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RU2010139087A - MOX FUEL DISSOLUTION METHOD - Google Patents

MOX FUEL DISSOLUTION METHOD Download PDF

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Publication number
RU2010139087A
RU2010139087A RU2010139087/05A RU2010139087A RU2010139087A RU 2010139087 A RU2010139087 A RU 2010139087A RU 2010139087/05 A RU2010139087/05 A RU 2010139087/05A RU 2010139087 A RU2010139087 A RU 2010139087A RU 2010139087 A RU2010139087 A RU 2010139087A
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RU
Russia
Prior art keywords
solution
gadolinium
nitric acid
dissolution
mol
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Application number
RU2010139087/05A
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Russian (ru)
Other versions
RU2451639C1 (en
Inventor
Сергей Николаевич Круглов (RU)
Сергей Николаевич Круглов
Анатолий Степанович Козырев (RU)
Анатолий Степанович Козырев
Валерий Владимирович Лазарчук (RU)
Валерий Владимирович Лазарчук
Александр Сергеевич Рябов (RU)
Александр Сергеевич Рябов
Андрей Иванович Сильченко (RU)
Андрей Иванович Сильченко
Елена Валерьевна Малышева (RU)
Елена Валерьевна Малышева
Михаил Григорьевич Поморцев (RU)
Михаил Григорьевич Поморцев
Николай Владимирович Дедов (RU)
Николай Владимирович Дедов
Original Assignee
Открытое акционерное общество "Сибирский химический комбинат" (RU)
Открытое акционерное общество "Сибирский химический комбинат"
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Application filed by Открытое акционерное общество "Сибирский химический комбинат" (RU), Открытое акционерное общество "Сибирский химический комбинат" filed Critical Открытое акционерное общество "Сибирский химический комбинат" (RU)
Priority to RU2010139087/05A priority Critical patent/RU2451639C1/en
Publication of RU2010139087A publication Critical patent/RU2010139087A/en
Application granted granted Critical
Publication of RU2451639C1 publication Critical patent/RU2451639C1/en

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    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E30/00Energy generation of nuclear origin
    • Y02E30/30Nuclear fission reactors

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  • Inorganic Compounds Of Heavy Metals (AREA)

Abstract

1. Способ растворения МОКС-топлива в растворе азотной кислоты с использованием фтор-иона и гадолиния, отличающийся тем, что растворение осуществляют при одновременном присутствии в растворе ионов фтора и гадолиния при следующих концентрациях в растворе: азотной кислоты (6-9) моль/л, фторида натрия (0,05-0,08) моль/л и нитрата гадолиния в пересчете на гадолиний (1,3-1,5) г/л. ! 2. Способ по п.1, отличающийся тем, что растворяют топливо состава: диоксид природного урана UO2 74-76 мас.%; диоксид оружейного плутония PuO2 24-26 мас.%, которое было получено плазмохимической денитрацией раствора азотнокислых солей урана и плутония. ! 3. Способ по п.1, отличающийся тем, что растворение осуществляют в течение трех суток при температуре 20-25°С, после чего к нерастворившемуся остатку приливают новую порцию раствора. 1. A method of dissolving MOX fuel in a nitric acid solution using a fluorine ion and gadolinium, characterized in that the dissolution is carried out with the simultaneous presence of fluorine and gadolinium ions in the solution at the following concentrations in the solution: nitric acid (6-9) mol / l , sodium fluoride (0.05-0.08) mol / l and gadolinium nitrate in terms of gadolinium (1.3-1.5) g / l. ! 2. The method according to claim 1, characterized in that dissolve the fuel composition: natural uranium dioxide UO2 74-76 wt.%; weapons-grade plutonium dioxide PuO2 24-26 wt.%, which was obtained by plasma-chemical denitration of a solution of nitric acid salts of uranium and plutonium. ! 3. The method according to claim 1, characterized in that the dissolution is carried out for three days at a temperature of 20-25 ° C, after which a new portion of the solution is poured to the undissolved residue.

Claims (3)

1. Способ растворения МОКС-топлива в растворе азотной кислоты с использованием фтор-иона и гадолиния, отличающийся тем, что растворение осуществляют при одновременном присутствии в растворе ионов фтора и гадолиния при следующих концентрациях в растворе: азотной кислоты (6-9) моль/л, фторида натрия (0,05-0,08) моль/л и нитрата гадолиния в пересчете на гадолиний (1,3-1,5) г/л.1. The method of dissolving MOX fuel in a solution of nitric acid using fluorine ion and gadolinium, characterized in that the dissolution is carried out with the simultaneous presence of fluorine and gadolinium ions in the solution at the following concentrations in the solution: nitric acid (6-9) mol / l , sodium fluoride (0.05-0.08) mol / L and gadolinium nitrate in terms of gadolinium (1.3-1.5) g / L. 2. Способ по п.1, отличающийся тем, что растворяют топливо состава: диоксид природного урана UO2 74-76 мас.%; диоксид оружейного плутония PuO2 24-26 мас.%, которое было получено плазмохимической денитрацией раствора азотнокислых солей урана и плутония.2. The method according to claim 1, characterized in that they dissolve the fuel composition: natural uranium dioxide UO 2 74-76 wt.%; weapons-grade plutonium dioxide PuO 2 24-26 wt.%, which was obtained by plasma-chemical denitration of a solution of nitrate salts of uranium and plutonium. 3. Способ по п.1, отличающийся тем, что растворение осуществляют в течение трех суток при температуре 20-25°С, после чего к нерастворившемуся остатку приливают новую порцию раствора. 3. The method according to claim 1, characterized in that the dissolution is carried out for three days at a temperature of 20-25 ° C, after which a new portion of the solution is added to the insoluble residue.
RU2010139087/05A 2010-09-22 2010-09-22 Method of dissolving mox fuel RU2451639C1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
RU2010139087/05A RU2451639C1 (en) 2010-09-22 2010-09-22 Method of dissolving mox fuel

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
RU2010139087/05A RU2451639C1 (en) 2010-09-22 2010-09-22 Method of dissolving mox fuel

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RU2010139087A true RU2010139087A (en) 2012-03-27
RU2451639C1 RU2451639C1 (en) 2012-05-27

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* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
RU2704310C1 (en) * 2019-04-30 2019-10-28 Федеральное государственное унитарное предприятие "Горно-химический комбинат" (ФГУП "ГХК") Method for dissolving off-grade pelletized products of mox-fuel production
RU2754354C1 (en) * 2021-01-11 2021-09-01 Федеральное государственное унитарное предприятие "Горно-химический комбинат" (ФГУП "ГХК") Method for dissolving substandard products of mox fuel production

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FR2742254B1 (en) * 1995-12-12 1998-02-13 Comurhex PROCESS FOR OBTAINING A MIXTURE OF POWDERY METAL OXIDES, BELONGING TO THE NUCLEAR INDUSTRY, FROM THEIR NITRATES
RU2112744C1 (en) * 1996-09-17 1998-06-10 Сибирский химический комбинат Method of processing high-concentration uranium
RU2203225C2 (en) * 1998-05-15 2003-04-27 Мазин Владимир Ильич Uranium hexafluoride conversion method
JP4312969B2 (en) * 2001-03-02 2009-08-12 東京電力株式会社 Reprocessing method of spent nuclear fuel

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Effective date: 20120923