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RU2030411C1 - Di-(2-tetrahydrofurylhydroxy)propane as a reagent for etching of paint and varnish coating - Google Patents

Di-(2-tetrahydrofurylhydroxy)propane as a reagent for etching of paint and varnish coating Download PDF

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RU2030411C1
RU2030411C1 SU4951963A RU2030411C1 RU 2030411 C1 RU2030411 C1 RU 2030411C1 SU 4951963 A SU4951963 A SU 4951963A RU 2030411 C1 RU2030411 C1 RU 2030411C1
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reagent
paint
propane
enamel
tetrahydrofurylhydroxy
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Russian (ru)
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Ю.Н. Поливин
Р.А. Караханов
М.В. Трофимова
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Государственная академия нефти и газа им.И.М.Губкина
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Abstract

FIELD: paint and varnish industry. SUBSTANCE: product: di-(2-tetrahydrofurylhydroxy)propane (I), empirical formula is C11H20O4, b. p. is 115-117 C/5 mm mercury column. Reagent 1: 2,5-dihydrofuran. Reagent 2: propandiol-1,3. Process conditions: molar ratio of reagents is 2:1 at 35-40 C. At 20 C compound (I) removes up to metal for 10 min 2 layers of enamel ПФ-223, АС-1115 (priming АR-069) - 15 min and enamel АС-1115 (priming АК-070) - 20 min. Compound (I) removes paint and varnish coating by 3-fold more rapidly as compared with that of N-methylpyrrolodone-2. EFFECT: increased effectiveness of reagent proposed. 1 tbl

Description

Изобретение относится к новому химическому соединению - ди-(2-тетрагидрофурилокси)-пропану (1), который может быть использован в качестве реагента для травления лакокрасочных покрытий (ЛКП). The invention relates to a new chemical compound - di- (2-tetrahydrofuryloxy) -propane (1), which can be used as a reagent for etching coatings (LCP).

Известно, что в качестве реагента для снятия лакокрасочного покрытия применяется N-метилпирролидон-2 формулы [1]. It is known that N-methylpyrrolidone-2 of the formula [1] is used as a reagent for removing paintwork.

Целью изобретения является изыскание реагента, позволяющего увеличить скорость снятия лакокрасочного покрытия с поверхности металла. The aim of the invention is to find a reagent that can increase the speed of removal of the paintwork from the metal surface.

Поставленная цель достигается тем, что в качестве такого реагента применяется ди-(2-тетрагидрокси)пропан, которое получают при смешивании 2,5-дигидрофурана и пропандиола-1,3 в присутствии соляной кислоты. The goal is achieved in that as such a reagent, di- (2-tetrahydroxy) propane is used, which is obtained by mixing 2,5-dihydrofuran and propanediol-1,3 in the presence of hydrochloric acid.

П р и м е р. К 1 моль пропандиол-1,3 добавляют 1-2 капли конц. HCl и прибавляют 2 моль 2,5-дигидрофурана с такой скоростью, чтобы температура реакционной смеси не превышала 35-40оС. Смесь оставляют стоять на ночь и затем реакционную смесь разлагают 0,1 н.раствором КОН. Водный слой отделяют, экстрагируют эфиром. Органический слой объединяют с эфирными вытяжками, сушат, растворитель отгоняют. Остаток перегоняют под вакуумом собирают фракцию 115-117оС 5 мм рт.ст.). Выход 0,84 моля (84%).PRI me R. To 1 mol of propanediol-1,3 add 1-2 drops conc. HCl and add 2 mol of 2,5-dihydrofuran at a rate such that the temperature of the reaction mixture did not exceed 35-40 ° C. The mixture was allowed to stand overnight and then the reaction mixture was decomposed with 0.1 n.rastvorom KOH. The aqueous layer was separated, extracted with ether. The organic layer is combined with ether extracts, dried, the solvent is distilled off. The residue is distilled under vacuum and the fraction 115-117 ° C 5 mm Hg). Yield 0.84 mol (84%).

Структура полученного соединения была доказана с помощью элементного анализа, данным ПМР и масс-спектров. Брутто-формула С11Н20О4.The structure of the obtained compound was proved using elemental analysis, data of PMR and mass spectra. The gross formula is C 11 H 20 O 4 .

Вычислено/найдено, мас.%: C 61,09/61,24; H 9,38/9,16. Calculated / found, wt.%: C 61.09 / 61.24; H 9.38 / 9.16.

m/z (Iотн): [M] +. 216 (01); [M-H]+ 215 (1); [M-CH2O]+ 186 (0,5); [M-C4H7O] + 145 (60); [M--C4H7O2] + 129 (50); [C4H7O2] + 87 (98); [C4H7O] + 71 (100); (б,м.д.): 1,8 м (2Н), 2,0 м (8Н), 3,8 м (4Н), 4,1 (4Н), 5,1 т (2Н).m / z (I Rel ): [M] +. 216 (01); [MH] + 215 (1); [M-CH 2 O] + 186 (0.5); [MC 4 H 7 O] + 145 (60); [M - C 4 H 7 O 2 ] + 129 (50); [C 4 H 7 O 2 ] + 87 (98); [C 4 H 7 O] + 71 (100); (b, ppm): 1.8 m (2H), 2.0 m (8H), 3.8 m (4H), 4.1 (4H), 5.1 t (2H).

Для экспериментальной проверки моющих свойств соединения 1 была исследована моющая способность по отношению к двум слоям эмали АС-1115 с подложками грунтов АК-069 и АК-070 соответственно, а также по отношению к двум слоям эмали ПФ-223. Нанесение грунта и эмали ведут пульверизатором, причем толщина слоя покрытия равна 40 г/м2 поверхности. На слой эмали наносят испытуемое соединение, которое выдерживают определенное время при 20оС, далее краситель снимают с поверхности металла.For an experimental verification of the washing properties of compound 1, the washing ability was studied with respect to two layers of AC-1115 enamel with soil substrates AK-069 and AK-070, respectively, as well as with respect to two layers of PF-223 enamel. The application of soil and enamel is carried out with a spray, and the thickness of the coating layer is 40 g / m 2 surface. On the enamel layer is applied to the test compound, which can withstand a certain time at 20 ° C, further dye is removed from the metal surface.

Соединение I вводили в рецептуру технического моющего средства "АФТ-1", используемого для удаления старых ЛКП, вместо органического растворителя в количестве 84%. Данные испытаний даны в таблице. Compound I was introduced into the formulation of the technical detergent "AFT-1" used to remove old paintwork, instead of an organic solvent in an amount of 84%. Test data are given in the table.

В аналогичных условиях 2 слоя эмали АС-1115 со слоем грунта АК-069 снимается за 50 мин, 2 слоя эмали АС-1115 и слой грунта АК-070 - 60 мин, 2 слоя эмали ПФ-223 - за 40 мин. N-метилпирролидоном-2. Under similar conditions, 2 layers of AC-1115 enamel with a layer of soil AK-069 can be removed in 50 minutes, 2 layers of enamel AC-1115 and a layer of soil AK-070 - 60 minutes, 2 layers of enamel PF-223 - in 40 minutes. N-methylpyrrolidone-2.

Таким образом, соединение 1 при 20оС за 10 мин удаляют до металла 2 слоя ПФ-223. Время удаления эмали АС-1115 (грунт АК-069) - 15 мин и эмали АС-1115 (грунт АК-070) - 20 мин. Удаление ЛКП соединением I в три раза быстрее, чем чистым N-метилпирролидоном-2.Thus, compound 1 at 20 ° C for 10 min to remove metal 2 PF-223 layer. The removal time of the AC-1115 enamel (AK-069 primer) is 15 minutes and the AC-1115 enamel (AK-070 primer) is 20 minutes. Removing LCP with compound I is three times faster than with pure N-methylpyrrolidone-2.

Claims (1)

ДИ-(2-ТЕТРАГИДРОФУРИЛОКСИ)ПРОПАН В КАЧЕСТВЕ РЕАГЕНТА ДЛЯ ТРАВЛЕНИЯ ЛАКОКРАСОЧНЫХ ПОКРЫТИЙ. DI- (2-TETRAHYDROFURILOXY) PROPANE AS A REAGENT FOR ETCHING OF PAINT AND COATINGS. Ди-(2-тетрагидрофурилокси)пропан формулы
Figure 00000001

в качестве реагента для травления лакокрасочных покрытий.
Di- (2-tetrahydrofuryloxy) propane of the formula
Figure 00000001

as a reagent for etching coatings.
SU4951963 1991-06-28 1991-06-28 Di-(2-tetrahydrofurylhydroxy)propane as a reagent for etching of paint and varnish coating RU2030411C1 (en)

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Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
Авторское свидетельство СССР N 998500, кл. C 11D 3/48, 1981. *

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