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DE3604063A1 - Gas purification downstream of waste incineration plants - Google Patents

Gas purification downstream of waste incineration plants

Info

Publication number
DE3604063A1
DE3604063A1 DE19863604063 DE3604063A DE3604063A1 DE 3604063 A1 DE3604063 A1 DE 3604063A1 DE 19863604063 DE19863604063 DE 19863604063 DE 3604063 A DE3604063 A DE 3604063A DE 3604063 A1 DE3604063 A1 DE 3604063A1
Authority
DE
Germany
Prior art keywords
downstream
waste incineration
heavy metals
gas purification
dry
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Granted
Application number
DE19863604063
Other languages
German (de)
Other versions
DE3604063C2 (en
Inventor
Heinz Dipl Ing Hoelter
Heinrich Dipl Ing Igelbuescher
Heinrich Ing Grad Gresch
Heribert Dipl Ing Dewert
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Individual
Original Assignee
Individual
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Individual filed Critical Individual
Priority to DE19863604063 priority Critical patent/DE3604063A1/en
Priority to EP87900093A priority patent/EP0248855A1/en
Priority to PCT/EP1986/000693 priority patent/WO1987003506A2/en
Publication of DE3604063A1 publication Critical patent/DE3604063A1/en
Application granted granted Critical
Publication of DE3604063C2 publication Critical patent/DE3604063C2/de
Granted legal-status Critical Current

Links

Classifications

    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01DSEPARATION
    • B01D53/00Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B01D53/34Chemical or biological purification of waste gases
    • B01D53/46Removing components of defined structure
    • B01D53/60Simultaneously removing sulfur oxides and nitrogen oxides

Landscapes

  • Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Biomedical Technology (AREA)
  • Environmental & Geological Engineering (AREA)
  • Analytical Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Treating Waste Gases (AREA)

Abstract

It is known to provide dry or wet gas purification plants or a combination thereof downstream of waste incineration plants. It is further known that HCl, HF and also SO2 as well as most heavy metals can be separated off in dry filters by addition of hydrated lime and a certain amount of moisture, but the gaseous heavy metals, such as mercury, can only be eliminated in a downstream wet separator. For residual emission removal of the acidic constituents still present in the flue gas after the dry filter, a wet separator is provided downstream, to the scrubbing water circulation of which are added calcium hydroxide solutions, an active substance of trimercapto-s-triazine being additionally added.

Description

Es ist bekannt, hinter Müllverbrennungsanlagen trockene oder nasse Gasreinigungsanlagen oder deren Kombination nachzuschalten.It is known behind waste incinerators dry or wet gas cleaning plants or their To add a combination.

Es ist bekannt, daß in Trockenfiltern, insbesondere durch Zugabe von Kalkhydrat und einer gewissen Feuchte HCl, HF und auch SO2 und die meisten Schwermetalle abgeschieden werden können, jedoch die gasförmigen Schwermetalle, wie z.B. Quecksilber sich nur in einem nachgeschalteten Naßabscheider abscheiden lassen.It is known that in dry filters, in particular by adding hydrated lime and a certain moisture, HCl, HF and also SO 2 and most heavy metals can be separated, but the gaseous heavy metals, such as mercury, can only be separated in a downstream wet separator.

Zur Restemissionsabscheidung der noch im Rauchgas nach dem Trockenfilter befindlichen sauren Bestandteile wird dazu ein Naßabscheider geschaltet, dessen Wasch­ wasserkreislauf Calciumhydrat zudosiert wird, wobei sich aus den Schwefeloxiden Calciumsulfit und Calcium­ sulfat bilden.To remove residual emissions from the flue gas acidic components in the dry filter a wet separator is switched to wash it water circuit calcium hydrate is added, whereby consist of the sulfur oxides calcium sulfite and calcium  form sulfate.

Um die flüchtigen Schwermetalle, insbesondere Quecksilber in der Naßwäsche aus dem Rauchgas zu binden, wird er­ findungsgemäß dem Waschwasser als Wirksubstanz Trimercapto-s-triazin zugegeben.The volatile heavy metals, especially mercury to bind from the flue gas in the wet wash, he will According to the washing water as an active substance Trimercapto-s-triazine added.

Eingesetzt wird das Trimercapto-s-triazin zweckdienlich in Form des Natriumsalzes.Trimercapto-s-triazine is useful in the form of the sodium salt.

Es besitzt eine hohe Umweltfreundlichkeit, die durch die Prüfung auf Fischschädlichkeit gemäß dem Goldorfen- Test nachgewiesen wurde.It has a high environmental friendliness due to the fish harm test according to the gold cast Test has been demonstrated.

Die gebildeten Feststoffe, bestehend aus dem Rückstands­ produkt CaSO3, CaSO4, dem freien CaOH2 mit den an Trimercapto-s-triazin gebundenen Schwermetallen, Quecksilber, Cadmium und Nickel, bilden in Wasser schwerlösliche stabile Verbindungen. The solids formed, consisting of the residue product CaSO 3 , CaSO 4 , the free CaOH 2 with the heavy metals bound to trimercapto-s-triazine, mercury, cadmium and nickel, form poorly soluble stable compounds in water.

Sie werden von verdünnten Säuren nicht angegriffen und weisen eine hohe Temperaturbeständigkeit auf.They are not attacked by dilute acids and have a high temperature resistance.

Diese Quecksilberverbindung zersetzt sich beispiels­ weise erst oberhalb von 210°C, wobei selbst unter diesen Bedingungen noch kein Quecksilber freigesetzt wird, sondern andere stabilere Verbindungen gebildet werden.This mercury compound decomposes, for example only above 210 ° C, even under no mercury released under these conditions is formed, but other more stable connections will.

Aus den abgelagerten Produkten hat sich gezeigt, daß Quecksilber nicht auslaugt.From the deposited products it has been shown that Mercury does not leach out.

Claims (1)

Verfahren zum Ausfällen von Schwermetallen, vorzugsweise Quecksilber in Waschlösungen, vorzugsweise hinter Müllverbrennungsanlagen, dadurch gekennzeichnet, daß der Naßwäscher, der vorzugsweise einer trockenen Abscheidestufe nachge­ schaltet wird, mit Calciumhydroxidlösungen geimpft wird, wobei zusätzlich eine Wirksubstanz von Trimercapto-s-triazin zugegeben wird.Process for the precipitation of heavy metals, preferably mercury in washing solutions, preferably behind waste incineration plants, characterized in that the wet scrubber, which is preferably switched to a dry separation stage, is inoculated with calcium hydroxide solutions, with an additional active ingredient of trimercapto-s-triazine being added.
DE19863604063 1985-12-04 1986-02-08 Gas purification downstream of waste incineration plants Granted DE3604063A1 (en)

Priority Applications (3)

Application Number Priority Date Filing Date Title
DE19863604063 DE3604063A1 (en) 1986-02-08 1986-02-08 Gas purification downstream of waste incineration plants
EP87900093A EP0248855A1 (en) 1985-12-04 1986-11-29 PROCESS FOR SINGLE OR MULTI-PHASE PREFERABLY SIMULTANEOUS SO 2? AND NO x? SEPARATION FROM FLUE GASES IN A WET PROCESS
PCT/EP1986/000693 WO1987003506A2 (en) 1985-12-04 1986-11-29 PROCESS FOR SINGLE OR MULTI-PHASE PREFERABLY SIMULTANEOUS SO2 AND NOx SEPARATION FROM FLUE GASES IN A WET PROCESS

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE19863604063 DE3604063A1 (en) 1986-02-08 1986-02-08 Gas purification downstream of waste incineration plants

Publications (2)

Publication Number Publication Date
DE3604063A1 true DE3604063A1 (en) 1987-08-13
DE3604063C2 DE3604063C2 (en) 1988-12-29

Family

ID=6293746

Family Applications (1)

Application Number Title Priority Date Filing Date
DE19863604063 Granted DE3604063A1 (en) 1985-12-04 1986-02-08 Gas purification downstream of waste incineration plants

Country Status (1)

Country Link
DE (1) DE3604063A1 (en)

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3704533A1 (en) * 1987-02-13 1988-08-25 Kernforschungsz Karlsruhe METHOD FOR CONTINUOUSLY MONITORING EMISSIONS AND IMMISSIONS FOR MERCURY
EP1040865A3 (en) * 1999-03-31 2001-11-14 McDermott Technology, Inc. Mercury removal in utility wet scrubber using a chelating agent
US9844752B2 (en) 2012-11-29 2017-12-19 Alfa Laval Corporate Ab System, a use of such a system and a multi system for cleaning exhaust gas

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE1669314A1 (en) * 1966-08-15 1970-08-13 Hitachi Ltd Process and device for desulphurization of industrial exhaust gases
FR2080451A5 (en) * 1970-02-05 1971-11-12 Osaka Soda Co Ltd
DE2132231C3 (en) * 1970-07-03 1973-08-30 Outokumpu Oy Process for separating and recovering mercury and / or selenium from gases containing mercury and / or selenium

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE1669314A1 (en) * 1966-08-15 1970-08-13 Hitachi Ltd Process and device for desulphurization of industrial exhaust gases
FR2080451A5 (en) * 1970-02-05 1971-11-12 Osaka Soda Co Ltd
DE2132231C3 (en) * 1970-07-03 1973-08-30 Outokumpu Oy Process for separating and recovering mercury and / or selenium from gases containing mercury and / or selenium

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3704533A1 (en) * 1987-02-13 1988-08-25 Kernforschungsz Karlsruhe METHOD FOR CONTINUOUSLY MONITORING EMISSIONS AND IMMISSIONS FOR MERCURY
EP1040865A3 (en) * 1999-03-31 2001-11-14 McDermott Technology, Inc. Mercury removal in utility wet scrubber using a chelating agent
US9844752B2 (en) 2012-11-29 2017-12-19 Alfa Laval Corporate Ab System, a use of such a system and a multi system for cleaning exhaust gas

Also Published As

Publication number Publication date
DE3604063C2 (en) 1988-12-29

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Legal Events

Date Code Title Description
OP8 Request for examination as to paragraph 44 patent law
D2 Grant after examination
8363 Opposition against the patent
8331 Complete revocation