FR3053693B1 - Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu apres polymerisation de la composition - Google Patents

Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu apres polymerisation de la composition Download PDF

Info

Publication number: FR3053693B1
Authority: FR; France
Prior art keywords: composition; polymerization; liquid; phosphorous additive; phosphorous
Prior art date: 2016-07-11
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.): Expired - Fee Related

Application number

FR1656649A

Other languages

English (en)

Other versions

FR3053693A1 (fr

Inventor

Pierre Gerard

Pierre ESCALE

Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)

Arkema France SA

Original Assignee

Arkema France SA

Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)

2016-07-11

Filing date

2016-07-11

Publication date

2018-08-17

2016-07-11 Priority to FR1656649A priority Critical patent/FR3053693B1/fr

2016-07-11 Application filed by Arkema France SA filed Critical Arkema France SA

2017-07-11 Priority to KR1020197003792A priority patent/KR102428178B1/ko

2017-07-11 Priority to PCT/EP2017/067377 priority patent/WO2018011193A1/fr

2017-07-11 Priority to CN202410718278.6A priority patent/CN118562063A/zh

2017-07-11 Priority to CA3029790A priority patent/CA3029790A1/fr

2017-07-11 Priority to EP17742400.9A priority patent/EP3481875B1/fr

2017-07-11 Priority to US16/316,360 priority patent/US11629212B2/en

2017-07-11 Priority to CN201780042920.1A priority patent/CN109415470A/zh

2017-07-11 Priority to JP2019500596A priority patent/JP2019522091A/ja

2017-07-11 Priority to MX2019000130A priority patent/MX2019000130A/es

2017-07-11 Priority to BR112019000007-0A priority patent/BR112019000007B1/pt

2017-07-11 Priority to EP20168328.1A priority patent/EP3744743A1/fr

2018-01-12 Publication of FR3053693A1 publication Critical patent/FR3053693A1/fr

2018-08-17 Application granted granted Critical

2018-08-17 Publication of FR3053693B1 publication Critical patent/FR3053693B1/fr

2022-01-27 Priority to JP2022010613A priority patent/JP7401573B2/ja

Status Expired - Fee Related legal-status Critical Current

2036-07-11 Anticipated expiration legal-status Critical

Classifications

- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F265/00—Macromolecular compounds obtained by polymerising monomers on to polymers of unsaturated monocarboxylic acids or derivatives thereof as defined in group C08F20/00
- C08F265/04—Macromolecular compounds obtained by polymerising monomers on to polymers of unsaturated monocarboxylic acids or derivatives thereof as defined in group C08F20/00 on to polymers of esters
- C08F265/06—Polymerisation of acrylate or methacrylate esters on to polymers thereof
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F2/00—Processes of polymerisation
- C08F2/44—Polymerisation in the presence of compounding ingredients, e.g. plasticisers, dyestuffs, fillers
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
- C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
- C08F220/10—Esters
- C08F220/12—Esters of monohydric alcohols or phenols
- C08F220/14—Methyl esters, e.g. methyl (meth)acrylate
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F220/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical or a salt, anhydride ester, amide, imide or nitrile thereof
- C08F220/02—Monocarboxylic acids having less than ten carbon atoms; Derivatives thereof
- C08F220/10—Esters
- C08F220/12—Esters of monohydric alcohols or phenols
- C08F220/16—Esters of monohydric alcohols or phenols of phenols or of alcohols containing two or more carbon atoms
- C08F220/18—Esters of monohydric alcohols or phenols of phenols or of alcohols containing two or more carbon atoms with acrylic or methacrylic acids
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
- C08J5/04—Reinforcing macromolecular compounds with loose or coherent fibrous material
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
- C08J5/04—Reinforcing macromolecular compounds with loose or coherent fibrous material
- C08J5/10—Reinforcing macromolecular compounds with loose or coherent fibrous material characterised by the additives used in the polymer mixture
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
- C08J5/24—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J5/00—Manufacture of articles or shaped materials containing macromolecular substances
- C08J5/24—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs
- C08J5/249—Impregnating materials with prepolymers which can be polymerised in situ, e.g. manufacture of prepregs characterised by the additives used in the prepolymer mixture
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/18—Oxygen-containing compounds, e.g. metal carbonyls
- C08K3/20—Oxides; Hydroxides
- C08K3/22—Oxides; Hydroxides of metals
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/49—Phosphorus-containing compounds
- C08K5/51—Phosphorus bound to oxygen
- C08K5/53—Phosphorus bound to oxygen bound to oxygen and to carbon only
- C08K5/5313—Phosphinic compounds, e.g. R2=P(:O)OR'
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L33/00—Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides or nitriles thereof; Compositions of derivatives of such polymers
- C08L33/04—Homopolymers or copolymers of esters
- C08L33/06—Homopolymers or copolymers of esters of esters containing only carbon, hydrogen and oxygen, which oxygen atoms are present only as part of the carboxyl radical
- C08L33/10—Homopolymers or copolymers of methacrylic acid esters
- C08L33/12—Homopolymers or copolymers of methyl methacrylate
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L51/00—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
- C08L51/003—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to macromolecular compounds obtained by reactions only involving unsaturated carbon-to-carbon bonds
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J2333/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides, or nitriles thereof; Derivatives of such polymers
- C08J2333/04—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides, or nitriles thereof; Derivatives of such polymers esters
- C08J2333/06—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and only one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides, or nitriles thereof; Derivatives of such polymers esters of esters containing only carbon, hydrogen, and oxygen, the oxygen atom being present only as part of the carboxyl radical
- C08J2333/10—Homopolymers or copolymers of methacrylic acid esters
- C08J2333/12—Homopolymers or copolymers of methyl methacrylate
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J2351/00—Characterised by the use of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Derivatives of such polymers
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/0008—Organic ingredients according to more than one of the "one dot" groups of C08K5/01 - C08K5/59
- C08K5/0066—Flame-proofing or flame-retarding additives
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2201/00—Properties
- C08L2201/02—Flame or fire retardant/resistant

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Chemical & Material Sciences (AREA)
Medicinal Chemistry (AREA)
Organic Chemistry (AREA)
Polymers & Plastics (AREA)
Health & Medical Sciences (AREA)
Chemical Kinetics & Catalysis (AREA)
Materials Engineering (AREA)
Engineering & Computer Science (AREA)
Manufacturing & Machinery (AREA)
Compositions Of Macromolecular Compounds (AREA)
Polymerisation Methods In General (AREA)
Reinforced Plastic Materials (AREA)
Fireproofing Substances (AREA)
Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
Processes Of Treating Macromolecular Substances (AREA)

FR1656649A 2016-07-11 2016-07-11 Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu apres polymerisation de la composition Expired - Fee Related FR3053693B1 (fr)

Priority Applications (13)

Application Number	Priority Date	Filing Date	Title
FR1656649A FR3053693B1 (fr)	2016-07-11	2016-07-11	Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu apres polymerisation de la composition
BR112019000007-0A BR112019000007B1 (pt)	2016-07-11	2017-07-11	Composição líquida compreendendo um aditivo com base em fósforo, processo de impregnação, material compósito polimérico, processo para fabricar peças mecânicas ou elementos estruturais e parte mecânica ou elemento estrutural
CN202410718278.6A CN118562063A (zh)	2016-07-11	2017-07-11	包含磷基添加剂的液体组合物、其用途以及在组合物聚合后获得的材料或组合物
CA3029790A CA3029790A1 (fr)	2016-07-11	2017-07-11	Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu(e) apres polymerisation de la composition
EP17742400.9A EP3481875B1 (fr)	2016-07-11	2017-07-11	Composition liquide comprenant un additif à base de phosphore, son utilisation et matériau ou composition obtenu(e) après polymérisation de la composition
US16/316,360 US11629212B2 (en)	2016-07-11	2017-07-11	Liquid composition comprising a phousphorus based additive, its use and material or composition obtained following polymerisation of composition
KR1020197003792A KR102428178B1 (ko)	2016-07-11	2017-07-11	인 기반 첨가제를 포함하는 액체 조성물, 이의 용도, 및 조성물의 중합 이후 수득된 재료 또는 조성물
JP2019500596A JP2019522091A (ja)	2016-07-11	2017-07-11	リン系添加剤を含む液体組成物、その使用、及び組成物の重合後に得られる材料又は組成物
MX2019000130A MX2019000130A (es)	2016-07-11	2017-07-11	Composicion liquida que comprende un aditivo a base de fosforo, su uso y material o composicion obtenida despues de la polimerizacion de la composicion.
PCT/EP2017/067377 WO2018011193A1 (fr)	2016-07-11	2017-07-11	Composition liquide comprenant un additif à base de phosphore, son utilisation et matériau ou composition obtenu(e) après polymérisation de la composition
EP20168328.1A EP3744743A1 (fr)	2016-07-11	2017-07-11	Composition liquide comprenant un additif à base de phosphore, son utilisation et matériau ou composition obtenu(e) après la polymérisation de la composition
CN201780042920.1A CN109415470A (zh)	2016-07-11	2017-07-11	包含磷基添加剂的液体组合物、其用途以及在组合物聚合后获得的材料或组合物
JP2022010613A JP7401573B2 (ja)	2016-07-11	2022-01-27	リン系添加剤を含む液体組成物、その使用、及び組成物の重合後に得られる材料又は組成物

Applications Claiming Priority (2)

Application Number	Priority Date	Filing Date	Title
FR1656649A FR3053693B1 (fr)	2016-07-11	2016-07-11	Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu apres polymerisation de la composition
FR1656649		2016-07-11

Publications (2)

Publication Number	Publication Date
FR3053693A1 FR3053693A1 (fr)	2018-01-12
FR3053693B1 true FR3053693B1 (fr)	2018-08-17

Family

ID=57348818

Family Applications (1)

Application Number	Title	Priority Date	Filing Date
FR1656649A Expired - Fee Related FR3053693B1 (fr)	2016-07-11	2016-07-11	Composition liquide comprenant un additif a base de phosphore, son utilisation et materiau ou composition obtenu apres polymerisation de la composition

Country Status (9)

Country	Link
US (1)	US11629212B2 (fr)
EP (2)	EP3744743A1 (fr)
JP (2)	JP2019522091A (fr)
KR (1)	KR102428178B1 (fr)
CN (2)	CN118562063A (fr)
CA (1)	CA3029790A1 (fr)
FR (1)	FR3053693B1 (fr)
MX (1)	MX2019000130A (fr)
WO (1)	WO2018011193A1 (fr)

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number	Priority date	Publication date	Assignee	Title
EP4378985A1 (fr) *	2022-12-01	2024-06-05	Trinseo Europe GmbH	Polymères acryliques ignifuges sans halogène destinés à être utilisés dans l'extrusion de feuilles et le traitement de moulage par injection multiple
KR102825637B1 (ko)	2025-02-13	2025-06-30	주식회사 세라웰	고기능성 준불연 첨가제의 제조방법

Family Cites Families (15)

* Cited by examiner, † Cited by third party
Publication number	Priority date	Publication date	Assignee	Title
DE2252258A1 (de)	1972-10-25	1974-05-09	Hoechst Ag	Schwerentflammbare thermoplastische polyester
DE2447727A1 (de)	1974-10-07	1976-04-08	Hoechst Ag	Schwerentflammbare polyamidformmassen
EP1013713A1 (fr)	1998-12-22	2000-06-28	H.B. Fuller Coatings Ltd.	Composition de polymère ignifuge
DE19917428A1 (de) *	1999-04-19	2000-10-26	Clariant Gmbh	Flammwidrige phosphormodifizierte Epoxidharze
DE10347012A1 (de)	2003-10-07	2005-05-25	Clariant Gmbh	Phosphorhaltige Flammschutzmittelagglomerate
WO2005061606A1 (fr)	2003-12-19	2005-07-07	Rhodia Engineering Plastics S.R.L.	Composition ignifugee a base de matrice thermoplastique
JP5614389B2 (ja) *	2005-12-01	2014-10-29	日立化成株式会社	樹脂組成物、並びに、プリプレグ、金属張積層板、封止材、感光性フィルム、レジストパターンの形成方法及びプリント配線板
WO2010051893A1 (fr) *	2008-11-07	2010-05-14	Clariant International Ltd	Procédé pour produire des acides, des esters et des sels dialkylphosphiniques au moyen de dérivés d'acide acrylique et leur utilisation
FR2981652B1 (fr)	2011-10-21	2015-03-27	Arkema France	Composites via la polymerisation in-situ de resines thermoplastiques methacryliques
DE102011121503A1 (de) *	2011-12-16	2013-06-20	Clariant International Ltd.	Gemische von Dioshinsäuren und Dialkylphosphinsäuren, ein Verfahren zu deren Herstellung und ihre Verwendung
DE102011121590A1 (de) *	2011-12-16	2013-06-20	Clariant International Ltd.	Gemische von Diphosphinsäuren und Alkylphosphinsäuren, ein Verfahren zu deren Herstellung und ihre Verwendung
DE102011121591A1 (de) *	2011-12-16	2013-06-20	Clariant International Ltd.	Gemische aus Dialkylphosphinsäuren und Alkylphosphonsäuren, ein Verfahren zu deren Herstellung und ihre Verwendung
DE102011121900A1 (de) *	2011-12-21	2013-06-27	Clariant International Ltd.	Gemische von mindestens einer Dialkylphosphinsäure mit mindestens einer anderen, davon unterschiedlichen Dialkylphosphinsäure, Verfahren zu deren Herstellung und ihre Verwendung
FR2993581B1 (fr)	2012-07-18	2016-01-22	Arkema France	Procede d'impregnation pour un substrat fibreux, sirop (meth)acrylique liquide pour le procede d'impregnation, son procede de polymerisation et produit structure obtenu a partir de celui-ci
FR3002943B1 (fr) *	2013-03-11	2015-03-27	Arkema France	Sirop (meth)acrylique liquide d'impregnation d'un substrat fibreux, procede d'impregnation d'un substrat fibreux, materiau composite obtenu apres polymerisation dudit substrat pre-impregne.

2016
- 2016-07-11 FR FR1656649A patent/FR3053693B1/fr not_active Expired - Fee Related
2017
- 2017-07-11 US US16/316,360 patent/US11629212B2/en active Active
- 2017-07-11 JP JP2019500596A patent/JP2019522091A/ja active Pending
- 2017-07-11 CN CN202410718278.6A patent/CN118562063A/zh active Pending
- 2017-07-11 MX MX2019000130A patent/MX2019000130A/es unknown
- 2017-07-11 CA CA3029790A patent/CA3029790A1/fr active Pending
- 2017-07-11 KR KR1020197003792A patent/KR102428178B1/ko active Active
- 2017-07-11 WO PCT/EP2017/067377 patent/WO2018011193A1/fr not_active Ceased
- 2017-07-11 EP EP20168328.1A patent/EP3744743A1/fr not_active Withdrawn
- 2017-07-11 EP EP17742400.9A patent/EP3481875B1/fr active Active
- 2017-07-11 CN CN201780042920.1A patent/CN109415470A/zh active Pending
2022
- 2022-01-27 JP JP2022010613A patent/JP7401573B2/ja active Active

Also Published As

Publication number	Publication date
KR20190026871A (ko)	2019-03-13
CA3029790A1 (fr)	2018-01-18
US20190225729A1 (en)	2019-07-25
EP3481875A1 (fr)	2019-05-15
KR102428178B1 (ko)	2022-08-01
FR3053693A1 (fr)	2018-01-12
JP2022068173A (ja)	2022-05-09
CN118562063A (zh)	2024-08-30
MX2019000130A (es)	2019-04-01
EP3481875B1 (fr)	2020-04-08
CN109415470A (zh)	2019-03-01
JP7401573B2 (ja)	2023-12-19
BR112019000007A2 (pt)	2019-04-16
US11629212B2 (en)	2023-04-18
JP2019522091A (ja)	2019-08-08
EP3744743A1 (fr)	2020-12-02
WO2018011193A1 (fr)	2018-01-18

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