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SU764607A3 - Method of extracting rare-earth elements from apatite - Google Patents

Method of extracting rare-earth elements from apatite Download PDF

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Publication number
SU764607A3
SU764607A3 SU742025344A SU2025344A SU764607A3 SU 764607 A3 SU764607 A3 SU 764607A3 SU 742025344 A SU742025344 A SU 742025344A SU 2025344 A SU2025344 A SU 2025344A SU 764607 A3 SU764607 A3 SU 764607A3
Authority
SU
USSR - Soviet Union
Prior art keywords
apatite
rare earth
earth elements
ions
ammonia
Prior art date
Application number
SU742025344A
Other languages
Russian (ru)
Inventor
Торвалл Мейделл Глер
Стерен Харальд
Original Assignee
Норск Гидро А.С. (Фирма)
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Publication date
Application filed by Норск Гидро А.С. (Фирма) filed Critical Норск Гидро А.С. (Фирма)
Application granted granted Critical
Publication of SU764607A3 publication Critical patent/SU764607A3/en

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    • CCHEMISTRY; METALLURGY
    • C22METALLURGY; FERROUS OR NON-FERROUS ALLOYS; TREATMENT OF ALLOYS OR NON-FERROUS METALS
    • C22BPRODUCTION AND REFINING OF METALS; PRETREATMENT OF RAW MATERIALS
    • C22B59/00Obtaining rare earth metals
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01FCOMPOUNDS OF THE METALS BERYLLIUM, MAGNESIUM, ALUMINIUM, CALCIUM, STRONTIUM, BARIUM, RADIUM, THORIUM, OR OF THE RARE-EARTH METALS
    • C01F17/00Compounds of rare earth metals
    • C01F17/20Compounds containing only rare earth metals as the metal element
    • C01F17/282Sulfates

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Geology (AREA)
  • Engineering & Computer Science (AREA)
  • General Life Sciences & Earth Sciences (AREA)
  • Environmental & Geological Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Manufacturing & Machinery (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Compounds Of Alkaline-Earth Elements, Aluminum Or Rare-Earth Metals (AREA)
  • Cosmetics (AREA)
  • Fertilizers (AREA)

Abstract

A concentrate of rare earth metal phosphates is produced by dissolving a crude phosphate in HNO3, removing a substantial part of Ca2+ ions in the form of crystalline Ca(NO3)2.4H2O, and another part of Ca2+ ions by pptn. with sulphate ions, and partly neutralising the soln. with ammonia. The sulphate ions are used in an amt. determined by means of a calibration curve based on the fluoride content of the soln. The rare earth metal phosphates are pptd. by addn. of water-free ammonia and sepd. by filtration; both operations are carried out rapidly (within 15 mins) whereby the filtering props of the ppte. are improved. The process can be carried out continuously.

Description

док отфильтровывают и вес фильтро вальной лепешки (включа  маточный раствор) составл ет 120 г на 1 кг нейтрализованной суспензии. Состав фильтровальной лепешки, вес.%: , Са 6,k, Р 12, N 7,8; К 0,7; 50,7; F 0,2 и t, 1 the dock is filtered off and the weight of the filter cake (including the mother liquor) is 120 g per 1 kg of neutralized suspension. The composition of the filter cake, wt.%:, CA 6, k, R 12, N 7,8; K 0.7; 50.7; F 0,2 and t, 1

В фильтровальной лепешке содержитс  95% содержани  цери  в сыром фосфате и 50% иттри . Содержание земель в фильтровальной лепёшке 4,1% по весу, счита  на , что соответствует 85% общего содерзканий редких земель в Кольском фосфа те.The filter cake contains 95% cerium in crude phosphate and 50% yttrium. The land content in the filter cake is 4.1% by weight, which is equivalent to 85% of the total rare earth content in the Kola phosphate.

Фильтруемость осадка соответствует примерно 3 суспензии на 1 м погруженной поверхности фильтра apautcuixaerocH барабанного фильтра при разрежении 100 Мм рт.ст. И тдлщине фильтровальной лепешки 5-6 мм.The filterability of the sediment corresponds to approximately 3 suspensions per 1 m of the immersed surface of the filter apautcuixaerocH drum filter with a vacuum of 100 Mm Hg. And tdline filter cake 5-6 mm.

Пример 2. В этом опыте примен ют тот же раствор, такое же добавление сульфата и метод снижени  содержани  фторидов, как в примере 1 Однако нейтрализацию газообразйьЫ аммиаком провод т при рН 2,5 (измеренном при разбавлении водой 1:10)Example 2. In this experiment, the same solution was used, the same sulfate addition and fluoride content reduction method as in Example 1 were used. However, the neutralization of gaseous ammonia was carried out at pH 2.5 (measured by diluting with water 1:10)

Врем  пребывани  в реакторе такое же, как в примере 1 и осадок немедленно отфильтровывают. Вес фильтровальной лепешки (включа  маточный раствор) составл ет 120 г на 1 кг нейтрализованной суспензии. Состав фильтровальной лепешки, вес.%: Са 5,5; Р 10,8; Н 9,1; К 0,8; ЗОдб.О F 0,2 и k,k.The residence time in the reactor is the same as in Example 1 and the precipitate is immediately filtered off. The weight of the filter cake (including the mother liquor) is 120 g per 1 kg of neutralized suspension. The composition of the filter cake, wt.%: Ca 5.5; R 10.8; H 9.1; K 0.8; SODB O F 0,2 and k, k.

В фильтровальной лепешке присутствует почти 100% цери , содержащегос  в сыром фосфате и 75% содержаще ,гос  в ней иттри . В фильтровальной лепешке присутствует 93% содержани  редких земель сырого фосфата. Фильтpyei CTb соответствует примерно 2 м УЧ суспензии на 1м погруженной фильтрующей поверхности барабанного вакуум-фильтра при разрежении 100 мм рт.ст. и толщине фильтровальной лепешки 5-6 мм.In the filter cake there is almost 100% cerium contained in the crude phosphate and 75% contained, it contains yttrium. The filter cake contains 93% of the rare earth content of raw phosphate. Filtpyei CTb corresponds to about 2 m of UCH suspension per 1 m of submerged filtering surface of the drum vacuum filter at a vacuum of 100 mm Hg. and the thickness of the filter cake 5-6 mm.

Предлагаемый способ позвол ет извлечь редкоземе;льные элементы из апатита на 85-93%.The proposed method allows rare-earth extraction; 85–93% of apatite is a common element.

Claims (1)

Формула изобретени Invention Formula Способ извлечени  редкоземельйых элементов из апатита, включаквдий разложение апатита азотйой кислоты, вымЬрЬкивание нитрата кальци , уда0 ленив фтор-иона, нейтрализацию раствора аммиаком и фильтрацию, отличают и   тем, что, с целью повышени  извлечени  редкоземельных элементов, после вымораживани The method for extracting rare earth elements from apatite, including decomposition of nitrate acid apatite, extinction of calcium nitrate, removing fluorine ion, neutralizing the solution with ammonia and filtering, is also distinguished by the fact that, to increase the extraction of rare earth elements, after freezing 5 осаждают сульфат кальци  с последующей нейтрализацией раствора в течение менее 15 мин, предпочтительно 3-5 мин.5 precipitated calcium sulfate, followed by neutralization of the solution for less than 15 minutes, preferably 3-5 minutes. п Источники информации,n Sources of information прин тые ВО внимание при экспертизе 1. Ст..Мазгай Выделение соединений редкоземельных элементов из апатита . - Сб. ст. Методы разделени  редкоземельных металлов. Изд. И.Л. М., 1961, с. 178-184.VOs taken into account during examination 1. Art. Mazgai Isolation of compounds of rare-earth elements from apatite. - Sat. Art. Methods for the separation of rare earth metals. Ed. I.L. M., 1961, p. 178-184.
SU742025344A 1973-05-02 1974-04-30 Method of extracting rare-earth elements from apatite SU764607A3 (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
NO01814/73A NO130109B (en) 1973-05-02 1973-05-02

Publications (1)

Publication Number Publication Date
SU764607A3 true SU764607A3 (en) 1980-09-15

Family

ID=19878449

Family Applications (1)

Application Number Title Priority Date Filing Date
SU742025344A SU764607A3 (en) 1973-05-02 1974-04-30 Method of extracting rare-earth elements from apatite

Country Status (7)

Country Link
DE (1) DE2419928A1 (en)
FI (1) FI59422C (en)
HU (1) HU168089B (en)
NO (1) NO130109B (en)
RO (1) RO69797A (en)
SE (1) SE395878B (en)
SU (1) SU764607A3 (en)

Also Published As

Publication number Publication date
HU168089B (en) 1976-02-28
NO130109B (en) 1974-07-08
SE395878B (en) 1977-08-29
FI59422B (en) 1981-04-30
RO69797A (en) 1981-06-30
DE2419928A1 (en) 1974-11-21
FI59422C (en) 1981-08-10

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