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CA2675424A1 - Polypropolyne compositions for the manufacture of microporous membranes - Google Patents

Polypropolyne compositions for the manufacture of microporous membranes Download PDF

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Publication number
CA2675424A1
CA2675424A1 CA002675424A CA2675424A CA2675424A1 CA 2675424 A1 CA2675424 A1 CA 2675424A1 CA 002675424 A CA002675424 A CA 002675424A CA 2675424 A CA2675424 A CA 2675424A CA 2675424 A1 CA2675424 A1 CA 2675424A1
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Canada
Prior art keywords
composition
molecular weight
less
polyethylene
microporous membrane
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Granted
Application number
CA002675424A
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French (fr)
Other versions
CA2675424C (en
Inventor
Patrick Brant
Jeffrey L. Brinen
Zerong Lin
Koichi Kono
Kohtaro Kimishima
Hiroyuki Ozaki
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Toray Industries Inc
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Individual
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Publication of CA2675424A1 publication Critical patent/CA2675424A1/en
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    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/10Homopolymers or copolymers of propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F10/00Homopolymers and copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F10/04Monomers containing three or four carbon atoms
    • C08F10/06Propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F210/00Copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F210/04Monomers containing three or four carbon atoms
    • C08F210/06Propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/10Homopolymers or copolymers of propene
    • C08L23/14Copolymers of propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/10Homopolymers or copolymers of propene
    • C08L23/14Copolymers of propene
    • C08L23/142Copolymers of propene at least partially crystalline copolymers of propene with other olefins
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F110/00Homopolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F110/02Ethene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F110/00Homopolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F110/04Monomers containing three or four carbon atoms
    • C08F110/06Propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/04Homopolymers or copolymers of ethene
    • C08L23/06Polyethene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/04Homopolymers or copolymers of ethene
    • C08L23/08Copolymers of ethene
    • C08L23/0807Copolymers of ethene with unsaturated hydrocarbons only containing four or more carbon atoms
    • C08L23/0815Copolymers of ethene with unsaturated hydrocarbons only containing four or more carbon atoms with aliphatic 1-olefins containing one carbon-to-carbon double bond
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/04Homopolymers or copolymers of ethene
    • C08L23/08Copolymers of ethene
    • C08L23/0846Copolymers of ethene with unsaturated hydrocarbons containing atoms other than carbon or hydrogen
    • C08L23/0853Ethene vinyl acetate copolymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L23/00Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
    • C08L23/02Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
    • C08L23/04Homopolymers or copolymers of ethene
    • C08L23/08Copolymers of ethene
    • C08L23/0846Copolymers of ethene with unsaturated hydrocarbons containing atoms other than carbon or hydrogen
    • C08L23/0869Copolymers of ethene with unsaturated hydrocarbons containing atoms other than carbon or hydrogen with unsaturated acids, e.g. [meth]acrylic acid; with unsaturated esters, e.g. [meth]acrylic acid esters
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10Energy storage using batteries

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Manufacture Of Porous Articles, And Recovery And Treatment Of Waste Products (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
  • Cell Separators (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
  • Laminated Bodies (AREA)

Abstract

Disclosed herein is a polymer composition, its manufacture and use, said composition may comprise greater than about 90 mole % propylene monomer, and having a unique combination of properties, including one or more of the following: a heat of fusion of more than about 108 J/g, a melting point of 165°C or higher, a Melt Flow Rate so low that it is essentially not measurable and a molecular weight of greater than about 1.5 x 106. Further disclosed herein are blends or mixtures of the present novel polymer composition and products, such as, for example, microporous film structures and the like comprising same.

Claims (20)

1. A polymeric composition comprising greater than 90 mole % propylene monomer, said composition having an intrinsic viscosity greater than 10 dl/g, a heat of fusion greater than 108 J/g, a melting point of 165°C or greater, a molecular weight greater than 1.5 x 10 6, a molecular weight distribution of from 2.5 to 7, a Melt Flow Rate at 230 °C of less than 0.01 dg/minute, an amount of extractable species of 0.5 wt.% or less based on the weight of the polymeric composition, and stereo defects less than 50 per 10,000 carbon atoms.
2. The polymeric composition of claim 1 having an mmmm pentad fraction of greater than 96 mol% mmmm pentads.
3. The polymeric composition of claims 1 or 2 comprising greater than 99.99 mol%
propylene monomer.
4. The polymeric composition of any of claims 1 - 3 having a molecular weight greater than 1.75 x 10 6.
5. The polymeric composition of any of claims 1 - 4 having an intrinsic viscosity greater than 11 dl/g, a heat of fusion greater than 110 J/g, a melting point of 166°C or greater, a molecular weight greater than 1.5 x 10 6, a molecular weight distribution of from 2.5 to 7, a Melt Flow Rate at 230 °C of less than 0.01 dg/minute, and stereo defects less than 40 per 10,000 carbon atoms.
6. The polymeric composition any of claims 1 - 5 comprising greater than 95 mole %
propylene monomer.
7. The polymeric composition of claim 5 comprising greater than 99.99 mole %
propylene monomer.
8. The polymeric composition of claim 5 having a molecular weight greater than 2.0 x 10 6.
9. The polymeric composition any of claims 1 - 8 and a second polyolefin.
10. A composition comprising polyethylene and a propylene polymer composition comprising greater than 90 mole % propylene monomer, said propylene polymer composition having an intrinsic viscosity greater than 10 dl/g, a heat of fusion greater than 108 J/g, a melting point of 165°C or greater, a molecular weight greater than 1.5 x 10 6, a molecular weight distribution of from 2.5 to 7, a Melt Flow Rate at 230 °C of less than 0.2 dg/minute, and stereo defects less than 50 per 10,000 carbon atoms.
11. The composition of claim 10 wherein the polyethylene comprises a first polyethylene having a molecular weight of 5 x 10 5 or more, a second polyethylene having a molecular weight of 1 x 10 4 or more and less than 5 x 10 5, or both the first and second polyethylenes.
12. The composition of claims 10 or 11, wherein the first polyethylene comprises ultra high molecular weight polyethylene and the second polyethylene comprises at least one of high-density polyethylene, medium-density polyethylene, branched low-density polyethylene, and linear low-density polyethylene.
13. The composition of any of claims 10 - 12 wherein the ultra high molecular weight polyethylene is an ethylene homopolymer or an ethylene/.alpha.-olefin copolymer containing a small amount of an .alpha.-olefin other than ethylene.
14. The composition of any of claims 10 - 13 wherein the propylene polymer composition has an intrinsic viscosity greater than 11 dl/g, a heat of fusion greater than 110 J/g, a melting point of 166°C or greater, a molecular weight greater than 1.5 x 10 6, a molecular weight distribution of from 2.5 to 7, a Melt Flow Rate at 230 °C of less than 0.01 dg/minute, an amount of extractable species of 0.5 wt.% or less based on the weight of the propylene polymer composition, and stereo defects less than 40 per 10,000 carbon atoms.
15. A microporous membrane comprising the composition of any of claims 10 -14.
16. A battery comprising an anode, a cathode, an electrolyte, and the microporous membrane of claim 15, wherein the microporous membrane is located at least between the anode and the cathode.
17. A method for producing a microporous membrane comprising the steps of (1) combining a diluent or solvent and a first polyolefin composition prepare a first polyolefin solution, the first polyolefin composition comprising greater than 90 mole %
propylene monomer and having one or more of the following (a) an intrinsic viscosity greater than 10 dl/g, (b) a heat of fusion greater than 108 J/g, a melting point of 165°C or greater, (c) a molecular weight greater than 1.5 x 10 6, (d) a molecular weight distribution of from 2.5 to 7, (e) a Melt Flow Rate at 230°C of less than 0.01 dg/minute, (f) an amount of extractable species of 0.5 wt.% or less based on the weight of the polyolefin composition, (g) a meso pentad fraction of greater thatn 96 mol% mmmm pentads, and (h) an amount of stereo defects less than 50 per 10,000 carbon atoms;
(3) extruding the first polyolefin solution through at least one die to form an extrudate, (5) removing at east a portion of the membrane-forming solvent from the cooled extrudate or extrudate to form a solvent-removed sheet, and (6) removing any volatile species from the sheet, e.g., by drying, to form the microporous membrane.
18. The method of claim 17, further comprising (7) stretching the microporous membrane after step (6), (8) contacting the microporous membrane with a hot solvent between steps (4) and (7), ment step (8), etc. can be conducted between steps (4) and (5), and after step (6), conducting one or more of (9) stretching the microporous membrane and (10) cross-linking step the microporous membrane using ionizing radiation.
19. The method of claim 17, further comprising (2) combining a second polyolefin composition and a second membrane-forming solvent to prepare a second polyolefin solution, and extruding the second polyolefin solution through at least one die to form a multilayer extrudate
20. The method of claims 17 or 19 further comprising (4) cooling the extrudate to form a cooled extrudate prior to step (5).
CA2675424A 2007-01-19 2008-01-17 Polypropolyne compositions for the manufacture of microporous membranes Active CA2675424C (en)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
US88124707P 2007-01-19 2007-01-19
US60/881,247 2007-01-19
PCT/US2008/051352 WO2008140835A1 (en) 2007-01-19 2008-01-17 Polymeric material and its manufacture and use

Publications (2)

Publication Number Publication Date
CA2675424A1 true CA2675424A1 (en) 2008-11-20
CA2675424C CA2675424C (en) 2012-04-03

Family

ID=37963782

Family Applications (1)

Application Number Title Priority Date Filing Date
CA2675424A Active CA2675424C (en) 2007-01-19 2008-01-17 Polypropolyne compositions for the manufacture of microporous membranes

Country Status (7)

Country Link
EP (1) EP2104711A1 (en)
JP (1) JP2010516842A (en)
KR (1) KR101126916B1 (en)
CN (1) CN101641406B (en)
CA (1) CA2675424C (en)
TW (1) TW200904883A (en)
WO (1) WO2008140835A1 (en)

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KR101630473B1 (en) * 2009-01-07 2016-06-14 가부시키가이샤 프라임 폴리머 Polypropylene resin composition for microporous film formation
SG174386A1 (en) * 2009-03-17 2011-10-28 Prime Polymer Co Ltd Polypropylene for film capacitor, polypropylene sheet for film capacitor, method for producing the same, and uses of the same
CN102355938B (en) 2009-03-30 2014-09-10 东丽电池隔膜株式会社 Microporous membrane and methods of making and using the same
CN102414014B (en) 2009-04-23 2015-01-14 东丽电池隔膜株式会社 Thermoplastic film, methods for making such film, and use of such film as battery separator film
EP2421699A1 (en) 2009-04-23 2012-02-29 Toray Tonen Specialty Separator Godo Kaisha Thermoplastic film, methods for making such film, and the use of such film as battery separator film
JP2012530802A (en) 2009-06-19 2012-12-06 東レバッテリーセパレータフィルム株式会社 Microporous membranes, methods for producing such membranes, and use of such membranes as battery separator films
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WO2011074696A1 (en) 2009-12-18 2011-06-23 Toray Tonen Specialty Separator Godo Kaisha Microporous membranes, methods for making same and their use as battery separator films
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CN112724509B (en) * 2020-12-18 2022-08-09 金发科技股份有限公司 Polypropylene composite material and preparation method and application thereof
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Also Published As

Publication number Publication date
CN101641406A (en) 2010-02-03
KR101126916B1 (en) 2012-03-21
WO2008140835A1 (en) 2008-11-20
CA2675424C (en) 2012-04-03
CN101641406B (en) 2012-12-26
EP2104711A1 (en) 2009-09-30
WO2008140835A8 (en) 2009-08-20
TW200904883A (en) 2009-02-01
KR20090116745A (en) 2009-11-11
JP2010516842A (en) 2010-05-20

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