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RU2054758C1 - Process of manufacture of base of electrode of chemical source of energy - Google Patents

Process of manufacture of base of electrode of chemical source of energy Download PDF

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RU2054758C1
RU2054758C1 RU92003415/07A RU92003415A RU2054758C1 RU 2054758 C1 RU2054758 C1 RU 2054758C1 RU 92003415/07 A RU92003415/07 A RU 92003415/07A RU 92003415 A RU92003415 A RU 92003415A RU 2054758 C1 RU2054758 C1 RU 2054758C1
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nickel
electrode
base
manufacture
metallization
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RU92003415/07A
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RU92003415A (en
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Алексей Борисович Степанов
Игорь Николаевич Варакин
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Алексей Борисович Степанов
Игорь Николаевич Варакин
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Priority to RU92003415/07A priority Critical patent/RU2054758C1/en
Priority to SK447-97A priority patent/SK283829B6/en
Priority to PCT/RU1995/000170 priority patent/WO1997007554A1/en
Priority claimed from PCT/RU1995/000170 external-priority patent/WO1997007554A1/en
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Publication of RU2054758C1 publication Critical patent/RU2054758C1/en
Publication of RU92003415A publication Critical patent/RU92003415A/en

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    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/02Electrodes composed of, or comprising, active material
    • H01M4/64Carriers or collectors
    • H01M4/66Selection of materials
    • H01M4/668Composites of electroconductive material and synthetic resins
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C18/00Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating
    • C23C18/16Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating by reduction or substitution, e.g. electroless plating
    • C23C18/1601Process or apparatus
    • C23C18/1633Process of electroless plating
    • C23C18/1635Composition of the substrate
    • C23C18/1639Substrates other than metallic, e.g. inorganic or organic or non-conductive
    • C23C18/1641Organic substrates, e.g. resin, plastic
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C18/00Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating
    • C23C18/16Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating by reduction or substitution, e.g. electroless plating
    • C23C18/1601Process or apparatus
    • C23C18/1633Process of electroless plating
    • C23C18/1655Process features
    • C23C18/1658Process features with two steps starting with metal deposition followed by addition of reducing agent
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C18/00Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating
    • C23C18/16Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating by reduction or substitution, e.g. electroless plating
    • C23C18/18Pretreatment of the material to be coated
    • C23C18/20Pretreatment of the material to be coated of organic surfaces, e.g. resins
    • C23C18/28Sensitising or activating
    • C23C18/30Activating or accelerating or sensitising with palladium or other noble metal
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C18/00Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating
    • C23C18/16Chemical coating by decomposition of either liquid compounds or solutions of the coating forming compounds, without leaving reaction products of surface material in the coating; Contact plating by reduction or substitution, e.g. electroless plating
    • C23C18/31Coating with metals
    • C23C18/32Coating with nickel, cobalt or mixtures thereof with phosphorus or boron
    • C23C18/34Coating with nickel, cobalt or mixtures thereof with phosphorus or boron using reducing agents
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/02Electrodes composed of, or comprising, active material
    • H01M4/64Carriers or collectors
    • H01M4/66Selection of materials
    • H01M4/661Metal or alloys, e.g. alloy coatings
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00Electrodes
    • H01M4/02Electrodes composed of, or comprising, active material
    • H01M4/64Carriers or collectors
    • H01M4/66Selection of materials
    • H01M4/665Composites
    • H01M4/667Composites in the form of layers, e.g. coatings
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00Secondary cells; Manufacture thereof
    • H01M10/06Lead-acid accumulators
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M10/00Secondary cells; Manufacture thereof
    • H01M10/24Alkaline accumulators
    • H01M10/30Nickel accumulators
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10Energy storage using batteries
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50Manufacturing or production processes characterised by the final manufactured product

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  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Electrochemistry (AREA)
  • Composite Materials (AREA)
  • Inorganic Chemistry (AREA)
  • Chemically Coating (AREA)
  • Electroplating Methods And Accessories (AREA)
  • Battery Electrode And Active Subsutance (AREA)

Abstract

FIELD: electrical engineering. SUBSTANCE: base of unwoven fibre polymer material with exchange capacitance in cations 0.5-6.0 mg-ekV/g is activated by saturation with ions of nickel followed by treatment in aqueous solution of boron hydrate of alkali metal with concentration 0.1-1.2 g/l at temperature 15-70 C for the course of 0.5-30 min. Chemical and galvanic metallizations are conducted after it. EFFECT: exclusion of usage of scarce materials in process of manufacture and prevention of decay of metallization solution. 1 tbl

Description

Изобретение относится к электротехнике и может быть использовано для изготовления электродов химических источников тока, например никель-кадмиевых и свинцовых аккумуляторов. The invention relates to electrical engineering and can be used for the manufacture of electrodes of chemical current sources, for example, Nickel-cadmium and lead batteries.

Известна конструкция электродов, которые изготавливают металлизацией полимерной подложки с последующим осаждением активного материала [1]
Наиболее близкий по технической сущности и достигаемому эффекту к предлагаемому изобретению способ изготовления основ электродов такой конструкции [2] состоит в активации нетканого полотна из полимерных, например полиолефиновых, волокон в растворе, содержащем олово и палладий, химическом никелировании полотна и гальваническом никелировании.
A known design of electrodes that are made by metallization of a polymer substrate with subsequent deposition of the active material [1]
The closest in technical essence and the achieved effect to the proposed invention, a method of manufacturing the bases of electrodes of this design [2] consists in activating a non-woven fabric from polymer, for example polyolefin, fibers in a solution containing tin and palladium, chemical nickel plating and galvanic nickel plating.

Недостатками прототипа являются использование больших количеств олова и применение дорогостоящего палладия. Расход палладия в случае металлизации волокнистых материалов оказывается особенно большим из-за развитой металлизируемой поверхности. При металлизации подготовленного таким образом полимерного волокнистого материала высока вероятность разложения раствора металлизации на случайно попавших в раствор с поверхности полимера частицах палладия. The disadvantages of the prototype are the use of large quantities of tin and the use of expensive palladium. The consumption of palladium in the case of metallization of fibrous materials is especially large due to the developed metallized surface. During metallization of a polymer fibrous material prepared in this way, there is a high probability of decomposition of the metallization solution into palladium particles that accidentally enter the solution from the polymer surface.

Целью изобретения является замена палладия и олова не менее дефицитные материалы. The aim of the invention is the replacement of palladium and tin no less scarce materials.

Цель достигается тем, что в качестве полимерного волокнистого материала берут материал обменной емкостью по катионам 0,5-6 мг-экв/г, а перед металлизацией проводят насыщение полимерного материала ионами никеля с последующей обработкой раствором, содержащим борогидрид щелочного металла при концентрации 0,1-1,2 г/л при температуре 15-70оС в течение 0,5-30 мин.The goal is achieved by the fact that as a polymer fibrous material, a material with an exchange capacity of cations of 0.5-6 mEq / g is taken, and before metallization, the polymer material is saturated with nickel ions, followed by treatment with a solution containing alkali metal borohydride at a concentration of 0.1 -1.2 g / l at a temperature of 15-70 ° C for 0.5-30 min.

Указанные параметры волокнистого материала и процесса активации являются оптимальными. При обменной емкости менее 0,5 мг-экв/г количество сорбированного никеля недостаточно для проведения активации, гарантирующей металлизацию всей поверхности волокон. При обменной емкости более 6 мг-экв/г никель расходуется нерационально, волокно в растворе металлизации и в электролите аккумулятора, что снижает прочность волокон и приводит к отслоению металлического покрытия. The specified parameters of the fibrous material and the activation process are optimal. When the exchange capacity is less than 0.5 mEq / g, the amount of sorbed nickel is not enough to carry out activation, which guarantees the metallization of the entire surface of the fibers. With an exchange capacity of more than 6 mEq / g, nickel is consumed irrationally, the fiber in the metallization solution and in the battery electrolyte, which reduces the strength of the fibers and leads to delamination of the metal coating.

При содержании борогидрида менее 0,1 г/л сорбированный никель не восстанавливается, а при содержании более 1,2 г/л большая часть его разлагается, не взаимодействуя с никелем. With a borohydride content of less than 0.1 g / l, sorbed nickel is not reduced, and with a content of more than 1.2 g / l, most of it decomposes without interacting with nickel.

При температуре ниже 15оС раствор борогидрида не восстанавливает сорбированный волокном никель, а при температуре выше 70оС разложение борогидрида происходит чрезмерно быстро и основная часть его расходуется непроизводительно.At temperatures below 15 ° C restores borohydride solution is sorbed fiber nickel, and at a temperature above 70 ° C the decomposition occurs too quickly borohydride and the main part of it is consumed unproductively.

При продолжительности обработки в растворе борогидрида менее 0,5 мин сорбированный никель не успевает восстановиться, а при обработке в течение более 30 мин борогидрид успевает полностью израсходоваться. If the duration of treatment in a borohydride solution is less than 0.5 min, sorbed nickel does not have time to recover, and if it is processed for more than 30 minutes, borohydride has time to completely be consumed.

Сущность предлагаемого изобретения поясняется следующими примерами. The essence of the invention is illustrated by the following examples.

П р и м е р 1. В качестве полимерного волокнистого катионообменного материала использован нетканый иглопробивной войлок на основе радиационно привитого полипропилена с обменной емкостью по никелю 5 мг-экв/г, с диаметром волокон 36 мкм, пористостью 87% с толщиной полотна 5 мм. Насыщение никелем проведено путем часовой выдержки войлока в водном растворе гидрокарбоната натрия с концентрацией 2% промывки деионизованной водой, получасовой обработки в растворе сернокислого никеля с концентрацией 3% и промывки. Насыщенные никелем заготовки обработаны в течение 15 мин при 50оС в растворе борогидрида натрия с концентрацией 0,5 г/л, содержащем добавку 2 г/л карбоната натрия. При обработке заготовки приобретают темно-серый цвет. Активированные таким образом заготовки химически заникелированы при комнатной температуре в растворе состава, г/л: Сернокислый никель 50 Хлористый аммоний 35
Фосфорноватистокислый натрий 40 Аммиак До рН 9
Затем заготовки никелированы гальванически в стандартной ванне Уотса до содержания никеля 0,5 г/см3. В таблице характеристики изготовленной таким образом электродной основы сопоставлены с изученными характеристиками электродной основы положительного электрода никель-кадмиевого аккумулятора типа Н фирмы "Hoppecke", конструкция которого аналогична описанной в аналоге и прототипе.
EXAMPLE 1. A nonwoven needle-punched felt based on radiation grafted polypropylene with a nickel exchange capacity of 5 mEq / g, with a fiber diameter of 36 μm, porosity of 87% and a web thickness of 5 mm was used as a polymer fibrous cation exchange material. Nickel saturation was carried out by hourly exposure of felt in an aqueous solution of sodium hydrogen carbonate with a concentration of 2% washing with deionized water, a half-hour treatment in a solution of nickel sulfate with a concentration of 3% and washing. Saturated nickel workpiece processed for 15 minutes at 50 ° C in sodium borohydride solution with a concentration of 0.5 g / L, comprising fines of 2 g / l of sodium carbonate. When processing workpieces acquire a dark gray color. The preforms activated in this way are chemically photographed at room temperature in a solution of the composition, g / l: Nickel sulfate 50 Ammonium chloride 35
Phosphoric Acid Sodium 40 Ammonia To pH 9
Then the workpieces are nickel-plated in a standard Watts bath to a nickel content of 0.5 g / cm 3 . In the table, the characteristics of the electrode base made in this way are compared with the studied characteristics of the electrode base of the positive electrode of a Hoppecke type H nickel-cadmium battery, the design of which is similar to that described in the analogue and prototype.

Из таблицы следует, что по основным важным для характеристик электрода параметрам основа, изготовленная в соответствии с предлагаемым изобретением, и основа электрода фирмы "Hoppecke" близки. It follows from the table that, in terms of the main parameters important for the characteristics of the electrode, the base made in accordance with the invention and the base of the Hoppecke electrode are close.

Claims (1)

СПОСОБ ИЗГОТОВЛЕНИЯ ОСНОВЫ ЭЛЕКТРОДА ХИМИЧЕСКОГО ИСТОЧНИКА ТОКА путем активации поверхности волокнистого полимерного материала, его химической и гальванической металлизации, отличающийся тем, что в качестве полимерного волокнистого материала берут материал с обменной емкостью по катионам 0,5 - 6 мг-экв/г, а перед металлизацией производят насыщение полимерного материала ионами никеля с последующей обработкой водным раствором борогидрида щелочного металла при концентрации 0,1 - 1,2 г/л при 15 - 70oС в течение 0,5 - 30 мин.METHOD FOR PRODUCING THE BASIS OF A CHEMICAL SOURCE ELECTRODE ELECTRODE by activating the surface of a fibrous polymeric material, its chemical and galvanic metallization, characterized in that as a polymeric fibrous material they take a material with an exchange capacity for cations of 0.5 - 6 mEq / g, and before metallization the polymer material is saturated with nickel ions, followed by treatment with an aqueous solution of alkali metal borohydride at a concentration of 0.1 - 1.2 g / l at 15 - 70 o C for 0.5 - 30 minutes
RU92003415/07A 1992-11-02 1992-11-02 Process of manufacture of base of electrode of chemical source of energy RU2054758C1 (en)

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RU92003415/07A RU2054758C1 (en) 1992-11-02 1992-11-02 Process of manufacture of base of electrode of chemical source of energy
SK447-97A SK283829B6 (en) 1992-11-02 1995-08-14 Method of manufacturing electrodes for chemical current sources
PCT/RU1995/000170 WO1997007554A1 (en) 1992-11-02 1995-08-14 Method of manufacturing electrodes for chemical current sources

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RU92003415/07A RU2054758C1 (en) 1992-11-02 1992-11-02 Process of manufacture of base of electrode of chemical source of energy
PCT/RU1995/000170 WO1997007554A1 (en) 1992-11-02 1995-08-14 Method of manufacturing electrodes for chemical current sources

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Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
RU2407112C1 (en) * 2009-12-28 2010-12-20 Открытое акционерное общество "Завод автономных источников тока" Method for manufacturing of oxide-nickel electrode for alkaline accumulator
RU2482569C1 (en) * 2011-09-23 2013-05-20 Открытое акционерное общество "Завод автономных источников тока" Method for manufacturing of fibre oxide-nickel electrode for alkaline nickel-cadmium accumulator
RU2510548C1 (en) * 2012-08-16 2014-03-27 Федеральное государственное бюджетное образовательное учреждение высшего профессионального образования "Южно-Российский государственный университет экономики и сервиса" (ФГБОУ ВПО "ЮРГУЭС") Method of making electrode base for chemical cell from carbon felt using asymmetrical alternating current
RU2616584C1 (en) * 2015-12-22 2017-04-18 федеральное государственное бюджетное образовательное учреждение высшего образования "Нижегородский государственный технический университет им. Р.Е. Алексеева" Method of producing metal-felt bases for oxide-nickel electrodes of alkaline accumulators
RU2672854C1 (en) * 2017-11-09 2018-11-20 Дмитрий Николаевич Галушкин Method of manufacturing the basis of the electrode of a chemical source of a current from a carbon tissue using a variable asymmetric current

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
1. Заявка Франции N 2472842, кл. H 01M 4/26, 1981. 2. Заявка ФРГ N 4004106, кл. H 01M 4/75, 1991. *

Cited By (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
RU2407112C1 (en) * 2009-12-28 2010-12-20 Открытое акционерное общество "Завод автономных источников тока" Method for manufacturing of oxide-nickel electrode for alkaline accumulator
DE112010005026T5 (en) 2009-12-28 2012-10-04 Joint-Stock Co., Opened "Autonomomous Power Sources Plant" The process for producing the Nikeloxid electrode for an alkaline battery
RU2482569C1 (en) * 2011-09-23 2013-05-20 Открытое акционерное общество "Завод автономных источников тока" Method for manufacturing of fibre oxide-nickel electrode for alkaline nickel-cadmium accumulator
RU2510548C1 (en) * 2012-08-16 2014-03-27 Федеральное государственное бюджетное образовательное учреждение высшего профессионального образования "Южно-Российский государственный университет экономики и сервиса" (ФГБОУ ВПО "ЮРГУЭС") Method of making electrode base for chemical cell from carbon felt using asymmetrical alternating current
RU2616584C1 (en) * 2015-12-22 2017-04-18 федеральное государственное бюджетное образовательное учреждение высшего образования "Нижегородский государственный технический университет им. Р.Е. Алексеева" Method of producing metal-felt bases for oxide-nickel electrodes of alkaline accumulators
RU2672854C1 (en) * 2017-11-09 2018-11-20 Дмитрий Николаевич Галушкин Method of manufacturing the basis of the electrode of a chemical source of a current from a carbon tissue using a variable asymmetric current

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