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EP0121274A1 - Procédé de phosphatation de surfaces métalliques - Google Patents

Procédé de phosphatation de surfaces métalliques Download PDF

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Publication number
EP0121274A1
EP0121274A1 EP84200316A EP84200316A EP0121274A1 EP 0121274 A1 EP0121274 A1 EP 0121274A1 EP 84200316 A EP84200316 A EP 84200316A EP 84200316 A EP84200316 A EP 84200316A EP 0121274 A1 EP0121274 A1 EP 0121274A1
Authority
EP
European Patent Office
Prior art keywords
metal surfaces
phosphating
nitrobenzenesulfonate
contact
brought
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Withdrawn
Application number
EP84200316A
Other languages
German (de)
English (en)
Inventor
Gerd Müller
Werner Dr. Rausch
Wolfgang Wuttke
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
GEA Group AG
Continentale Parker Ste
Continentale Parker SA
Original Assignee
Metallgesellschaft AG
Continentale Parker Ste
Continentale Parker SA
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Metallgesellschaft AG, Continentale Parker Ste, Continentale Parker SA filed Critical Metallgesellschaft AG
Publication of EP0121274A1 publication Critical patent/EP0121274A1/fr
Withdrawn legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C22/00Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals
    • C23C22/05Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions
    • C23C22/06Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6
    • C23C22/07Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6 containing phosphates
    • C23C22/08Orthophosphates
    • C23C22/12Orthophosphates containing zinc cations
    • C23C22/13Orthophosphates containing zinc cations containing also nitrate or nitrite anions
    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23CCOATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C22/00Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals
    • C23C22/05Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions
    • C23C22/06Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6
    • C23C22/07Chemical surface treatment of metallic material by reaction of the surface with a reactive liquid, leaving reaction products of surface material in the coating, e.g. conversion coatings, passivation of metals using aqueous solutions using aqueous acidic solutions with pH less than 6 containing phosphates
    • C23C22/08Orthophosphates
    • C23C22/12Orthophosphates containing zinc cations
    • C23C22/14Orthophosphates containing zinc cations containing also chlorate anions

Definitions

  • the invention relates to a method for applying P HOS phatüberratn on metal surfaces by means of nitrite accelerated phosphating solutions based on zinc phosphate.
  • aqueous acidic zinc phosphate solution to accelerate the film formation and oxidation of the dissolved iron in the trivalent form of nitrites, in particular A lkalinitrite to add (DE-PSs 845 135 907 966 D E-ASs 10 31 083, 12 77 645, DE-OS 17 71 769).
  • the methods are widely used in practice. They are characterized by a high degree of phosphating, however, provide a layer refinement unless specific substances, such as P olyphos- phosphates (E-AS 10 62 083) are added to phosphate layers having relatively high basis weights.
  • the object of the invention is to provide a method which does not have the disadvantages of the known methods and, with a high acceleration effect, provides extremely fine-grained, flexible phosphate layers with a low basis weight.
  • the object is achieved by designing the method of the type mentioned at the outset in accordance with the invention in such a way that the metal surfaces are brought into contact with a phosphating solution additionally containing nitrobenzenesulfonate, the nitrobenzenesulfonate content of which is such that the resulting layer weight is less than 2 g / m 2.
  • the method according to the invention is intended in particular for the treatment of iron and steel. However, it is also suitable for phosphating zinc and aluminum materials as well as steel with coatings made of zinc, zinc alloys, aluminum and aluminum alloys, which are produced using a wide variety of processes.
  • the metal surfaces can be treated by spraying, flooding and also immersion. However, it is also possible with combined working methods, e.g. Splash-diving, diving-spraying, splash-diving-spraying and the like are applicable.
  • the contact times for the phosphating solution with the metal surface are in the usual range and can e.g. 45 seconds to 3 minutes for spraying, 2 to 10 minutes for diving and 20 seconds of spraying and 3 minutes for diving.
  • the temperatures of the phosphating solutions used in the process according to the invention are usually between 30 and 60 ° C. The lower the temperature, the longer i.a. the contact time.
  • the desired layer weights can be set by suitable dosing below 2 g / m 2 .
  • Layer weights of up to approximately 1 g / m 2 can be set.
  • an advantageous embodiment of the invention provides the metal surface with an P hospha- t istsown be brought into contact, the Nitrobenzolsulfonatgehalt is dimensioned such that the resulting S chichtactis below 1.5 g / m 2.
  • the metal surfaces it is advantageous to bring the metal surfaces into contact with a phosphating solution whose nitrobenzenesulfonate content is at least 300 mg / l.
  • the contents of the individual effective bath components are within the usual limits.
  • the nitrite content is preferably in the range from 10 to 300 mg / l.
  • the upper limit for the content of nitrobenzenesulfonate is about 2 g / 1. Higher levels are practically associated with no additional effect.
  • nitrite and nitrobenzenesulfonate accelerators are usually added to the phosphating bath in the form of the alkali salts.
  • the nitrobenzenesulfonate can also be introduced as the corresponding sulfonic acid.
  • aqueous acidic solutions based on zinc phosphate to be used in the context of the invention contain primary zinc phosphate and a certain amount of free acid which is matched to the respective building concentration, type of application and bath temperature.
  • the pH of the baths is between 2.0 and 3.9, depending on the process conditions.
  • the baths can also contain other cations known in phosphating technology, for example Ni, Co, Cu, Mn, Ca, Mg, Fe, Na, K , Li, NH 4 and others.
  • other anions different from phosphate for example NO 3 , C10 3 , Cl, SO 4 , F, BF 4 , SiF 6 , citrate, tartrate, etc., may be necessary or desirable .
  • the metal surfaces to be brought into contact with a phosphating solution in which the weight ratio of Zn to P 2 O 5 is set to 1: (8 to 85), or the metal surfaces with a Phos to bring phating solution in contact, in which the weight ratio of Zn to P 2 0 5 is set to 1: (0.3 to 7).
  • phosphate layers with a high proportion of phosphophyllite to hopite are formed on steel. Because of their excellent corrosion protection, these coatings are particularly suitable as a preparation for painting, with the best protective properties being achieved in connection with cathodic electrocoating.
  • Steel sheets were degreased in an alkaline, aqueous cleaner, rinsed with water and then treated with various phosphating solutions by spraying at 55 ° C. for 2 minutes.

Landscapes

  • Chemical & Material Sciences (AREA)
  • General Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Chemical Treatment Of Metals (AREA)
EP84200316A 1983-03-31 1984-03-06 Procédé de phosphatation de surfaces métalliques Withdrawn EP0121274A1 (fr)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DE3311738 1983-03-31
DE19833311738 DE3311738A1 (de) 1983-03-31 1983-03-31 Verfahren zur phosphatierung von metalloberflaechen

Publications (1)

Publication Number Publication Date
EP0121274A1 true EP0121274A1 (fr) 1984-10-10

Family

ID=6195182

Family Applications (1)

Application Number Title Priority Date Filing Date
EP84200316A Withdrawn EP0121274A1 (fr) 1983-03-31 1984-03-06 Procédé de phosphatation de surfaces métalliques

Country Status (9)

Country Link
EP (1) EP0121274A1 (fr)
AU (1) AU2629184A (fr)
BR (1) BR8401487A (fr)
CA (1) CA1206852A (fr)
DE (1) DE3311738A1 (fr)
ES (1) ES8504270A1 (fr)
GB (1) GB2137231B (fr)
PT (1) PT78335B (fr)
ZA (1) ZA842173B (fr)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP0258922A1 (fr) * 1986-09-05 1988-03-09 Metallgesellschaft Ag Procédé pour produire des revêtements de phosphate et leur utilisation
EP0287133A1 (fr) * 1987-04-11 1988-10-19 Metallgesellschaft Ag Procédé de phosphatation avant la peinture électrophorétique par immersion

Families Citing this family (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3408577A1 (de) * 1984-03-09 1985-09-12 Metallgesellschaft Ag, 6000 Frankfurt Verfahren zur phosphatierung von metallen
US5234509A (en) * 1984-12-20 1993-08-10 Henkel Corporation Cold deformation process employing improved lubrication coating
CA1257527A (fr) * 1984-12-20 1989-07-18 Thomas W. Tull Procede de deformation a froid avec enduction lubrifiante amelioree
US4595424A (en) * 1985-08-26 1986-06-17 Parker Chemical Company Method of forming phosphate coating on zinc
USRE35958E (en) * 1985-08-26 1998-11-17 Henkel Corporation Method of forming phosphate coating on zinc
GB8523572D0 (en) * 1985-09-24 1985-10-30 Pyrene Chemicals Services Ltd Coating metals
US5236565A (en) * 1987-04-11 1993-08-17 Metallgesellschaft Aktiengesellschaft Process of phosphating before electroimmersion painting
DE3871031D1 (de) * 1987-08-19 1992-06-17 Metallgesellschaft Ag Verfahren zur phosphatierung von metallen.

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3016576A1 (de) * 1980-04-30 1981-11-05 Metallgesellschaft Ag, 6000 Frankfurt Verfahren zur phosphatierung von metalloberflaechen sowie dessen anwendung
EP0069950A1 (fr) * 1981-07-13 1983-01-19 Metallgesellschaft Ag Procédé de phosphatation de surfaces métalliques

Family Cites Families (8)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2884351A (en) * 1956-01-25 1959-04-28 Parker Rust Proof Co Method of cold rolling ferrous strip stock
FR1258855A (fr) * 1960-02-18 1961-04-21 Parker Ste Continentale Procédé perfectionné de phosphatation de surfaces métalliques
FR2110784A5 (fr) * 1970-10-30 1972-06-02 Parker Ste Continentale
NL7114590A (fr) * 1971-10-22 1973-04-25
SE441105B (sv) * 1976-04-05 1985-09-09 Amchem Prod Forfarande for framstellning av en amorf, lett, hart fastsittande fosfatbeleggning
GB1542222A (en) * 1977-01-06 1979-03-14 Pyrene Chemical Services Ltd Phosphate coating compositions
JPS5456038A (en) * 1977-10-12 1979-05-04 Nippon Paint Co Ltd Controlling method for acidic phosphate film forming liquid
DE2908376C2 (de) * 1979-03-03 1985-09-26 Akzo Gmbh, 5600 Wuppertal Verfahren zur Herstellung einer antistatischen Teppichfaser

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3016576A1 (de) * 1980-04-30 1981-11-05 Metallgesellschaft Ag, 6000 Frankfurt Verfahren zur phosphatierung von metalloberflaechen sowie dessen anwendung
EP0069950A1 (fr) * 1981-07-13 1983-01-19 Metallgesellschaft Ag Procédé de phosphatation de surfaces métalliques

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP0258922A1 (fr) * 1986-09-05 1988-03-09 Metallgesellschaft Ag Procédé pour produire des revêtements de phosphate et leur utilisation
EP0287133A1 (fr) * 1987-04-11 1988-10-19 Metallgesellschaft Ag Procédé de phosphatation avant la peinture électrophorétique par immersion

Also Published As

Publication number Publication date
ES531002A0 (es) 1985-05-01
GB8408006D0 (en) 1984-05-10
DE3311738A1 (de) 1984-10-04
GB2137231A (en) 1984-10-03
ZA842173B (en) 1984-10-31
ES8504270A1 (es) 1985-05-01
CA1206852A (fr) 1986-07-02
AU2629184A (en) 1984-10-04
GB2137231B (en) 1986-06-18
PT78335A (en) 1984-04-01
PT78335B (en) 1986-04-30
BR8401487A (pt) 1984-11-13

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PUAI Public reference made under article 153(3) epc to a published international application that has entered the european phase

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Effective date: 19850112

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Withdrawal date: 19860409

RIN1 Information on inventor provided before grant (corrected)

Inventor name: WUTTKE, WOLFGANG

Inventor name: RAUSCH, WERNER, DR.

Inventor name: MUELLER, GERD