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CN111803390A - Hypochlorous acid water nanogel and preparation method thereof - Google Patents

Hypochlorous acid water nanogel and preparation method thereof Download PDF

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Publication number
CN111803390A
CN111803390A CN202010729988.0A CN202010729988A CN111803390A CN 111803390 A CN111803390 A CN 111803390A CN 202010729988 A CN202010729988 A CN 202010729988A CN 111803390 A CN111803390 A CN 111803390A
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hypochlorous acid
acid water
nanogel
glycerol
trehalose
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Inventor
杨广群
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Guangqun Cosmetics Science And Technology Research Institute Guangzhou Co ltd
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Guangqun Cosmetics Science And Technology Research Institute Guangzhou Co ltd
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    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K8/00Cosmetics or similar toiletry preparations
    • A61K8/02Cosmetics or similar toiletry preparations characterised by special physical form
    • A61K8/04Dispersions; Emulsions
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    • A61K8/8141Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides or nitriles thereof; Compositions of derivatives of such polymers
    • A61K8/8147Homopolymers or copolymers of acids; Metal or ammonium salts thereof, e.g. crotonic acid, (meth)acrylic acid; Compositions of derivatives of such polymers
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    • A61K8/8141Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides or nitriles thereof; Compositions of derivatives of such polymers
    • A61K8/8152Homopolymers or copolymers of esters, e.g. (meth)acrylic acid esters; Compositions of derivatives of such polymers
    • AHUMAN NECESSITIES
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    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K8/00Cosmetics or similar toiletry preparations
    • A61K8/18Cosmetics or similar toiletry preparations characterised by the composition
    • A61K8/72Cosmetics or similar toiletry preparations characterised by the composition containing organic macromolecular compounds
    • A61K8/81Cosmetics or similar toiletry preparations characterised by the composition containing organic macromolecular compounds obtained by reactions involving only carbon-to-carbon unsaturated bonds
    • A61K8/8141Compositions of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by only one carboxyl radical, or of salts, anhydrides, esters, amides, imides or nitriles thereof; Compositions of derivatives of such polymers
    • A61K8/8158Homopolymers or copolymers of amides or imides, e.g. (meth) acrylamide; Compositions of derivatives of such polymers
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    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61PSPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
    • A61P31/00Antiinfectives, i.e. antibiotics, antiseptics, chemotherapeutics
    • A61P31/02Local antiseptics
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    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
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    • A61P31/00Antiinfectives, i.e. antibiotics, antiseptics, chemotherapeutics
    • A61P31/04Antibacterial agents
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    • A61PSPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
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    • A61P31/10Antimycotics
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    • A61QSPECIFIC USE OF COSMETICS OR SIMILAR TOILETRY PREPARATIONS
    • A61Q17/00Barrier preparations; Preparations brought into direct contact with the skin for affording protection against external influences, e.g. sunlight, X-rays or other harmful rays, corrosive materials, bacteria or insect stings
    • A61Q17/005Antimicrobial preparations
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    • A61Q19/00Preparations for care of the skin
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    • A61QSPECIFIC USE OF COSMETICS OR SIMILAR TOILETRY PREPARATIONS
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    • A61Q19/10Washing or bathing preparations
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    • A61K2800/00Properties of cosmetic compositions or active ingredients thereof or formulation aids used therein and process related aspects
    • A61K2800/40Chemical, physico-chemical or functional or structural properties of particular ingredients
    • A61K2800/41Particular ingredients further characterized by their size
    • A61K2800/413Nanosized, i.e. having sizes below 100 nm
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    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61KPREPARATIONS FOR MEDICAL, DENTAL OR TOILETRY PURPOSES
    • A61K2800/00Properties of cosmetic compositions or active ingredients thereof or formulation aids used therein and process related aspects
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Abstract

The invention discloses hypochlorous acid water nanogel and a preparation method thereof, wherein the hypochlorous acid water nanogel is composed of the following raw materials: hypochlorous acid water, glycerol, trehalose and an auxiliary agent, and the preparation method comprises the following steps: under the condition of low temperature, firstly, performing micromolecular treatment on hypochlorous acid water, adding trehalose, and dissolving for later use; dispersing the thickener with glycerol at low temperature; adding hypochlorous acid water into the thickening agent, and soaking for 5-10 minutes until the hypochlorous acid water is completely soaked; homogenizing for 5min, adding neutralizer, and stirring to obtain hypochlorous acid water nanogel. The hypochlorous acid water is subjected to micromolecular treatment, so that the activity of the hypochlorous acid water is stronger, and the hypochlorous acid water can easily penetrate into the deep layer of the skin to be sterilized and cleaned; the hypochlorous acid water which is unstable and difficult to preserve for a long time is gelatinized, the preservation period of the hypochlorous acid water is prolonged, the use is more convenient, the hypochlorous acid water contained in the gel is slowly released, and the utilization efficiency and the use effect are improved.

Description

Hypochlorous acid water nanogel and preparation method thereof
Technical Field
The invention relates to the field of hypochlorous acid water preparation, and particularly relates to hypochlorous acid water nanogel and a preparation method thereof.
Background
Hypochlorous acid is oxyacid of chlorine element, has a chemical formula of HClO and a structural formula of H-O-Cl, wherein the valence of the chlorine element is +1 valence, and is the lowest-valence oxyacid of the chlorine element, but the oxidability of the hypochlorous acid is extremely strong in the oxyacid of the chlorine element, and is the second-strong acid oxidized in the oxyacid of the chlorine element, and the hypochlorous acid exists in a solution only, the concentrated solution is yellow, the dilute solution is colorless and extremely unstable, is a very weak acid which is weaker than carbonic acid and is equivalent to hydrogen sulfuric acid, and the hypochlorous acid has the effects of disinfection, cleaning and sterilization, and can be used for cleaning the face and killing mites.
In the prior art, the hypochlorous acid cleaning agent sold in the market is large in bottled amount, and after the hypochlorous acid cleaning agent is used once, the unspent hypochlorous acid cleaning agent is easy to decompose, is difficult to effectively preserve, easily causes unnecessary resource waste, and needs to be further processed.
Disclosure of Invention
In order to solve the problems, the invention aims to provide hypochlorous acid water nanogel and a preparation method thereof.
In order to achieve the above object, the present invention adopts the following aspects
The hypochlorous acid water nanogel is composed of the following raw materials: hypochlorous acid water, glycerol, trehalose and an auxiliary agent.
Preferably, the hypochlorous acid water nanogel is composed of the following raw materials: hypochlorous acid water, glycerol, trehalose, an ammonium acryloyldimethyl taurate/VP copolymer and deionized water.
Preferably, the hypochlorous acid water nanogel consists of the following raw materials in percentage by mass: 95.7% of hypochlorous acid water, 3% of glycerol, 0.5% of trehalose, 0.5% of acryloyl dimethyl taurate/VP copolymer and 0.3% of deionized water.
Preferably, the hypochlorous acid water nanogel is composed of the following raw materials: hypochlorous acid water, glycerol, trehalose, carbome 20 and triethanolamine.
Preferably, the hypochlorous acid water nanogel consists of the following raw materials in percentage by mass: 95.5% of hypochlorous acid water, 3% of glycerol, 0.5% of trehalose, 200.5% of carbomer and 0.5% of triethanolamine.
Preferably, the hypochlorous acid water nanogel is composed of the following raw materials: hypochlorous acid water, glycerol, trehalose, polyacrylate cross-linked polymer-6 and triethanolamine.
Preferably, the hypochlorous acid water nanogel consists of the following raw materials in percentage by mass: 95.5 percent of hypochlorous acid water, 3 percent of glycerol, 0.5 percent of trehalose, 60.5 percent of polyacrylate cross-linked polymer and 0.5 percent of triethanolamine.
The preparation method of the hypochlorous acid water nanogel comprises the following steps:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing the acryloyl dimethyl ammonium taurate/VP copolymer by using glycerol at low temperature;
s3, adding hypochlorous acid water into the acryloyl dimethyl ammonium taurate/VP copolymer, and soaking for 5-10 minutes until the acryloyl dimethyl ammonium taurate/VP copolymer is completely soaked;
and S4, homogenizing for 5min, adding deionized water, and uniformly stirring to obtain the hypochlorous acid water nanogel.
The preparation method of the hypochlorous acid water nanogel comprises the following steps:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing carbomer U20 with glycerol at low temperature;
s3, adding hypochlorous acid water into carbomer U20, and soaking for 5-10 minutes until carbomer U20 is completely soaked;
and S4, homogenizing for 5min, adding triethanolamine, and stirring uniformly to obtain the hypochlorous acid water nanogel.
The preparation method of the hypochlorous acid water nanogel comprises the following steps:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing the polyacrylate cross-linked polymer-6 with glycerol under the low-temperature condition;
s3, adding hypochlorous acid water into the polyacrylate cross-linked polymer-6, and soaking for 5-10 minutes until the polyacrylate cross-linked polymer-6 is completely foamed;
and S4, homogenizing for 5min, adding triethanolamine, and stirring uniformly to obtain the hypochlorous acid water nanogel.
Preferably, the hypochlorous acid water is reduced in molecular weight by subjecting the hypochlorous acid water to a strong magnetization treatment or irradiating the hypochlorous acid water with far infrared rays to split the molecular groups.
The application of the hypochlorous acid water nanogel can be used as a cosmetic raw material to be added into a cream cosmetic, and the hypochlorous acid water nanogel can be used in the cream to play a triple role, namely, sterilization is performed, a protective layer is formed on skin after the hypochlorous acid water nanogel is used, and external bacteria are isolated; whitening, which can accelerate the metabolism of skin cells, rapidly metabolize melanin and promote the regeneration of horny layer; and thirdly, the preservative is replaced, and other preservatives do not need to be added after the preservative is added.
In the invention:
trehalose, a typical stress metabolite, can form a unique protective film on the cell surface under severe environmental conditions such as high temperature, high cold, high osmotic pressure, dry dehydration and the like, and effectively protects the biomolecular structure from being damaged, thereby maintaining the life process and biological characteristics of a living body.
Acryloyl dimethyl ammonium taurate/VP copolymer, english name: arisroflex AVC, a synthetic polymer, is used as a gelling agent for clear systems and as a thickener for oil-in-water emulsions.
Carbomer U20, cross-linked acrylic acid polymer, INCI name Carbomer, foreign trade name Carbopol, carboxyl groups in Carbomer molecules are neutralized and ionized by alkali, negative charges repel each other, molecular chains are dispersed and stretched, and the Carbomer greatly swells to form transparent gel. A small amount of carbomer can enable the system to have good rheological property, and enable the particles or oil drops to be suspended permanently.
Polyacrylate crosslinked polymer-6, abbreviated as ZEN, high molecular polymer, is used as thickener and film-forming agent in cosmetics.
Triethanolamine, TEA for short, is used as an emulsifier, moisturizer, thickener, PH balancer in cosmetics (including skin washes, eye gels, moisturizers, shampoos, etc.). It is used in cosmetic formulations for neutralization with fatty acids to form soaps and with sulfated fatty acids to form amine salts. The triethanolamine is a common emulsifier in cream preparations, and cream products emulsified by the triethanolamine have the characteristics of fine and smooth cream and bright white cream, and in addition, the colloid phase formed by the triethanolamine and higher fatty acid or higher fatty alcohol has good stability, stable product quality and high specific gravity of the added components. Triethanolamine is the most common neutralizer of acidic polymer gel containing carbomer and the like, and forms a stable polymer structure through neutralization with carboxyl of carbomer, so that the application effects of thickening and moisturizing are achieved.
The invention has the beneficial effects that:
the invention carries out micromolecular treatment on the hypochlorous acid water, so that the activity of the hypochlorous acid water is stronger, and the hypochlorous acid water can be easier to go deep into the skin for sterilization and cleaning.
The hypochlorous acid water which is unstable and difficult to preserve for a long time is gelatinized, the preservation period of the hypochlorous acid water is prolonged, the use is more convenient, the hypochlorous acid water contained in the gel is slowly released, and the utilization efficiency and the use effect are improved.
The hypochlorous acid water nanogel can be directly used for cleaning skin, can also be used as a cosmetic raw material to be added into cream cosmetics and used in the cream to play a triple role, and firstly, sterilization is carried out, a protective layer is formed on the skin after the hypochlorous acid water nanogel is used, and external bacteria are isolated; whitening, which can accelerate the metabolism of skin cells, rapidly metabolize melanin and promote the regeneration of horny layer; and thirdly, the preservative is replaced, and other preservatives do not need to be added after the preservative is added.
Detailed Description
In order to make those skilled in the art better understand the technical solutions in the present application, the following will clearly and completely describe the technical solutions in the present application with reference to the embodiments, and it is obvious that the described embodiments are only a part of the embodiments of the present application, and all other embodiments obtained by a person of ordinary skill in the art without making creative efforts based on the embodiments in the present application shall fall within the protection scope of the present application.
Example 1
The hypochlorous acid water nanogel comprises the following raw materials in percentage by mass: 95.7% of hypochlorous acid water, 3% of glycerol, 0.5% of trehalose, 0.5% of acryloyl dimethyl taurate/VP copolymer and 0.3% of deionized water.
The preparation method of the hypochlorous acid water nanogel comprises the following steps:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing the acryloyl dimethyl ammonium taurate/VP copolymer by using glycerol at low temperature;
s3, adding hypochlorous acid water into the acryloyl dimethyl ammonium taurate/VP copolymer, and soaking for 5-10 minutes until the acryloyl dimethyl ammonium taurate/VP copolymer is completely soaked;
and S4, homogenizing for 5min, adding deionized water, and uniformly stirring to obtain the hypochlorous acid water nanogel.
Example 2
The composite material consists of the following raw materials in percentage by mass: 95.5% of hypochlorous acid water, 3% of glycerol, 0.5% of trehalose, 200.5% of carbomer and 0.5% of triethanolamine.
The preparation method of the hypochlorous acid water nanogel comprises the following steps:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing carbomer U20 with glycerol at low temperature;
s3, adding hypochlorous acid water into carbomer U20, and soaking for 5-10 minutes until carbomer U20 is completely soaked;
and S4, homogenizing for 5min, adding triethanolamine, and stirring uniformly to obtain the hypochlorous acid water nanogel.
Example 3
The hypochlorous acid water nanogel comprises the following raw materials in percentage by mass: 95.5 percent of hypochlorous acid water, 3 percent of glycerol, 0.5 percent of trehalose, 60.5 percent of polyacrylate cross-linked polymer and 0.5 percent of triethanolamine.
The preparation method of the hypochlorous acid water nanogel comprises the following steps:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing the polyacrylate cross-linked polymer-6 with glycerol under the low-temperature condition;
s3, adding hypochlorous acid water into the polyacrylate cross-linked polymer-6, and soaking for 5-10 minutes until the polyacrylate cross-linked polymer-6 is completely foamed;
and S4, homogenizing for 5min, adding triethanolamine, and stirring uniformly to obtain the hypochlorous acid water nanogel.
Experimental example 1
Safety and toxicology experiments
Experiment 1: the experimental mice are divided into three groups, five mice are used in each group, the hypochlorous acid water nanogel prepared in the embodiment 1-3 is smeared on an experimental block on the back of the experimental mouse, the hair is removed, the experiment is carried out twice a day, the hypochlorous acid water nanogel is kept on the experimental part for at least ten minutes each time, the experiment is continuously carried out for 10 days, and whether the surface of the experimental part of the experimental mouse has abnormity or abnormal conditions is observed.
Experiment 2: the experimental mice were divided into three groups of five mice each, and the hypochlorous acid water nanogel prepared in examples 1 to 3 was intragastrically administered to the experimental mice once every three days for three consecutive experiments, and the experimental mice were observed for adverse reactions or death. The results are shown in Table 1.
Figure BDA0002602944310000061
TABLE 1
As can be seen from the experimental data in Table 1, the hypochlorous acid water nanogel prepared by the method has no obvious adverse effect on experimental animals, so that the method is determined to have no adverse reaction or weak adverse reaction, and the use safety is guaranteed.
Experimental example two
Experiment of bactericidal Effect
The hypochlorous acid water nanogels prepared in examples 1 to 3 were subjected to a sterilization effect test, and the sterilization effects were respectively tested by using staphylococcus aureus, colibacillus, candida albicans, bacillus subtilis var niger and poliovirus as examples.
Selecting ten sterile wet tissues, dividing the sterile wet tissues into two groups, respectively dripping five viruses with certain concentrations, then simply cleaning one group, smearing hypochlorous acid water nanogel on all the wet tissues, and sampling at different time points after smearing to detect the virus content.
Table 2 shows experimental data of the hypochlorous acid water nanogel prepared in example 1, table 3 shows experimental data of the hypochlorous acid water nanogel prepared in example 2, and table 4 shows experimental data of the hypochlorous acid water nanogel prepared in example 3.
Figure BDA0002602944310000071
TABLE 2
Figure BDA0002602944310000072
Figure BDA0002602944310000081
TABLE 3
Figure BDA0002602944310000082
TABLE 4
As can be seen from the experimental data in tables 2, 3 and 4, the bactericidal effect of the hypochlorous acid water nanogel prepared by the invention reaches or even exceeds the national requirement on the effect of the hypochlorous acid water on killing microorganisms.
Finally, the above embodiments are only used for illustrating the technical solutions of the present invention and not for limiting, and other modifications or equivalent substitutions made by the technical solutions of the present invention by those of ordinary skill in the art should be covered within the scope of the claims of the present invention as long as they do not depart from the spirit and scope of the technical solutions of the present invention.

Claims (10)

1. The hypochlorous acid water nanogel is characterized by consisting of the following raw materials:
hypochlorous acid water, glycerol, trehalose and an auxiliary agent.
2. The hypochlorous acid water nanogel of claim 1, comprising the following raw materials: hypochlorous acid water, glycerol, trehalose, an ammonium acryloyldimethyl taurate/VP copolymer and deionized water.
3. The hypochlorous acid water nanogel of claim 2, which consists of the following raw materials in percentage by mass: 95.7% of hypochlorous acid water, 3% of glycerol, 0.5% of trehalose, 0.5% of acryloyl dimethyl taurate/VP copolymer and 0.3% of deionized water.
4. The hypochlorous acid water nanogel of claim 1, comprising the following raw materials: hypochlorous acid water, glycerol, trehalose, carbome 20 and triethanolamine.
5. The hypochlorous acid water nanogel of claim 4, which consists of the following raw materials in percentage by mass: 95.5% of hypochlorous acid water, 3% of glycerol, 0.5% of trehalose, 200.5% of carbomer and 0.5% of triethanolamine.
6. The hypochlorous acid water nanogel of claim 1, which consists of the following raw materials in percentage by mass: 95.5 percent of hypochlorous acid water, 3 percent of glycerol, 0.5 percent of trehalose, 60.5 percent of polyacrylate cross-linked polymer and 0.5 percent of triethanolamine.
7. The method of preparing a nanogel of hypochlorous acid as defined in claim 2, comprising the steps of:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing the acryloyl dimethyl ammonium taurate/VP copolymer by using glycerol at low temperature;
s3, adding hypochlorous acid water into the acryloyl dimethyl ammonium taurate/VP copolymer, and soaking for 5-10 minutes until the acryloyl dimethyl ammonium taurate/VP copolymer is completely soaked;
and S4, homogenizing for 5min, adding deionized water, and uniformly stirring to obtain the hypochlorous acid water nanogel.
8. The method of preparing a nanogel of hypochlorous acid as defined in claim 4, comprising the steps of:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing carbomer U20 with glycerol at low temperature;
s3, adding hypochlorous acid water into carbomer U20, and soaking for 5-10 minutes until carbomer U20 is completely soaked;
and S4, homogenizing for 5min, adding triethanolamine, and stirring uniformly to obtain the hypochlorous acid water nanogel.
9. The method of preparing a nanogel of hypochlorous acid as defined in claim 6, comprising the steps of:
s1, under the low temperature condition, firstly, performing micromolecular treatment on hypochlorous acid water, then adding trehalose, and dissolving for later use;
s2, dispersing the polyacrylate cross-linked polymer-6 with glycerol under the low-temperature condition;
s3, adding hypochlorous acid water into the polyacrylate cross-linked polymer-6, and soaking for 5-10 minutes until the polyacrylate cross-linked polymer-6 is completely foamed;
and S4, homogenizing for 5min, adding triethanolamine, and stirring uniformly to obtain the hypochlorous acid water nanogel.
10. The use of the hypochlorous acid aqueous nanogel according to claim 1, wherein the hypochlorous acid aqueous nanogel is used as a cosmetic raw material added to a cream cosmetic to play a triple role in sterilizing, forming a protective layer on the skin after use to isolate external bacteria; whitening, which can accelerate the metabolism of skin cells, rapidly metabolize melanin and promote the regeneration of horny layer; and thirdly, the preservative is replaced, and other preservatives do not need to be added after the preservative is added.
CN202010729988.0A 2020-07-27 2020-07-27 Hypochlorous acid water nanogel and preparation method thereof Pending CN111803390A (en)

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