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GB1340025A - Thermoplastic compositions - Google Patents

Thermoplastic compositions

Info

Publication number
GB1340025A
GB1340025A GB2674171*A GB2674171A GB1340025A GB 1340025 A GB1340025 A GB 1340025A GB 2674171 A GB2674171 A GB 2674171A GB 1340025 A GB1340025 A GB 1340025A
Authority
GB
United Kingdom
Prior art keywords
methacrylate
acrylate
stage
styrene
methyl
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
GB2674171*A
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Rohm and Haas Co
Original Assignee
Rohm and Haas Co
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Rohm and Haas Co filed Critical Rohm and Haas Co
Publication of GB1340025A publication Critical patent/GB1340025A/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F285/00Macromolecular compounds obtained by polymerising monomers on to preformed graft polymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F265/00Macromolecular compounds obtained by polymerising monomers on to polymers of unsaturated monocarboxylic acids or derivatives thereof as defined in group C08F20/00
    • C08F265/04Macromolecular compounds obtained by polymerising monomers on to polymers of unsaturated monocarboxylic acids or derivatives thereof as defined in group C08F20/00 on to polymers of esters
    • C08F265/06Polymerisation of acrylate or methacrylate esters on to polymers thereof
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L27/00Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Compositions of derivatives of such polymers
    • C08L27/02Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L27/04Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen; Compositions of derivatives of such polymers not modified by chemical after-treatment containing chlorine atoms
    • C08L27/06Homopolymers or copolymers of vinyl chloride
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L33/00Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides or nitriles thereof; Compositions of derivatives of such polymers
    • C08L33/04Homopolymers or copolymers of esters
    • C08L33/06Homopolymers or copolymers of esters of esters containing only carbon, hydrogen and oxygen, which oxygen atoms are present only as part of the carboxyl radical
    • C08L33/10Homopolymers or copolymers of methacrylic acid esters
    • C08L33/12Homopolymers or copolymers of methyl methacrylate
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L51/00Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L51/00Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
    • C08L51/003Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to macromolecular compounds obtained by reactions only involving unsaturated carbon-to-carbon bonds

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Graft Or Block Polymers (AREA)
  • Compositions Of Macromolecular Compounds (AREA)

Abstract

1340025 Multi-stage graft polymers ROHM & HAAS CO 19 April 1971 [13 April 1970] 26741/71 Heading C3G A multi-stage sequentially produced polymer comprises (A) a first elastomeric portion polymerized from a monomer mix comprising at least 50% by weight of one or more alkyl or aralkyl acrylates, 0À05-5À0% by weight of one or more cross-linking monomers, 0À05-5À0% by weight of one or more graft-linking monomers having two or more addition polymerizable unsaturated groups which participate in the polymerization reaction at substantially different rates, adapted to attach the elastomeric phase to the rigid phase defined hereinafter, 0-10À0% by weight hydrophilic monomer or non-hydrophilic monomer which is converted to hydrophilic mers in the elastomeric portion, the balance, if any, of said monomer mix being composed of one or more other copolymerizable ethylenically unsaturated monomars; and (B) a final, rigid thermoplastic portion polymerized, in the presence of said elastomeric portion, from a monomer mix comprising at least 50% by weight alkyl methacrylate, wherein said elastomeric portion and said thermoplastic portion have a minimum attachment level as hereinbefore defined of 20%. The multi-stage polymer material may be prepared by emulsion polymerization of an appropriate monomer charge to form the elastomeric portion and then continuing the emulsion polymerization with the addition of the monomer mix constituting the rigid portion material. The polymerization reactions may be initiated by either thermal or redox type initiator systems and conven- tional emulsifiers may also be present. Numerous examples of all the different monomer units are given. The composition of the multi-stage polymers in the specific examples (1-6) all of which refer to two-stage polymers is as follows: (1) a base polymer of butyl acrylate ("acrylate"), 1,3-butylene glycol diacrylate ("crosslinker"), allyl methacrylate ("graft-linker"), and styrene Œ acrylonitrile, hydroxy ethyl acrylate or methacrylamide units on to which is grafted monomer units of methyl methacrylate ; (2) a base polymer of butyl acrylate, 1,3, butylene glycol diacrylate, allyl methacrylate, styrene Œ hydroxyethyl acrylate, hydroxyethyl methacrylate or acrylamide on to which is grafted methyl methacrylate Œ hydroxyethyl methacrylate; (3) a base polymer of butyl i acrylate, 1,3-butylene diacrylate, allyl meth- acrylate, styrene, and either methacrylamide, N-ispropyl acrylamide or hydroxy propyl methacrylate on to which is grafted methyl methacrylate; and (4), (5), (6) a base polymer of butyl acrylate, 1,3-butylene glycol diacrylate, allyl methacrylate, styrene, hydroxypropyl methacrylate, ethylthioethyl methacrylate on to which is grafted a mixture of methyl methacrylate and methyl acrylate. Examples (8) and (9) refer to three stage polymers in which the 1st stage is constituted of butyl acrylate, styrene, ethylthioethyl methacrylate, butylene glycol diacrylate and allyl methacrylate; the 2nd stage of styrene, butyl acrylate, divinyl benzene and allyl methacrylate; and the 3rd stage (rigid portion) of either (a) methyl methacrylate, styrene and methyl acrylate or (b) methyl methacrylate, α-methyl styrene and methyl acrylate. The multi-stage polymer may be blended with a rigid thermoplastic polymer such as poly- (methyl methacrylate), copolymer of methyl methacrylate and ethyl acrylate, and vinyl halide homo- or co-polymers. In addition lubricants, dyes, fillers and plasticizers may be incorporated.
GB2674171*A 1970-04-13 1971-04-19 Thermoplastic compositions Expired GB1340025A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US2799670A 1970-04-13 1970-04-13

Publications (1)

Publication Number Publication Date
GB1340025A true GB1340025A (en) 1973-12-05

Family

ID=21840986

Family Applications (1)

Application Number Title Priority Date Filing Date
GB2674171*A Expired GB1340025A (en) 1970-04-13 1971-04-19 Thermoplastic compositions

Country Status (10)

Country Link
AU (1) AU2759171A (en)
BE (1) BE763809A (en)
BR (1) BR7102116D0 (en)
DE (1) DE2116653A1 (en)
ES (1) ES390495A1 (en)
FR (1) FR2092389A5 (en)
GB (1) GB1340025A (en)
IL (1) IL36593A0 (en)
NL (1) NL7104937A (en)
ZA (1) ZA712265B (en)

Cited By (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2253689A1 (en) * 1971-11-05 1973-05-10 Rohm & Haas THERMOPLASTIC PLASTIC COMPOUND
US4255308A (en) 1979-07-12 1981-03-10 E. I. Du Pont De Nemours And Company Water based acrylic lacquer composition
EP0110123A1 (en) * 1982-10-28 1984-06-13 Mitsubishi Rayon Co., Ltd. Delustering thermoplastic resin compostion
EP0143991A3 (en) * 1983-11-02 1986-10-08 Mitsubishi Rayon Co. Ltd. Impact-resistant methacrylic resin composition
EP0182558A3 (en) * 1984-11-12 1987-07-15 Mitsubishi Rayon Co. Ltd. Non-rigid vinyl chloride polymer resin composition
US7829610B2 (en) 2002-08-19 2010-11-09 Ticona Gmbh Impact-resistant polyoxymethylene molding compositions, use thereof and moldings produced therefrom
WO2017213827A1 (en) 2016-06-06 2017-12-14 Baxter International Inc. Methods of improving adhesion of non-di-(2-ethylhexyl)phthalate polyvinyl chloride to an acrylic- or abs-based polymer

Families Citing this family (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS515674B2 (en) * 1972-05-26 1976-02-21
DE2444584C3 (en) * 1974-09-18 1982-01-21 Basf Ag, 6700 Ludwigshafen Thermoplastic polyester molding compounds
US4152495A (en) * 1976-04-06 1979-05-01 Rohm And Haas Company Foamed thermoplastic resin composition containing multiple stage polymeric modifiers
DE2749579A1 (en) * 1977-11-05 1979-05-10 Basf Ag PROCESS FOR THE PRODUCTION OF MIXED GRAFT POLYMERISATES
FR2610328B1 (en) * 1987-01-30 1989-08-25 Charbonnages Ste Chimique INTERPOLYMER STRENGTHENING MATERIAL OF RIGID THERMOPLASTIC MATRICES, PREPARATION THEREOF AND CORRESPONDING REINFORCED COMPOSITIONS
DE19617068A1 (en) * 1996-04-29 1997-10-30 Basf Ag Molded parts made from thermoplastic molding compounds
FR2831546B1 (en) * 2001-10-31 2007-03-23 Atofina THERMOPLASTIC POLYMER MATERIAL FOR AUDIO AND / OR OPTICAL INFORMATION RECORDING MEDIA
FR2833962A1 (en) * 2001-12-21 2003-06-27 Atofina Discs for audio and/or optical data recording comprise two molded discs bonded together with an adhesive comprising methyl methacrylate and (meth)acrylic acid

Cited By (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2253689A1 (en) * 1971-11-05 1973-05-10 Rohm & Haas THERMOPLASTIC PLASTIC COMPOUND
US4255308A (en) 1979-07-12 1981-03-10 E. I. Du Pont De Nemours And Company Water based acrylic lacquer composition
EP0110123A1 (en) * 1982-10-28 1984-06-13 Mitsubishi Rayon Co., Ltd. Delustering thermoplastic resin compostion
EP0143991A3 (en) * 1983-11-02 1986-10-08 Mitsubishi Rayon Co. Ltd. Impact-resistant methacrylic resin composition
EP0182558A3 (en) * 1984-11-12 1987-07-15 Mitsubishi Rayon Co. Ltd. Non-rigid vinyl chloride polymer resin composition
US7829610B2 (en) 2002-08-19 2010-11-09 Ticona Gmbh Impact-resistant polyoxymethylene molding compositions, use thereof and moldings produced therefrom
WO2017213827A1 (en) 2016-06-06 2017-12-14 Baxter International Inc. Methods of improving adhesion of non-di-(2-ethylhexyl)phthalate polyvinyl chloride to an acrylic- or abs-based polymer

Also Published As

Publication number Publication date
AU2759171A (en) 1972-10-19
DE2116653A1 (en) 1971-10-28
NL7104937A (en) 1971-10-15
ES390495A1 (en) 1974-05-16
FR2092389A5 (en) 1972-01-21
BR7102116D0 (en) 1973-03-08
ZA712265B (en) 1972-05-31
IL36593A0 (en) 1971-06-23
BE763809A (en) 1971-09-06

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Legal Events

Date Code Title Description
PS Patent sealed [section 19, patents act 1949]
PLNP Patent lapsed through nonpayment of renewal fees