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SU596659A1 - Method of protecting graphite articles from destruction - Google Patents

Method of protecting graphite articles from destruction

Info

Publication number
SU596659A1
SU596659A1 SU762380937A SU2380937A SU596659A1 SU 596659 A1 SU596659 A1 SU 596659A1 SU 762380937 A SU762380937 A SU 762380937A SU 2380937 A SU2380937 A SU 2380937A SU 596659 A1 SU596659 A1 SU 596659A1
Authority
SU
USSR - Soviet Union
Prior art keywords
coating
graphite
vacuum
boron
products
Prior art date
Application number
SU762380937A
Other languages
Russian (ru)
Inventor
Сергей Сергеевич Кипарисов
Виктория Сергеевна Дергунова
Иван Александрович Соболь
Анатолий Николаевич Шуршаков
Нина Александровна Новикова
Original Assignee
Предприятие П/Я М-5409
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Предприятие П/Я М-5409 filed Critical Предприятие П/Я М-5409
Priority to SU762380937A priority Critical patent/SU596659A1/en
Application granted granted Critical
Publication of SU596659A1 publication Critical patent/SU596659A1/en

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C16/00Chemical coating by decomposition of gaseous compounds, without leaving reaction products of surface material in the coating, i.e. chemical vapour deposition [CVD] processes
    • C23C16/22Chemical coating by decomposition of gaseous compounds, without leaving reaction products of surface material in the coating, i.e. chemical vapour deposition [CVD] processes characterised by the deposition of inorganic material, other than metallic material
    • C23C16/30Deposition of compounds, mixtures or solid solutions, e.g. borides, carbides, nitrides
    • C23C16/34Nitrides
    • C23C16/342Boron nitride
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C16/00Chemical coating by decomposition of gaseous compounds, without leaving reaction products of surface material in the coating, i.e. chemical vapour deposition [CVD] processes
    • C23C16/22Chemical coating by decomposition of gaseous compounds, without leaving reaction products of surface material in the coating, i.e. chemical vapour deposition [CVD] processes characterised by the deposition of inorganic material, other than metallic material
    • C23C16/30Deposition of compounds, mixtures or solid solutions, e.g. borides, carbides, nitrides
    • C23C16/34Nitrides

Landscapes

  • Chemical & Material Sciences (AREA)
  • Inorganic Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Crystals, And After-Treatments Of Crystals (AREA)

Claims (3)

(54) СПОСОБ ЗАЩИТЫ ГРАФИТОВЫХ ИЗДЕЛИЙ ОТ РАЗРУШЕНИЯ , более плавок в вакууме и на воздухе, не загр зн ют расплавы посторонними примес ми, обеспечивают хорошую извле каемость слитков после охлаждени . Пример 1,На внутреннюю поверхность графитового тигл  диаметром 90x80 мм и высотой 50 мм нанос т покры тие нитрида бора пиролитическим осаждением из парогазовой смеси треххлори того бора, аммиака и азота в соотноше НИИ 2:1:10 при в течение 3 ч. Затем деталь пропитывают расплавленным кремнием при 1500°С в течение 15 мин, Пропитку детали ведут со стороны поверхности не защищенной покрытием.При необходимости перед пропиткой с нерабочей поверхности детали покрытие уда л ли. Полученное изделие выдерживает 8 плавок в вакууме и 6-8 плавок на во духе. П р и м е р 2. Нанесение покрыти  осуществл ют как в примере 1. Пропитку ведут в расплаве кремни , с 15% бора при 2000С в течение 30 мин. Полученное изделие выдерживает 15 гшавок в вакууме и 10-12 плавок на воздухе, П р и м е р 3. На внутреннюю;повер ность графитового тигл  нанос т покры тие из нитрида бора пиролитическим осаждением из парогазовой смеси .треххлористого бора, аммиака, и; а.зота в соотношении 1:1:8 при 1200с в течение 2 ч. Пропитку .ос.уществл ют как в примере 2, но при 1900°С в-течение 20 мин. Изделие выдерживает 8-3.0 плавок медного с.плава.-на воздухе и 10-15 плавок в вакууме. Предложенный способ позвол ет в 7-10 раз повысить срок эксплуатации изделий из графита при их контакте с расплавами металлов, Способ может быть использован дл  защитьг изделий из пористого графита, в частности ГМЗ, силицированного графита СГ-М, боросилицированного .графита БСГ-30, ПРОГ-24оЬ. Формула изобретени  , Способ защиты графитовых изделий от разрушени  путем пиролитического нанесени  на рабочую поверхность покрыти  из нитрида бора, о т л и ч аю щ и и с   тем, что, с целью повышени  стойкости изделий в процессе контактировани  с расплавленными металлами , изделие с пр.крытчем дополнительно пропитывают. расплавом кремни  или его сплава с.10-15% бора в вакууме 10 - фт,ст. при 15002100°С в течение .15-30 мин со стороны, не защиденнрй; цокрйтием. Источники/информации, прин тые во внимание при экспертизе: 1.. Патент США №3288573,кл.29-182.8, 1966. (54) METHOD FOR PROTECTING GRAPHITE PRODUCTS FROM DESTRUCTION, more melts in vacuum and in air, do not contaminate the melts with impurities, provide good extraction of ingots after cooling. Example 1: Boron nitride is coated on the inner surface of a graphite crucible with a diameter of 90x80 mm and a height of 50 mm by pyrolytic precipitation from a vapor-gas mixture of trichlorine boron, ammonia and nitrogen in the ratio of scientific research institute 2: 1: 10 for 3 hours. molten silicon at 1500 ° C for 15 min. The impregnation of the part is carried out on the surface side not protected by the coating. If necessary, the coating was removed from the non-working surface of the part before impregnation. The resulting product can withstand 8 heats in a vacuum and 6-8 heats in the spirit. EXAMPLE 2 The coating is carried out as in Example 1. The impregnation is carried out in a melt of silicon, with 15% boron at 2000 ° C for 30 minutes. The product obtained can withstand 15 gas columns in vacuum and 10–12 melts in air, Example 3. An internal coating of graphite crucible is coated with boron nitride by pyrolytic precipitation from a vapor-gas mixture of boron trichloride, ammonia, and; a.ot in a ratio of 1: 1: 8 at 1200 s for 2 hours. Impregnation of the os. is carried out as in example 2, but at 1900 ° C for 20 min. The product withstands 8-3.0 heats of copper sflav.-in the air and 10-15 heats in a vacuum. The proposed method makes it possible to increase the service life of graphite products by 7-10 times when they come into contact with metal melts. The method can be used to protect products from porous graphite, in particular GMP, siliconized SG-M, borosilicated graphite BSH-30, PROG-24o. Claims The method of protecting graphite products from destruction by pyrolytic coating of boron nitride coating on the working surface is so that, in order to increase the resistance of products in the process of contact with molten metals, Krytchem additionally soaked. melt of silicon or its alloy p.10-15% boron in a vacuum of 10 - ft, st. at 15002100 ° С for .15-30 minutes from the side, not zaschdennry; cling to Sources / information taken into account in the examination: 1 .. US Patent No. 3288573, CL 29-182.8, 1966. 2.Авторское свидетельство СССР № 350326, кл, В 22 В 41/10, 1971. 2. USSR author's certificate No. 350326, class, B 22 B 41/10, 1971. 3.Авторское свидетельство СССР fJ 460275, кл. С 04 Е 35/54, 1973. 4 о Авторское свидетельство СССР 420559, кл. С 01 В 31/04, 1971.3. USSR author's certificate fJ 460275, cl. C 04 E 35/54, 1973. 4 o Copyright Certificate of the USSR 420559, cl. From 01 to 31/04, 1971
SU762380937A 1976-06-30 1976-06-30 Method of protecting graphite articles from destruction SU596659A1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
SU762380937A SU596659A1 (en) 1976-06-30 1976-06-30 Method of protecting graphite articles from destruction

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
SU762380937A SU596659A1 (en) 1976-06-30 1976-06-30 Method of protecting graphite articles from destruction

Publications (1)

Publication Number Publication Date
SU596659A1 true SU596659A1 (en) 1978-02-08

Family

ID=20668732

Family Applications (1)

Application Number Title Priority Date Filing Date
SU762380937A SU596659A1 (en) 1976-06-30 1976-06-30 Method of protecting graphite articles from destruction

Country Status (1)

Country Link
SU (1) SU596659A1 (en)

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4402925A (en) * 1981-09-28 1983-09-06 Union Carbide Corporation Porous free standing pyrolytic boron nitride articles
US4849146A (en) * 1985-02-28 1989-07-18 Denki Kagaku Kogyo Kabushiki Kaisha Method for producing pyrolytic boron nitride article
RU2168557C2 (en) * 1996-04-02 2001-06-10 Адванст Керамикс Корпорейшн Method forming coatings based on pyrolytic silicon nitride which is boron
RU2319250C1 (en) * 2006-05-16 2008-03-10 Федеральное государственное унитарное предприятие "Научно-производственное предприятие "Алмаз" Traveling-wave tube

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4402925A (en) * 1981-09-28 1983-09-06 Union Carbide Corporation Porous free standing pyrolytic boron nitride articles
US4849146A (en) * 1985-02-28 1989-07-18 Denki Kagaku Kogyo Kabushiki Kaisha Method for producing pyrolytic boron nitride article
RU2168557C2 (en) * 1996-04-02 2001-06-10 Адванст Керамикс Корпорейшн Method forming coatings based on pyrolytic silicon nitride which is boron
RU2319250C1 (en) * 2006-05-16 2008-03-10 Федеральное государственное унитарное предприятие "Научно-производственное предприятие "Алмаз" Traveling-wave tube

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