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US1940372A - Method of obtaining phytosterol, fatty acids and resin acids from raw soap or liquidresin obtained in the manufacture of cellulose according to the sulphate method - Google Patents

Method of obtaining phytosterol, fatty acids and resin acids from raw soap or liquidresin obtained in the manufacture of cellulose according to the sulphate method Download PDF

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Publication number
US1940372A
US1940372A US556716A US55671631A US1940372A US 1940372 A US1940372 A US 1940372A US 556716 A US556716 A US 556716A US 55671631 A US55671631 A US 55671631A US 1940372 A US1940372 A US 1940372A
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Prior art keywords
soap
acids
manufacture
fatty acids
phytosterol
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Expired - Lifetime
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US556716A
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Sandqvist Emma Emelie
Lindstrom Torsten Hjalmarsson
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    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07JSTEROIDS
    • C07J9/00Normal steroids containing carbon, hydrogen, halogen or oxygen substituted in position 17 beta by a chain of more than two carbon atoms, e.g. cholane, cholestane, coprostane
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07JSTEROIDS
    • C07J75/00Processes for the preparation of steroids in general

Definitions

  • Liquid resin is generally obtained from said soap. Since the beginning of this century tests have been made technically to use the constituents of these products but still no satisfying solution of this problem seems to be at hand.
  • phytosterols may be extensively employed in obtaining emulsions of a certain type inter alia of hydrated salves, the question of utilizing this soap may be regarded from quite a new point of view, for instance, in the production of water-absorbing salve bases by means of vaseline, parafllne and the like possesses a very high economic value.
  • the raw soap or liquid resin, obtained in the manufacture of cellulose according to the sulphate process is extracted in a dried condition or in a highly concentrated solution by means of a suitable solvent, in which phytosterol and non-saponiflable substances are soluble.
  • the said soap is diluted with a suitable quantity of water for instance 1 to 2 parts, the solution being extracted for example by means of ether, carbon disulphide, carbon tetrachloride, benzol or the like.
  • the said soap is dried at about 100 C. at an extremely reduced pressure, for instance at a pressure below mm. of mercury, and is then obtained in aporous condition being very suitable for the extraction.
  • the extraction is carried out for instance by means of ether.
  • Benzine is unsuitable as an extraction agent, phytosterol being comparatively diiiiculty soluble in the same.
  • Benzol is unsuitable in the extraction of dried soap, beneaol dissolving great quantities of the very soap.
  • the extract obtained in one way or the other is shaked out by'means of caustic soda lye, the treatment absorbing dark-colored and smeary impurities, which are then removed,
  • An improved method of obtaining phytosterol, fatty acids and resin acids from raw tall oil soap obtained in the manufacture of cellulose by the sulphate method comprising drying said soap at an extremely reduced pressure, that is at a pressure below that represented by 30 mm. of mercury, extracting the raw tall oil soap in a concentrated state with a solvent in which phytosterol and non-saponiflable substances are soluble, removing impurities from the extract by shaking with an alkaline material, and distilling off the solvent and crystallizing the remainder to obtain pure phytosterol.
  • An improved method of obtaining phytosterol, Iatty'acids and resin acids from raw tall oil soap obtained in the manufacture of cellulose by the sulphate method comprising drying said soap at an extremely reduced pressure, that is at a pressure below that represented by 30 mm.
  • EMMA SANDQVIBT, Administratri: of the estate of Hakan Sandqvist, deceased. 'I'ORSTEN OLOI" HJAL- meson memoir.

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Detergent Compositions (AREA)

Description

Patented Dec. 19, 1933 UNITED STATES PATENT OFFICE Hakan Sandqvist, deceased, late of Stockholm,
Sweden, by Emma (Emelie) Sandqvist, Stockholm, Sweden,
administr atrix, and Torsten Olof Hjalmarsson Lindstriim, Kosta, Sweden No Drawing. Application August 12, 1931, Serial No. 556,716, and in Sweden March 22, .1928
2 Claims.
lye said soap containing indifferent substances,
resinand fatty acids in addition to water and alkali. Liquid resin is generally obtained from said soap. Since the beginning of this century tests have been made technically to use the constituents of these products but still no satisfying solution of this problem seems to be at hand.
Among the indifferent substances. of the said soap there are inter alia one or maybe two phytosterols. As phytosterols may be extensively employed in obtaining emulsions of a certain type inter alia of hydrated salves, the question of utilizing this soap may be regarded from quite a new point of view, for instance, in the production of water-absorbing salve bases by means of vaseline, parafllne and the like possesses a very high economic value.
According to the invention the raw soap or liquid resin, obtained in the manufacture of cellulose according to the sulphate process is extracted in a dried condition or in a highly concentrated solution by means of a suitable solvent, in which phytosterol and non-saponiflable substances are soluble. In the last-mentioned case the said soap is diluted with a suitable quantity of water for instance 1 to 2 parts, the solution being extracted for example by means of ether, carbon disulphide, carbon tetrachloride, benzol or the like. In the first-mentioned case the said soap is dried at about 100 C. at an extremely reduced pressure, for instance at a pressure below mm. of mercury, and is then obtained in aporous condition being very suitable for the extraction. The extraction is carried out for instance by means of ether. Benzine is unsuitable as an extraction agent, phytosterol being comparatively diiiiculty soluble in the same. Benzol is unsuitable in the extraction of dried soap, beneaol dissolving great quantities of the very soap. The extract obtained in one way or the other is shaked out by'means of caustic soda lye, the treatment absorbing dark-colored and smeary impurities, which are then removed,
after which the solvent is distilled from the extract and the remainder. is recrystallized from alcohol- Awhite and fine crystallized phytosterol in a quantity of about 2% of the soap employed (with 30% of water) isob 1 Fatty and resin acids are precipitated from the extracted soap by meansv of a diluted acid for instance sulphuric acid' ";iwhereby-sodium (c1. aw-4) sulphate is obtained as a by-product about 10% of the weight of the soap). The fatty acids are extracted by means of petroleum ether, benzine, ligroin, or other suitable solvents, in which the resin acids are difiicultly soluble. The fatty acids are extracted from the obtained acid mixture in its present state or after having been absorbed by some suitable solvent, such as ether and having been filtered and from which the solvent has been removed by distillation.
Having nowdescribed our invention, what we claim as new and desire to secure by Letters Patent is 1. An improved method of obtaining phytosterol, fatty acids and resin acids from raw tall oil soap obtained in the manufacture of cellulose by the sulphate method, comprising drying said soap at an extremely reduced pressure, that is at a pressure below that represented by 30 mm. of mercury, extracting the raw tall oil soap in a concentrated state with a solvent in which phytosterol and non-saponiflable substances are soluble, removing impurities from the extract by shaking with an alkaline material, and distilling off the solvent and crystallizing the remainder to obtain pure phytosterol.
2. An improved method of obtaining phytosterol, Iatty'acids and resin acids from raw tall oil soap obtained in the manufacture of cellulose by the sulphate method, comprising drying said soap at an extremely reduced pressure, that is at a pressure below that represented by 30 mm. of mercury, extracting the raw tall oil soap in a concentrated state with a solvent in which phytosterol and non-saponiflable substances are soluble, treating the'residue of extracted soap with dilute acid to decompose the same and precipitate organic acids, treating the precipitated organic acids with a solvent, such as for instance a solvent selected from the group consisting of petroleum ether, benzine and ligroin and in which the resin acids are difllcultly soluble but in which the fatty acids are very soluble to separate the fatty and resin acids, and recovering the fatty acids from the solution.
EMMA (EMELIE) SANDQVIBT, Administratri: of the estate of Hakan Sandqvist, deceased. 'I'ORSTEN OLOI" HJAL- meson memoir.
US556716A 1928-03-22 1931-08-12 Method of obtaining phytosterol, fatty acids and resin acids from raw soap or liquidresin obtained in the manufacture of cellulose according to the sulphate method Expired - Lifetime US1940372A (en)

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SE1940372X 1928-03-22

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Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2437643A (en) * 1942-05-12 1948-03-09 American Cyanamid Co Separation of neutral fat from tall oil
US2580496A (en) * 1948-07-14 1952-01-01 Fulwal Chemical Corp Separation of rosin acids
US2807607A (en) * 1953-10-06 1957-09-24 Eric O Ridgway Recovery of rosin acids

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2437643A (en) * 1942-05-12 1948-03-09 American Cyanamid Co Separation of neutral fat from tall oil
US2580496A (en) * 1948-07-14 1952-01-01 Fulwal Chemical Corp Separation of rosin acids
US2807607A (en) * 1953-10-06 1957-09-24 Eric O Ridgway Recovery of rosin acids

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