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DE1948185A1 - Continuous measuring equipment for halogen - concentration in gas mixtures - Google Patents

Continuous measuring equipment for halogen - concentration in gas mixtures

Info

Publication number
DE1948185A1
DE1948185A1 DE19691948185 DE1948185A DE1948185A1 DE 1948185 A1 DE1948185 A1 DE 1948185A1 DE 19691948185 DE19691948185 DE 19691948185 DE 1948185 A DE1948185 A DE 1948185A DE 1948185 A1 DE1948185 A1 DE 1948185A1
Authority
DE
Germany
Prior art keywords
halogen
halogens
concentration
cathode
noble metal
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
DE19691948185
Other languages
German (de)
Inventor
Werner Dr Melzer
Helmut Schroeder
Leo Schupmehl
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Hoechst AG
Original Assignee
Hoechst AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoechst AG filed Critical Hoechst AG
Priority to DE19691948185 priority Critical patent/DE1948185A1/en
Publication of DE1948185A1 publication Critical patent/DE1948185A1/en
Pending legal-status Critical Current

Links

Classifications

    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N27/00Investigating or analysing materials by the use of electric, electrochemical, or magnetic means
    • G01N27/62Investigating or analysing materials by the use of electric, electrochemical, or magnetic means by investigating the ionisation of gases, e.g. aerosols; by investigating electric discharges, e.g. emission of cathode
    • G01N27/626Investigating or analysing materials by the use of electric, electrochemical, or magnetic means by investigating the ionisation of gases, e.g. aerosols; by investigating electric discharges, e.g. emission of cathode using heat to ionise a gas

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Physics & Mathematics (AREA)
  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Analytical Chemistry (AREA)
  • Biochemistry (AREA)
  • General Health & Medical Sciences (AREA)
  • General Physics & Mathematics (AREA)
  • Immunology (AREA)
  • Pathology (AREA)
  • Other Investigation Or Analysis Of Materials By Electrical Means (AREA)

Abstract

A precious metal anode and precious metal heated cathode are included in a cell of non-conductive material with an inlet and outlet for the gas under examination. The halogens are dissociated into atoms at the hot cathode, have electrons added to them and are accelerated in a field of between 50 and 500V. Precious metal anode is e.g. Pt and the cathode is e.g. Pt, Pd, Pd Ir, Ir/Nb or Au.

Description

Verfahren und Vorrichtung zum kontinuierlichen Messen von Halogenen Gegenstand der Erfindung ist ein Verfahren und eine Vorrichtung zur kontinuierlichen Konzentrationsmessung von Halogenen bzw. halogenhaltigen Gasen und Dämpfen.Method and device for the continuous measurement of halogens The invention is a method and a device for continuous Concentration measurement of halogens or gases and vapors containing halogens.

Es ist bereits die Halogenlecksuchmethode bekannt. Sie beruht darauf, dass beim Auftreffen von Halogenen oder Halogenverbindungen auf eine glühende Platin-Anode positive Ionen emittiert werden, deren Menge ein Mass für die Leckrate ist. Diese Geräte eignen sich nicht zur kontinuierlichen Konzentrationsmessung von Halogenen bzw, halogenhaltigen Gasen und Dämpfen.The halogen leak detection method is already known. It is based on that when halogens or halogen compounds hit a glowing platinum anode positive ions are emitted, the amount of which is a measure of the leak rate. These Devices are not suitable for continuous measurement of the concentration of halogens or halogen-containing gases and vapors.

Es wurde nun ein Verfahren zur kontinuierlichen Konzentrationsmessung vC>n Halogenen bzw. halogenhaltigen Gasen und Dämpfen gefunden, das dadurch gekennzeichnet ist, dass man die zu messenden Halogen-Moleküle an einer heissen Edelmetall-Kathode, vorzugsweise aus Platin, zu Atomen dissoziiert, ihnen Elektronen anlagert und sie in einem Potentialfeid von - )rOO V beschleunigt.There has now been a method for continuous concentration measurement vC> n halogens or gases and vapors containing halogens found, which is characterized by this is that the halogen molecules to be measured are attached to a hot noble metal cathode, preferably made of platinum, dissociated into atoms, electrons attached to them and they accelerated in a potential field of -) rOO V.

Zur Durchführung des Verfahrens eignet slch ein nicht leitender Behälter (Messzelle), der mit einem Ein- und Auslass für das zu mc:;:;ene Gas versehen ist und worin eine beheizte Edelmetall-Kathode und eine Edelmetall-Anode in bekannter Weise angeordnet sind.A non-conductive container is suitable for carrying out the process (Measuring cell), which is provided with an inlet and outlet for the gas to be mc:;:; ene and wherein a heated noble metal cathode and a noble metal anode in known Way are arranged.

Die Figur zeigt ein Schaltbild einer Messvorrichtung in beispielsweiser Ausführung.The figure shows a circuit diagram of a measuring device in an example Execution.

Das in Bezug auf Halogene zu untersuchende Cas strömt kontinu@erlich durch einen Gaseinlass (9) in eine Messzelle (1), deren Gehause (10)nicht leitend ist und verlässt die Messzelle durch den Gasauslass (11). Die im Gas mitgeführten Halogenmoleküle werden an der heissen Edelmetall-Kathode (2), die z.B. aus Platin, Palladium, Palladium/Iridium, Iridium/Niob oder Gold bestehen kann, negativ ionisiert und von der gegenüber der Kathode angeordneten positiven Platin-Anode (3) angezogen. Der halogenproportionale negative Ionenstrom fliesst über einen hochohmigen Arbeitswiderstand (4) und erzeugt so einen Spannungsabfall, der nach entsprechender Verstärkung (5) mit einem Messgerät (6) angezeigt werden kann. Der Messeffekt ist dabei unter anderem abhängig von Materialart, Oberfläche und Temperatur der Kathode sowie dem Elektrodenabstand; ferner von der elektrischen Feldstärke zwischen den Elektroden und der Gasmenge pro Stünde, die durch die Messzelle strömt.The Cas to be examined with regard to halogens flows continuously through a gas inlet (9) into a measuring cell (1), their housing (10) is not conductive and leaves the measuring cell through the gas outlet (11). the Halogen molecules carried along in the gas are deposited on the hot noble metal cathode (2), which consist e.g. of platinum, palladium, palladium / iridium, iridium / niobium or gold can, negatively ionized and from the positive opposite the cathode Platinum anode (3) tightened. The halogen-proportional negative ion current flows via a high-ohmic working resistor (4) and thus generates a voltage drop, which are displayed with a measuring device (6) after the corresponding amplification (5) can. The measuring effect depends, among other things, on the type of material and surface and temperature of the cathode and the electrode spacing; also from the electrical one Field strength between the electrodes and the amount of gas per hour passing through the measuring cell flows.

Ei.n Teil dieser Einflussgrössen ist durch Auslegung der Messzelle festgelegt4 Die Temperatur der Kathode lässt sich in bekannter Weise durch einen Regelwiderstand (12) im Heizstromkreis, die elektrische Feldstärke durch Ändern der Saugspannung (8) variieren. Der Gasdurchfluss ist ebenfalls mit bekannten Mitteln regelbar.One part of these influencing variables is the design of the measuring cell determined4 The temperature of the cathode can be determined in a known manner by a Variable resistor (12) in the heating circuit, the electric field strength by changing the suction tension (8) vary. The gas flow is also by known means adjustable.

Claims (2)

P a t e n t a n 5 p r U c h eP a t e n t a n 5 p r U c h e lerfahren zur kontinuierlichen Konzentrationsmessung von Halogenen in Gasen, dadurch gekennzeichnet, dass man die zu messenden Halogene an einer heissen Edelmetall-Kathode zu Atomen dissoziiert, ihnen Elektronen anlagert und-sie in einem Potentialfeld von 50 - 500 V beschleunigt.Experience in continuous measurement of the concentration of halogens in gases, characterized in that the halogens to be measured are hot on one Noble metal cathode dissociates into atoms, they attach electrons and they in one Potential field accelerated from 50 - 500 V. 2. Vorrichtung zur Durchführung des Verfahrens nach Anspruch 1 dadurch gekennzeichnet, dass ein nicht leitender Behälter mit einem Ein- und Auslass für das zu untersuchende Gas versehen ist und darin eine geheizte Edelmetall-Kathode und eine Edelmetall-Anode in bekannter Weise angeordnet sind.2. Apparatus for performing the method according to claim 1 thereby characterized in that a non-conductive container with an inlet and outlet for the gas to be examined is provided and in it a heated noble metal cathode and a noble metal anode are arranged in a known manner. L e e r s e i t eL e r s e i t e
DE19691948185 1969-09-24 1969-09-24 Continuous measuring equipment for halogen - concentration in gas mixtures Pending DE1948185A1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DE19691948185 DE1948185A1 (en) 1969-09-24 1969-09-24 Continuous measuring equipment for halogen - concentration in gas mixtures

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE19691948185 DE1948185A1 (en) 1969-09-24 1969-09-24 Continuous measuring equipment for halogen - concentration in gas mixtures

Publications (1)

Publication Number Publication Date
DE1948185A1 true DE1948185A1 (en) 1971-04-01

Family

ID=5746309

Family Applications (1)

Application Number Title Priority Date Filing Date
DE19691948185 Pending DE1948185A1 (en) 1969-09-24 1969-09-24 Continuous measuring equipment for halogen - concentration in gas mixtures

Country Status (1)

Country Link
DE (1) DE1948185A1 (en)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2337885A1 (en) * 1976-01-08 1977-08-05 Westinghouse Electric Corp ALKALINE IONIZATION DETECTOR
EP0015495A1 (en) * 1979-02-27 1980-09-17 Hewlett-Packard Company Electron capture detector

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2337885A1 (en) * 1976-01-08 1977-08-05 Westinghouse Electric Corp ALKALINE IONIZATION DETECTOR
EP0015495A1 (en) * 1979-02-27 1980-09-17 Hewlett-Packard Company Electron capture detector

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