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SE2350922A1 - Metal removal in recycling of cellulosic textiles - Google Patents

Metal removal in recycling of cellulosic textiles

Info

Publication number
SE2350922A1
SE2350922A1 SE2350922A SE2350922A SE2350922A1 SE 2350922 A1 SE2350922 A1 SE 2350922A1 SE 2350922 A SE2350922 A SE 2350922A SE 2350922 A SE2350922 A SE 2350922A SE 2350922 A1 SE2350922 A1 SE 2350922A1
Authority
SE
Sweden
Prior art keywords
during
cellulose
carried out
recycling
textile material
Prior art date
Application number
SE2350922A
Inventor
Gunnar Henriksson
Christoffersson Kristina Elg
Sara Starrsjö
Stefan Antonsson
Original Assignee
Circulose AB
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Circulose AB filed Critical Circulose AB
Priority to SE2350922A priority Critical patent/SE2350922A1/en
Priority to PCT/EP2024/069560 priority patent/WO2025021524A1/en
Priority to EP24743729.6A priority patent/EP4522800A1/en
Publication of SE2350922A1 publication Critical patent/SE2350922A1/en

Links

Classifications

    • DTEXTILES; PAPER
    • D01NATURAL OR MAN-MADE THREADS OR FIBRES; SPINNING
    • D01FCHEMICAL FEATURES IN THE MANUFACTURE OF ARTIFICIAL FILAMENTS, THREADS, FIBRES, BRISTLES OR RIBBONS; APPARATUS SPECIALLY ADAPTED FOR THE MANUFACTURE OF CARBON FILAMENTS
    • D01F13/00Recovery of starting material, waste material or solvents during the manufacture of artificial filaments or the like
    • D01F13/02Recovery of starting material, waste material or solvents during the manufacture of artificial filaments or the like of cellulose, cellulose derivatives or proteins
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08BPOLYSACCHARIDES; DERIVATIVES THEREOF
    • C08B16/00Regeneration of cellulose
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J11/00Recovery or working-up of waste materials
    • C08J11/04Recovery or working-up of waste materials of polymers
    • DTEXTILES; PAPER
    • D01NATURAL OR MAN-MADE THREADS OR FIBRES; SPINNING
    • D01FCHEMICAL FEATURES IN THE MANUFACTURE OF ARTIFICIAL FILAMENTS, THREADS, FIBRES, BRISTLES OR RIBBONS; APPARATUS SPECIALLY ADAPTED FOR THE MANUFACTURE OF CARBON FILAMENTS
    • D01F2/00Monocomponent artificial filaments or the like of cellulose or cellulose derivatives; Manufacture thereof
    • D01F2/02Monocomponent artificial filaments or the like of cellulose or cellulose derivatives; Manufacture thereof from solutions of cellulose in acids, bases or salts
    • DTEXTILES; PAPER
    • D21PAPER-MAKING; PRODUCTION OF CELLULOSE
    • D21CPRODUCTION OF CELLULOSE BY REMOVING NON-CELLULOSE SUBSTANCES FROM CELLULOSE-CONTAINING MATERIALS; REGENERATION OF PULPING LIQUORS; APPARATUS THEREFOR
    • D21C3/00Pulping cellulose-containing materials
    • D21C3/02Pulping cellulose-containing materials with inorganic bases or alkaline reacting compounds, e.g. sulfate processes
    • DTEXTILES; PAPER
    • D21PAPER-MAKING; PRODUCTION OF CELLULOSE
    • D21CPRODUCTION OF CELLULOSE BY REMOVING NON-CELLULOSE SUBSTANCES FROM CELLULOSE-CONTAINING MATERIALS; REGENERATION OF PULPING LIQUORS; APPARATUS THEREFOR
    • D21C3/00Pulping cellulose-containing materials
    • D21C3/22Other features of pulping processes
    • D21C3/222Use of compounds accelerating the pulping processes
    • DTEXTILES; PAPER
    • D21PAPER-MAKING; PRODUCTION OF CELLULOSE
    • D21CPRODUCTION OF CELLULOSE BY REMOVING NON-CELLULOSE SUBSTANCES FROM CELLULOSE-CONTAINING MATERIALS; REGENERATION OF PULPING LIQUORS; APPARATUS THEREFOR
    • D21C5/00Other processes for obtaining cellulose, e.g. cooking cotton linters ; Processes characterised by the choice of cellulose-containing starting materials
    • DTEXTILES; PAPER
    • D21PAPER-MAKING; PRODUCTION OF CELLULOSE
    • D21HPULP COMPOSITIONS; PREPARATION THEREOF NOT COVERED BY SUBCLASSES D21C OR D21D; IMPREGNATING OR COATING OF PAPER; TREATMENT OF FINISHED PAPER NOT COVERED BY CLASS B31 OR SUBCLASS D21G; PAPER NOT OTHERWISE PROVIDED FOR
    • D21H11/00Pulp or paper, comprising cellulose or lignocellulose fibres of natural origin only
    • D21H11/12Pulp from non-woody plants or crops, e.g. cotton, flax, straw, bagasse
    • DTEXTILES; PAPER
    • D21PAPER-MAKING; PRODUCTION OF CELLULOSE
    • D21HPULP COMPOSITIONS; PREPARATION THEREOF NOT COVERED BY SUBCLASSES D21C OR D21D; IMPREGNATING OR COATING OF PAPER; TREATMENT OF FINISHED PAPER NOT COVERED BY CLASS B31 OR SUBCLASS D21G; PAPER NOT OTHERWISE PROVIDED FOR
    • D21H11/00Pulp or paper, comprising cellulose or lignocellulose fibres of natural origin only
    • D21H11/14Secondary fibres
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02WCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00Technologies for solid waste management
    • Y02W30/50Reuse, recycling or recovery technologies
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02WCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00Technologies for solid waste management
    • Y02W30/50Reuse, recycling or recovery technologies
    • Y02W30/66Disintegrating fibre-containing textile articles to obtain fibres for re-use

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Medicinal Chemistry (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Textile Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Polymers & Plastics (AREA)
  • Sustainable Development (AREA)
  • Biochemistry (AREA)
  • Materials Engineering (AREA)
  • Inorganic Chemistry (AREA)
  • Chemical Or Physical Treatment Of Fibers (AREA)
  • Processing Of Solid Wastes (AREA)
  • Paper (AREA)

Abstract

A method for removal of metal ions during recycling of textiles comprising cellulose, said method comprising the sequential steps of providing at least one textile material comprising cellulose, treating the material to swell the cellulose, under alkaline and reducing conditions, wherein at least one reducing agent is present at least during a part of the swelling, and treating the material according to at least one of the following steps: i) decreasing the pH to 5.5 or below, and ii) adding a chelating agent. The metal ion content of the material is thereby reduced. The process gives a more efficient metal removal during textile recycling.

Claims (20)

Claims
1. A method for removal of metal ions during recycling of textiles comprising cellulose, said method comprising the sequential steps of: a.providing at least one textile material comprising cellulose, b.treating the material to swell the cellulose, under alkaline and reducing conditions, wherein at least one reducing agent is present at least during a part of the swelling, and c.treating the material according to at least one of the following steps: i. decreasing the pH to 5.5 or below, and ii. adding a chelating agent.
2. The method according to claim 1, wherein the at least one textile material comprises at least one selected from the group consisting of cotton, and viscose. lyocell, rayon,
3. The method according to claim 1, wherein the at least one textile material comprises cotton.
4. The method according to any one of claims 1-3, wherein the at least one textile material is mechanically disintegrated before step b).
5. The method according to any one of claims 1-4, wherein the pH during step b) is above 7.
6. The method according to any one of claims 1-5, wherein the pH during step b) is in the range of 9-13.
7. The method according to any one of claims 1-6, wherein NaOH is present during step b) in a concentration from 0.01 to 0.5 mol/l.
8. The method according to any one of claims 1-7, wherein the temperature during step b) is in the range 50-°C.
9. The method according to any one of claims 1-8, wherein the at least one reducing agent comprises sodium dithionite, Na2SflM.
10. The method according to any one of claims 1-9, wherein step c i) is performed and the pH is decreased in step c i) to below
11. The method according to any one of claims 1-10, wherein step c i) is performed and the pH is decreased by addition of at least one of CO2 and HQCO
12. The method according to any one of claims 1-11, wherein step c i) is carried out at a temperature in the interval 60-120 °C.
13. The method according to any one of claims 1-12, wherein step c i) is carried out during 20 minutes-24 hours.
14. The method according to any one of claims 1-13, wherein step c ii) is performed and the chelating agent is EDTA.
15. The method according to any one of claims 1-14, wherein step c ii) is carried out at a temperature in the interval 40-100 °C.
16. The method according to any one of claims 1-15, wherein step c ii)
17. The method according to any one of claims 1-16, wherein a wash is carried out before step c).
18. The method according to any one of claims 1-17, wherein the material is dewatered to a water content of less than 66 wt% before step c).
19. Recycled cellulose material obtained by the method according to any one of claims 1-
20. Use of recycled cellulosic material according to claim 19 in a process for production of viscose. is carried out during 20 minutes-24 hours.
SE2350922A 2023-07-25 2023-07-25 Metal removal in recycling of cellulosic textiles SE2350922A1 (en)

Priority Applications (3)

Application Number Priority Date Filing Date Title
SE2350922A SE2350922A1 (en) 2023-07-25 2023-07-25 Metal removal in recycling of cellulosic textiles
PCT/EP2024/069560 WO2025021524A1 (en) 2023-07-25 2024-07-10 Metal removal in recycling of cellulosic textiles
EP24743729.6A EP4522800A1 (en) 2023-07-25 2024-07-10 Metal removal in recycling of cellulosic textiles

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
SE2350922A SE2350922A1 (en) 2023-07-25 2023-07-25 Metal removal in recycling of cellulosic textiles

Publications (1)

Publication Number Publication Date
SE2350922A1 true SE2350922A1 (en) 2025-01-26

Family

ID=91958965

Family Applications (1)

Application Number Title Priority Date Filing Date
SE2350922A SE2350922A1 (en) 2023-07-25 2023-07-25 Metal removal in recycling of cellulosic textiles

Country Status (3)

Country Link
EP (1) EP4522800A1 (en)
SE (1) SE2350922A1 (en)
WO (1) WO2025021524A1 (en)

Citations (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2015077807A1 (en) * 2013-11-26 2015-06-04 Lenzing Ag Process for pretreating reclaimed cotton fibres to be used in the production of moulded bodies from regenerated cellulose
WO2018073177A1 (en) * 2016-10-19 2018-04-26 Re:Newcell Ab Recycling of cellulosic textiles
WO2018104330A1 (en) * 2016-12-06 2018-06-14 Re:Newcell Ab Cellulose fibers
WO2021185704A1 (en) * 2020-03-16 2021-09-23 Re:Newcell Ab One stage method for acid metal rewoval and bleach
WO2022139651A1 (en) * 2020-12-21 2022-06-30 Valmet Ab Method for bleaching pulp from recycled textile material
CN115536754A (en) * 2022-09-20 2022-12-30 赛得利(江苏)纤维有限公司 Production process of wet pulp for producing viscose by recycling cotton textiles

Family Cites Families (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20030019596A1 (en) * 2001-04-17 2003-01-30 Ragauskas Arthur J. Metal substituted xerogels for improved peroxide bleaching of kraft pulps
PT2817448T (en) 2012-02-20 2017-02-21 Re:Newcell Ab Regeneration of cellulose

Patent Citations (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2015077807A1 (en) * 2013-11-26 2015-06-04 Lenzing Ag Process for pretreating reclaimed cotton fibres to be used in the production of moulded bodies from regenerated cellulose
WO2018073177A1 (en) * 2016-10-19 2018-04-26 Re:Newcell Ab Recycling of cellulosic textiles
WO2018104330A1 (en) * 2016-12-06 2018-06-14 Re:Newcell Ab Cellulose fibers
WO2021185704A1 (en) * 2020-03-16 2021-09-23 Re:Newcell Ab One stage method for acid metal rewoval and bleach
WO2022139651A1 (en) * 2020-12-21 2022-06-30 Valmet Ab Method for bleaching pulp from recycled textile material
CN115536754A (en) * 2022-09-20 2022-12-30 赛得利(江苏)纤维有限公司 Production process of wet pulp for producing viscose by recycling cotton textiles

Also Published As

Publication number Publication date
WO2025021524A1 (en) 2025-01-30
EP4522800A1 (en) 2025-03-19

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