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DE3428691A1 - Process for the conversion of EDTA and sulphur-nitrogen compounds from waste waters of NOX scrubber units - Google Patents

Process for the conversion of EDTA and sulphur-nitrogen compounds from waste waters of NOX scrubber units

Info

Publication number
DE3428691A1
DE3428691A1 DE19843428691 DE3428691A DE3428691A1 DE 3428691 A1 DE3428691 A1 DE 3428691A1 DE 19843428691 DE19843428691 DE 19843428691 DE 3428691 A DE3428691 A DE 3428691A DE 3428691 A1 DE3428691 A1 DE 3428691A1
Authority
DE
Germany
Prior art keywords
water
nitrogen compounds
edta
sulphur
conversion
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Withdrawn
Application number
DE19843428691
Other languages
German (de)
Inventor
Heribert Dipl.-Ing. 4390 Gladbeck Dewert
Heinrich Ing.(grad.) 4600 Dortmund Gresch
Heinz Dipl.-Ing. Hölter
Heinrich Dipl.-Ing. 4390 Gladbeck Igelbüscher
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Individual
Original Assignee
Individual
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Individual filed Critical Individual
Priority to DE19843428691 priority Critical patent/DE3428691A1/en
Publication of DE3428691A1 publication Critical patent/DE3428691A1/en
Withdrawn legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/02Treatment of water, waste water, or sewage by heating
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01DSEPARATION
    • B01D53/00Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B01D53/34Chemical or biological purification of waste gases
    • B01D53/46Removing components of defined structure
    • B01D53/60Simultaneously removing sulfur oxides and nitrogen oxides
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F11/00Treatment of sludge; Devices therefor
    • C02F11/06Treatment of sludge; Devices therefor by oxidation
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02ATECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE
    • Y02A50/00TECHNOLOGIES FOR ADAPTATION TO CLIMATE CHANGE in human health protection, e.g. against extreme weather
    • Y02A50/20Air quality improvement or preservation, e.g. vehicle emission control or emission reduction by using catalytic converters

Landscapes

  • Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Environmental & Geological Engineering (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Hydrology & Water Resources (AREA)
  • Water Supply & Treatment (AREA)
  • Organic Chemistry (AREA)
  • Biomedical Technology (AREA)
  • Analytical Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Health & Medical Sciences (AREA)
  • Treating Waste Gases (AREA)

Abstract

The invention relates to a process for the conversion of EDTA and sulphur-nitrogen compounds and carboxylic acid compounds from waste waters of SO2 and NOX scrubber units. Because of the chlorine content of the coal, a part-amount of the water must be discharged in order to prevent salination of the scrubbing waters. This partial discharge of scrubbing water from the circulation also removes the additive EDTA and the sulphur-nitrogen compounds formed together with the water. In order to remedy this disadvantage, it is proposed according to the invention that a desired amount of waste water from the scrubbing water circulation of one or, simultaneously, of a plurality or of all scrubber stages is fed, via a pump, to a nozzle apparatus which opens in the hot region of the untreated gases, preferably in the region of the boiler, upstream and/or downstream of the electrostatic precipitator.

Description

Beschreibung und Erläuterung zur PatentanmeldungDescription and explanation of the patent application

"Verfahren zur Wandlung von ED#A und Schwefelstickstoffverbindungen aus Abwässern von NOx-Waschanlagen"."Process for the Conversion of ED # A and Sulfur-Nitrogen Compounds from waste water from NOx washing plants ".

Es ist bekannt, S02 und NO, simultan und/oder mehrstufig aus Rauchgasen von Fossilkraftwerken auszuwaschen.It is known that SO2 and NO, simultaneously and / or in multiple stages, from flue gases washed out by fossil fuel power plants.

Aufgrund des Chlorgehaltes in der Kohle muß eine Teilwassermenge abgeführt werden, um eine Aufsalzung der Waschwässer zu verhindern.Due to the chlorine content in the coal, part of the water has to be removed to prevent salt build-up in the washing water.

Zwangsläufig werden mit dieser Teilabgabemenge von Waschwasser aus dem Kreislauf auch das Additiv EDTA und die sich gebildeten Schwefelstickstoffverbindungen mit dem Wasser ausgetragen.Inevitably, with this partial delivery amount of wash water The EDTA additive and the sulfur-nitrogen compounds formed are also added to the cycle discharged with the water.

Das Aufbereiten der Teilabgabemenge in biologischen Abwasserbehandlungsanlagen oder durch chemische Aufoxidation ist aufwendig und soll durch die nachstehende Erfindung gemindert werden.The preparation of the partial delivery quantity in biological wastewater treatment plants or by chemical oxidation is expensive and should be replaced by the following Invention are diminished.

Erfindungsgemäß wird Wasser, das mit EDTA und/oder Schwefel-Stickstoff-Verbindungen und/oder Polycarbonsäuren angereichert ist, in den Bereich der heißesten Rohgaszuführung aufgegeben, vorzugsweise unmittelbar hinter dem Elektrofilter.According to the invention, water containing EDTA and / or sulfur-nitrogen compounds is used and / or polycarboxylic acids is enriched in the area of the hottest raw gas supply abandoned, preferably immediately after the electrostatic precipitator.

Hier werden bei Temperaturen von größer 13000 das genannte EDTA und/oder die Schwefelstickstoffverbindungen thermisch zersetzt und ungefährlich dem Waschprozeß der 1. Waschstufe zugeführt.Here, at temperatures greater than 13,000, the named EDTA and / or the sulfur-nitrogen compounds thermally decomposed and harmless to the washing process fed to the 1st washing stage.

Aus der 1. Waschstufe, die zur Verbesserung der Auswaschung von 502 und/oder NO auch mit Carbonsäuren und/oder Polycarbonsäuren betrieben wird, wird erfindungsgemäß vorgeschlagen, ebenfalls eine Teilwassermenge in die heißesten Bereiche der Rohgaszuführung aufzugeben, vor und/oder hinter dem Elektrofilter oder in die Feuerung, mit z.B. Zugabe über die zu verbrennende Kohle, so daß alle Schadstoffe thermisch so weit aufgespalten werden, daß sie für die Umwelt nicht mehr schädigend austreten können.From the 1st washing stage, which is used to improve the washout of 502 and / or NO is also operated with carboxylic acids and / or polycarboxylic acids proposed according to the invention, too a partial amount of water in abandon the hottest areas of the raw gas supply, in front of and / or behind the electrostatic precipitator or in the furnace, with e.g. addition over the coal to be burned, so that all Pollutants are broken down thermally to such an extent that they are not harmful to the environment can leak more damaging.

Erfindunsgemä ist der Gedanke in der Weise gegeben, daß grundsätzlich Teilmengen aus dem Waschbereich, aus dem Wasser abgegeben werden muß, dem Rohgasbereich zugeführt werden, in dem durch thermische Zersetzung die Schadstoffe unschädlich gemacht werden.According to the invention, the idea is given in such a way that fundamentally Partial quantities from the scrubbing area from which the water must be released, the raw gas area are supplied in which by thermal decomposition the pollutants are harmless be made.

Patentanspruch;Claim;

Claims (1)

Patentanspruch: Verfahren zur Wandlung von EDUA und Schwefel-Stickstoff-Verbindungen und Carbonsäure-Verbindungen aus Abwässern der S02 und/oder NO##Waschanlagen, dadurch gekennzeichnet, daß eine gewünschte Abwassermenge aus dem Waschwasserkreislauf einer oder gleichzeitig mehrerer oder aller Waschstufen über eine Pumpe einer Düsvorrichtung zugegeben wird, die im Xeißbereich der Rohgase mündet, vorzugsweise im Bereich der Kessel vor und/oder hinter dem Elektrofilter.Claim: Process for converting EDUA and sulfur-nitrogen compounds and carboxylic acid compounds from wastewater from S02 and / or NO ## washing plants, thereby characterized in that a desired amount of waste water from the wash water circuit a or simultaneously several or all washing stages via a pump of a nozzle device is added, which opens in the Xeißbereich the raw gases, preferably in the area of Boiler in front of and / or behind the electrostatic precipitator.
DE19843428691 1984-08-03 1984-08-03 Process for the conversion of EDTA and sulphur-nitrogen compounds from waste waters of NOX scrubber units Withdrawn DE3428691A1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DE19843428691 DE3428691A1 (en) 1984-08-03 1984-08-03 Process for the conversion of EDTA and sulphur-nitrogen compounds from waste waters of NOX scrubber units

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE19843428691 DE3428691A1 (en) 1984-08-03 1984-08-03 Process for the conversion of EDTA and sulphur-nitrogen compounds from waste waters of NOX scrubber units

Publications (1)

Publication Number Publication Date
DE3428691A1 true DE3428691A1 (en) 1986-02-06

Family

ID=6242301

Family Applications (1)

Application Number Title Priority Date Filing Date
DE19843428691 Withdrawn DE3428691A1 (en) 1984-08-03 1984-08-03 Process for the conversion of EDTA and sulphur-nitrogen compounds from waste waters of NOX scrubber units

Country Status (1)

Country Link
DE (1) DE3428691A1 (en)

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2548346A1 (en) * 1974-11-06 1976-05-13 Kureha Chemical Ind Co Ltd Sulphur dioxide removal from combustion gases - by absorption in soln. contg. alkali salt or org. acid and manganous or cupric
DE2619145A1 (en) * 1975-05-06 1976-11-25 Fuji Kasui Eng Co Ltd PROCESS FOR SEPARATING NITROGEN OXYDES AND SIMULTANEOUSLY SEPARATING NITROGEN OXYDE AND SULFUR OXYDE FROM EXHAUST GASES

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2548346A1 (en) * 1974-11-06 1976-05-13 Kureha Chemical Ind Co Ltd Sulphur dioxide removal from combustion gases - by absorption in soln. contg. alkali salt or org. acid and manganous or cupric
DE2619145A1 (en) * 1975-05-06 1976-11-25 Fuji Kasui Eng Co Ltd PROCESS FOR SEPARATING NITROGEN OXYDES AND SIMULTANEOUSLY SEPARATING NITROGEN OXYDE AND SULFUR OXYDE FROM EXHAUST GASES

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
THOME-KOZMIENSKY K.J.: Müllverbrennung und Rauchgasreinigung, 1983, S. 595-609 *

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Legal Events

Date Code Title Description
OM8 Search report available as to paragraph 43 lit. 1 sentence 1 patent law
OP8 Request for examination as to paragraph 44 patent law
8139 Disposal/non-payment of the annual fee