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SK279429B6 - Method of liquid's composition and properties determination - Google Patents

Method of liquid's composition and properties determination Download PDF

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Publication number
SK279429B6
SK279429B6 SK3598-91A SK359891A SK279429B6 SK 279429 B6 SK279429 B6 SK 279429B6 SK 359891 A SK359891 A SK 359891A SK 279429 B6 SK279429 B6 SK 279429B6
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Slovakia
Prior art keywords
mercury
composition
liquid
properties
measured
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SK3598-91A
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Slovak (sk)
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SK359891A3 (en
Inventor
Jozef Polakovič
Jozefína Polakovičová
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Chemickotechnologická Fakulta Stu
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Publication of SK359891A3 publication Critical patent/SK359891A3/en
Publication of SK279429B6 publication Critical patent/SK279429B6/en

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Abstract

A capillary tube, with a longlife mercury drop, is dipped into a liquid sample to be measured. Mercury is dripping upon a mercury electrode while the charging current "in" and life length "tau" of a mercury drop dependency is continually measured. The liquid's composition and properties are determined according to time dependency of the charging current in = f (t).

Description

Vynález sa týka spôsobu na kontinuálne stanovenie zloženia a vlastností kvapalín, najmä odpadových vôd, na základe merania parametrov kvapiek ortuti.The invention relates to a method for continuously determining the composition and properties of liquids, in particular waste water, by measuring the parameters of mercury droplets.

Doterajší stav technikyBACKGROUND OF THE INVENTION

V súčasnosti sa na stanovenie zloženia kvapalín používajú rozličné polarografícké metódy, podstatou ktoiých je meranie parametrov kvapiek ortuti odkvapkávajúcej z kapiláry, najčastejšie meranie závislosti faradaického prúdu if od koncentrácie. Pri raste kvapky ortuti, ako dôsledok zväčšovania jej povrchu v kvapalnom prostredí, vždy vzniká nabíjací prúd i„. V klasickej polarografii je tento prúd nežiaduci, pretože sa superponuje s faradaickým prúdom if na celkový prúd ic, pričom platí:At present various polarographic methods are used to determine the composition of liquids, which is based on the measurement of the parameters of mercury droplets dripping from the capillary, most often the measurement of the dependence of the faradic current i f on the concentration. When a drop of mercury grows as a result of its surface increasing in a liquid environment, a charging current is always produced. In classical polarography, this stream is undesirable because it is superimposed with the faradic stream i f to the total stream i c , with:

lc lf t lnNakoľko pri analytických aplikáciách polarografických metód je dôležitá závislosť faradaického prúdu if, od koncentrácie, a nie závislosť celkového prúdu ic, ktorý je zaznamenávaný polarografom, vyvíja sa veľké úsilie na eliminovanie nabíjacieho prúdu in. Jeho meraniu a vyhodnocovaniu sa v súčasnosti nevenuje pozornosť, a preto nie sú známe a dostupné spôsoby na jeho meranie a vyhodnocovanie.I C - lf th n Since the polarographic methods of analysis applications, it is important dependent faradaic current i f, the concentration, and no dependence of the total current I C that is recorded polarography was developed to eliminate any charging current I n. Its measurement and evaluation is currently ignored and therefore there are no known and available ways to measure and evaluate it.

Podstata vynálezuSUMMARY OF THE INVENTION

Uvedenú problematiku rieši spôsob stanovenia zloženia a vlastností kvapalín, najmä odpadových vôd podľa vynálezu, ktorého podstatou je, že sa do vzorky meranej kvapaliny ponorí kapilára, z ktorej odkvapkáva ortuť na veľkoplošnú ortuťovú elektródu, pričom sa kontinuálne meria veľkosť nabíjacieho prúdu i„, čas τ života kvapky a z časovej závislosti nabíjacieho prúdu i„ = f(t) sa stanoví zloženie a vlastnosti kvapaliny, pričom sa meranie uskutočňuje pomocou kapiláry s dlhým časom života kvapky.A method for determining the composition and properties of liquids, in particular waste water according to the invention, consists in immersing a capillary into a sample of the liquid to be measured, from which mercury drips onto a large-area mercury electrode, continuously measuring the charge current i ", time τ The composition and properties of the liquid are determined and the measurement is performed by means of a capillary with a long lifetime of the drop.

Spôsob podľa vynálezu využíva skutočnosť, že z fyzikálno-chemického hľadiska časová závislosť i„ = f(t) reprezentuje vznikanie elektrickej dvojvrstvy na fázovom rozhraní ortuť-kvapalina v čase t a tým je nositeľom informácie o všetkých faktoroch, ktoré tento proces ovplyvňujú, t. j. predovšetkým zloženie a vlastnosti kvapaliny.The method according to the invention takes advantage of the fact that, from a physicochemical point of view, the time dependence i n = f (t) represents the formation of an electric bilayer at the mercury-liquid phase interface at time t and thus carries information about all factors influencing this process. j. especially the composition and properties of the liquid.

Výhodou spôsobu podľa vynálezu je, že jednoduchou cestou poskytuje informácie o zložení a vlastnostiach meranej kvapaliny. V prípade sledovania odpadových vôd tieto informácie sa môžu využiť na kontinuálne zisťovanie znečistenia alebo na jeho signalizáciu.An advantage of the method according to the invention is that it provides information on the composition and properties of the liquid to be measured in a simple way. In the case of waste water monitoring, this information may be used to continuously detect or signal pollution.

znázornená na obr. 1. Ako registračné zariadenie sa použil jednolíniový zapisovač. Ako vyplýva z obr. 1, možno získať kvantitatívne údaje o čase života ortuťovej kvapky τ, hodnote nabíjacieho prúdu (i„)max v maxime a priebehu nabíjacieho prúdu in počas tvorby ortuťovej kvapky i„ = f(t). Všetky tieto údaje sú zdrojom informácií o zložení a vlastnostiach sledovanej kvapaliny. Zistenie znečistenia, resp. zloženia sa zakladá na poznaní závislosti napr. času života ortuťovej kvapky od koncentrácie vodu znečisťujúcich látok. Na obr. 2, je znázornená takáto závislosť pre vodný roztok cetylpyridínium bromidu (CPBr). Ako vyplýva z obr. 2; citlivosť spôsobu je vysoká a umožňuje spoľahlivo rozlíšiť koncentrácie ΚΓ1 mol.drrí3 a 10'3 mol.dm'3 shown in FIG. 1. A single-line recorder was used as the recording device. As shown in FIG. 1, quantitative data on the mercury drop life time τ, the charge current value (i ") max at maximum and the charge current course i n during mercury drop formation i" = f (t) can be obtained. All these data are a source of information on the composition and properties of the liquid under investigation. Detection of contamination, resp. the composition is based on knowing the dependence e.g. mercury drop time from the concentration of water pollutants. In FIG. 2, such dependence is shown for an aqueous solution of cetylpyridinium bromide (CPBr). As shown in FIG. 2; the process sensitivity is high and allows to reliably distinguish concentrations of ΚΓ 1 mol.dr 3 and 10 ' 3 mol.dm 3

Signalizácia znečistenia vyžaduje registráciu závislosti in = f(t) v počítači. Signál o znečistení vznikne z porovnania hodnoty nameranej na kontrolovanej vode s referenčnou hodnotou τΓ. Ak sa zistí rozdiel (v prípade vodného roztoku CPBr - obr. 2 - sú tieto hodnoty napr. τ = 179 s a τΓ = 195 s), počítač vydá signál o znečistení alebo zistenú informáciu využije iným spôsobom.Pollution signaling requires registration of the dependence i n = f (t) in the computer. The pollution signal is generated by comparing the value measured on the controlled water with the reference value τ Γ . If a difference is found (in the case of an aqueous CPBr solution - Fig. 2 - these values are eg τ = 179 s τ Γ = 195 s), the computer gives a signal of contamination or uses the information found in another way.

Podobne sa môže postupovať pri využití časových závislostí (i„)max a i„Similarly, the time dependence of (i ") max and i"

Priemyselná využiteľnosťIndustrial usability

Vynález možno využiť najmä na kontinuálne zisťovanie zloženia a vlastností odpadových vôd a na okamžitú signalizáciu znečistenia.In particular, the invention can be used to continuously detect the composition and properties of wastewater and to promptly signal contamination.

Claims (2)

PATENTOVÉ NÁROKY Spôsob stanovenia zloženia a vlastností kvapalín, najmä odpadových vôd, pri ktorom sa do vzorky meranej kvapaliny ponorí kapilára, z ktorej odkvapkáva ortuť na veľkoplošnú ortuťovú elektródu, vyznačujúci sa tým, že sa kontinuálne meria veľkosť nabíjacieho prúdu in, čas τ života kvapky a z časovej závislosti nabíjacieho prúdu i„ = f(t) sa stanoví zloženie a vlastnosti kvapaliny, pričom sa meranie uskutočňuje pomocou kapiláry s dlhým časom života.A method for determining the composition and properties of liquids, in particular waste water, by immersing a capillary into a sample of the liquid to be measured, from which mercury drips onto a large-area mercury electrode, characterized in that the charge current in The time dependence of the charging current i = f (t) is determined by the composition and properties of the liquid, the measurement being carried out by means of a long life capillary. 1 výkres1 drawing Prehľad obrázkov na výkresochBRIEF DESCRIPTION OF THE DRAWINGS Na obr. 1 je znázornená časová závislosť nabíjacieho prúdu i„ = f(t) nameraná pre destilovanú vodu a na obr.In FIG. 1 shows the time dependence of the charging current i = f (t) measured for distilled water, and FIG. 2 je znázornená závislosť času τ života ortuťovej kvapky od koncentrácie znečistenia pre vodný roztok CPBr.2 shows the dependence of the mercury droplet life time τ on the contamination concentration for an aqueous solution of CPBr. Príklady uskutočnenia vynálezuDETAILED DESCRIPTION OF THE INVENTION PríkladExample Spôsobom podľa vynálezu sa merala časová závislosť nabíjacieho prúdu i„ = f(t) pre destilovanú vodu, ktorá jeThe method according to the invention measured the time dependence of the charging current i '= f (t) for distilled water, which is
SK3598-91A 1991-11-27 1991-11-27 Method of liquid's composition and properties determination SK279429B6 (en)

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CS359891 1991-11-27

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SK279429B6 true SK279429B6 (en) 1998-11-04

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Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2012150031A1 (en) 2011-05-04 2012-11-08 Samuel Grega Method for physically working and/or heating media, in particular liquids, and device for carrying out the method

Families Citing this family (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
UA108714C2 (en) * 2011-10-01 2015-05-25 THE METHOD OF SNOW AND DEVICE FOR THE IMPLEMENTATION OF THE METHOD

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2012150031A1 (en) 2011-05-04 2012-11-08 Samuel Grega Method for physically working and/or heating media, in particular liquids, and device for carrying out the method

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