By (15)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1475581A1 (fr) 2003-05-09 2004-11-10 Paul Scherrer Institut Réacteur pour utilisation indirecte de rayonnements thermiques externes
EP1656990A1 (fr) * 2004-11-08 2006-05-17 Paul Scherrer Institut Réacteur rotatif utilisant de l'énergie solaire
EP1658892A1 (fr) * 2004-11-17 2006-05-24 Paul Scherrer Institut Réacteur pour des procédés thérmiques ou chimique-thérmiques avec capacité de nettoyage and procédé pour nettoyer une surface interne chaude d'un réacteur utilisé pour des procédés thérmiques ou chimique-thérmiques
WO2006048224A3 (fr) * 2004-11-08 2006-07-20 Scherrer Inst Paul Reacteur pour utilisation directe de chaleur de rayonnement externe dans le traitement thermique ou thermochimique de materiaux
WO2013096813A1 (fr) * 2011-12-22 2013-06-27 University Of Florida Research Foundation, Inc. Réacteur thermochimique solaire, procédés de sa fabrication et de son utilisation et thermogravimètre
US8865100B2 (en) 2008-06-02 2014-10-21 Exxonmobil Upstream Research Company Monetizing remote gas using high energy materials
EP2944894A3 (fr) * 2014-04-28 2016-01-20 Adnan Ayman Al-Maaitah Procédé et appareil pour le suivi et la concentration des ondes électromagnétiques provenant d'une source mobile vers un point focal fixe
US9776154B2 (en) 2012-12-21 2017-10-03 University Of Florida Research Foundation, Inc. Material comprising two different non-metallic parrticles having different particle sizes for use in solar reactor
US9966171B2 (en) 2011-07-08 2018-05-08 University Of Florida Research Foundation, Inc. Porous stabilized beds, methods of manufacture thereof and articles comprising the same
WO2018205043A1 (fr) * 2017-05-10 2018-11-15 Synhelion Sa Procédé pour faire fonctionner un récepteur et récepteur pour mettre en œuvre le procédé
CH713765A1 (de) * 2017-05-10 2018-11-15 Synhelion Sa C/O Avv Luca Tenchio Verfahren zum Betrieb eines Receivers und Receiver zur Ausführung des Verfahrens.
US10239036B2 (en) 2011-12-22 2019-03-26 University Of Florida Research Foundation Solar thermochemical reactor, methods of manufacture and use thereof and thermogravimeter
US10906017B2 (en) 2013-06-11 2021-02-02 University Of Florida Research Foundation, Inc. Solar thermochemical reactor and methods of manufacture and use thereof
WO2022253716A1 (fr) * 2021-06-01 2022-12-08 Deutsches Zentrum für Luft- und Raumfahrt e.V. Système de réacteur thermochimique
CN118079827A (zh) * 2024-02-26 2024-05-28 哈尔滨工业大学 一种太阳能反应器装置及试验方法

Citations (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2793018A (en) * 1952-07-24 1957-05-21 Centre Nat Rech Scient Furnace for the treatment of substances by means of the energy supplied by a concentrated radiation
US4030890A (en) * 1975-10-20 1977-06-21 Diggs Richard E Solar power system
US4033118A (en) * 1974-08-19 1977-07-05 Powell William R Mass flow solar energy receiver
US4432344A (en) 1981-07-15 1984-02-21 Focus Environmental Systems Method and apparatus for solar destruction of toxic and hazardous materials
US4549528A (en) 1984-02-21 1985-10-29 Focus Environmental Systems Method and apparatus for solar destruction of toxic and hazardous materials
US4706651A (en) 1986-02-24 1987-11-17 The United States Of America As Represented By The United States Department Of Energy Solar solids reactor
US5128115A (en) * 1991-04-08 1992-07-07 The United States Of America As Represented By The United States Department Of Energy Manufacture of silicon carbide using solar energy
DE4109044A1 (de) * 1991-03-15 1992-09-17 Noell K & K Abfalltech Verfahren zur thermischen entsorgung von reststoffen aus der rauchgasreinigung
US5421322A (en) 1992-01-23 1995-06-06 Yeda Research And Development Company Limited Central solar receiver
DE19937188C1 (de) * 1999-08-06 2000-12-14 Thermoselect Ag Vaduz Verfahren zur Verwertung von Gasen aus dem Absetzbecken
DE19952174A1 (de) * 1999-10-29 2001-05-10 Bathen Dieter Empfänger für konzentrierte Solarstrahlung zur Durchführung von Hochtemperaturprozessen

Patent Citations (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2793018A (en) * 1952-07-24 1957-05-21 Centre Nat Rech Scient Furnace for the treatment of substances by means of the energy supplied by a concentrated radiation
US4033118A (en) * 1974-08-19 1977-07-05 Powell William R Mass flow solar energy receiver
US4030890A (en) * 1975-10-20 1977-06-21 Diggs Richard E Solar power system
US4432344A (en) 1981-07-15 1984-02-21 Focus Environmental Systems Method and apparatus for solar destruction of toxic and hazardous materials
US4549528A (en) 1984-02-21 1985-10-29 Focus Environmental Systems Method and apparatus for solar destruction of toxic and hazardous materials
US4706651A (en) 1986-02-24 1987-11-17 The United States Of America As Represented By The United States Department Of Energy Solar solids reactor
DE4109044A1 (de) * 1991-03-15 1992-09-17 Noell K & K Abfalltech Verfahren zur thermischen entsorgung von reststoffen aus der rauchgasreinigung
US5128115A (en) * 1991-04-08 1992-07-07 The United States Of America As Represented By The United States Department Of Energy Manufacture of silicon carbide using solar energy
US5421322A (en) 1992-01-23 1995-06-06 Yeda Research And Development Company Limited Central solar receiver
DE19937188C1 (de) * 1999-08-06 2000-12-14 Thermoselect Ag Vaduz Verfahren zur Verwertung von Gasen aus dem Absetzbecken
DE19952174A1 (de) * 1999-10-29 2001-05-10 Bathen Dieter Empfänger für konzentrierte Solarstrahlung zur Durchführung von Hochtemperaturprozessen

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
ARISTOV Y I ET AL: "COMPARATIVE CHARACTERISTICS OF SOLAR CATALYTIC REACTORS WITH TRANSPARENT AND OPAQUE RADIATION-RECEIVING SURFACES", APPLIED SOLAR ENERGY (GELIOTEKHNIKA), ALLERTON PRESS INC, NEW YORK, US, vol. 25, no. 5, 1989, pages 61 - 65, XP000134997, ISSN: 0003-701X *

Cited By (23)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1475581A1 (fr) 2003-05-09 2004-11-10 Paul Scherrer Institut Réacteur pour utilisation indirecte de rayonnements thermiques externes
EP1656990A1 (fr) * 2004-11-08 2006-05-17 Paul Scherrer Institut Réacteur rotatif utilisant de l'énergie solaire
WO2006048224A3 (fr) * 2004-11-08 2006-07-20 Scherrer Inst Paul Reacteur pour utilisation directe de chaleur de rayonnement externe dans le traitement thermique ou thermochimique de materiaux
US8083520B2 (en) 2004-11-08 2011-12-27 Paul Scherrer Institut Reactor for direct utilization of external radiation heat for thermal or thermo-chemical material processes
EP1658892A1 (fr) * 2004-11-17 2006-05-24 Paul Scherrer Institut Réacteur pour des procédés thérmiques ou chimique-thérmiques avec capacité de nettoyage and procédé pour nettoyer une surface interne chaude d'un réacteur utilisé pour des procédés thérmiques ou chimique-thérmiques
US8865100B2 (en) 2008-06-02 2014-10-21 Exxonmobil Upstream Research Company Monetizing remote gas using high energy materials
US9966171B2 (en) 2011-07-08 2018-05-08 University Of Florida Research Foundation, Inc. Porous stabilized beds, methods of manufacture thereof and articles comprising the same
US12119148B2 (en) 2011-07-08 2024-10-15 University Of Florida Research Foundation, Inc. Porous stabilized beds, methods of manufacture thereof and articles comprising the same
US11705255B2 (en) 2011-07-08 2023-07-18 University Of Florida Research Foundation, Inc. Porous stabilized beds, methods of manufacture thereof and articles comprising the same
US10991490B2 (en) 2011-07-08 2021-04-27 University Of Florida Research Foundation, Inc. Porous stabilized beds, methods of manufacture thereof and articles comprising the same
WO2013096813A1 (fr) * 2011-12-22 2013-06-27 University Of Florida Research Foundation, Inc. Réacteur thermochimique solaire, procédés de sa fabrication et de son utilisation et thermogravimètre
US10239036B2 (en) 2011-12-22 2019-03-26 University Of Florida Research Foundation Solar thermochemical reactor, methods of manufacture and use thereof and thermogravimeter
US10239035B2 (en) 2011-12-22 2019-03-26 University Of Florida Research Foundation, Inc. Solar thermochemical reactor, methods of manufacture and use thereof and thermogravimeter
US9669379B2 (en) 2011-12-22 2017-06-06 University Of Florida Research Foundation, Inc Solar thermochemical reactor, methods of manufacture and use thereof and thermogravimeter
US9776154B2 (en) 2012-12-21 2017-10-03 University Of Florida Research Foundation, Inc. Material comprising two different non-metallic parrticles having different particle sizes for use in solar reactor
US10906017B2 (en) 2013-06-11 2021-02-02 University Of Florida Research Foundation, Inc. Solar thermochemical reactor and methods of manufacture and use thereof
EP2944894A3 (fr) * 2014-04-28 2016-01-20 Adnan Ayman Al-Maaitah Procédé et appareil pour le suivi et la concentration des ondes électromagnétiques provenant d'une source mobile vers un point focal fixe
WO2018205043A1 (fr) * 2017-05-10 2018-11-15 Synhelion Sa Procédé pour faire fonctionner un récepteur et récepteur pour mettre en œuvre le procédé
CH713765A1 (de) * 2017-05-10 2018-11-15 Synhelion Sa C/O Avv Luca Tenchio Verfahren zum Betrieb eines Receivers und Receiver zur Ausführung des Verfahrens.
US12078389B2 (en) 2017-05-10 2024-09-03 Synhelion Sa Method for operating a receiver and receiver for carrying out the method
WO2022253716A1 (fr) * 2021-06-01 2022-12-08 Deutsches Zentrum für Luft- und Raumfahrt e.V. Système de réacteur thermochimique
CN118079827A (zh) * 2024-02-26 2024-05-28 哈尔滨工业大学 一种太阳能反应器装置及试验方法
CN118079827B (zh) * 2024-02-26 2024-10-25 哈尔滨工业大学 一种太阳能反应器装置及试验方法

Also Published As

Publication number Publication date
WO2003004942A8 (fr) 2003-10-02
AU2002315618A1 (en) 2003-01-21

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