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CA1160988A - Apparatus for regenerating active carbon - Google Patents

Apparatus for regenerating active carbon

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Publication number
CA1160988A
CA1160988A CA000351085A CA351085A CA1160988A CA 1160988 A CA1160988 A CA 1160988A CA 000351085 A CA000351085 A CA 000351085A CA 351085 A CA351085 A CA 351085A CA 1160988 A CA1160988 A CA 1160988A
Authority
CA
Canada
Prior art keywords
active carbon
desorption
carrier passage
particles
adsorbed material
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
CA000351085A
Other languages
French (fr)
Inventor
Osamu Mihara
Yoyoji Kumada
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Individual
Original Assignee
Individual
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Individual filed Critical Individual
Application granted granted Critical
Publication of CA1160988A publication Critical patent/CA1160988A/en
Expired legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/28Treatment of water, waste water, or sewage by sorption
    • C02F1/283Treatment of water, waste water, or sewage by sorption using coal, charred products, or inorganic mixtures containing them
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01JCHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J19/00Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J19/08Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor
    • B01J19/087Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor employing electric or magnetic energy
    • B01J19/088Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor employing electric or magnetic energy giving rise to electric discharges
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01BNON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B32/00Carbon; Compounds thereof
    • C01B32/30Active carbon
    • C01B32/354After-treatment
    • C01B32/36Reactivation or regeneration
    • C01B32/366Reactivation or regeneration by physical processes, e.g. by irradiation, by using electric current passing through carbonaceous feedstock or by using recyclable inert heating bodies

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Toxicology (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Environmental & Geological Engineering (AREA)
  • Water Supply & Treatment (AREA)
  • Engineering & Computer Science (AREA)
  • Hydrology & Water Resources (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Solid-Sorbent Or Filter-Aiding Compositions (AREA)
  • Carbon And Carbon Compounds (AREA)

Abstract

Abstract of the Disclosure The disclosure teaches an apparatus for re-generating active carbon, in which a pulse voltage is applied so as to generate spark discharges between particles of used active carbon and desorb the ad-sorbed material. Thus a greater amount of spark dis-charge is generated and the desorption of the adsorbed material can be performed more easily and efficiently.
And by adjusting pulse width, temperature control dur-ing the operation is made possible, therefore, useful adsorbed material can be recovered without decomposition, and harmful and useless substance can be decomposed or burnt out at elevated temperature. In the continuous regeneration apparatus, a number of baffle boards are provided on the suitable portion of the swinging carrier path of the active carbon to intercept the fed active carbon particles temporarily and pass the same selec-tively according to the order of desorption degree, to make the process of desorption more perfectly.

Description

1 1 6~88 This invention relates to an apparatus for regenerating used active carbon.
The purification treatment of waste gas or water discharged from factories and other facilities has been an important problem for a long time, and recently it became a more urgent problem, as the polu-tion problem became a subject of much discussion.
Many processes of the treating waste gas or water have been proposed, but among these a process of using ac-tive carbon is widely adopted.
Active carbon is a favorable reagent becauseof its strong adsorptive power, but it must be regen-erated in case of reuse, when it becomes inactive as the adsorption goes on and saturated with adsorbed matter. In the conventional method for activating and regenerating used active carbon, the same is heated, as for instance, in an oil fired rotary kiln at a temp-erature of 800C or higher, and the water vapor is introduced concurrently to regenerate the carbon by a process of water gas reaction.

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.

' 1 1 60~8~

However, this method requires a long time heating at such high temperature, so that it needs a considerable amount of fuel, as well as, an expensive installation cost.
Further, there is an excessive burning loss of the active carbon There is also an use of Juole's heat generated by conducting electric current through the active carbon for heating the same and desorbing or liberating adsorbed material, but this method also needs e~pensive installation cost, especially for the electrical equipment, as it requires very heavy current.
After repeating many experiments to find out an efficient and economical method for regenerating used active carbon, one of the inventors of the present invention develop-ed and disclosed an apparatus, in which a vibration is applied to the active carbon powder while conducting electric current so as to generate spark discharge 6 between particles of the active carbon and liberate the adsorbed material.
(For reference:
Publication of Japanese Patent Application Disclosure No.52-6393 and Japanese Utility Model Registration Application . Disclosure No.52-14351) However, it was found that this process still has the following disadvantages:

,:.

1 1 6~88 With carbon particles which contact longer time with each other, Joule's heat generates locally and consumes much amount of current, and this causes lowering of efficiency. This also causes difficulties in controll-ing temperature during the operation, and becomes diff-icult to recover liberated or desorbed material, even if it is useful, as it decomposes at such high temper-ature caused by Joule's heat.
The present invention relates particularly to improvements in an apparatus for carrying out the above-mentioned spark discharge process for activating and regenerating used active carbon, and characterized in that the apparatus includes means for applying a pulse voltage between the used active carbon particles so as to generate spark discharges therebetween and desorb the adsorbed material. Thus the occurrence of the spark discharge between carbon particles increases extremely and the generation of Joule's heat decreases, so that desorption of the adsorbed material can be performed more easily and efficiently.
Another advantage of this apparatus is to be able to control temperature during the desorption by adjusting pulse width of the applied voltage, i.e., if the adsorbed material is useful, it can be recovered without decomposition, by desorbing at relatively low temperature. On the contrary, if the adsorbed material is harmful and useless, it can be decomposed or burnt out on the place, by desorbing at high temperature. Further, by applying a swinging motion to the carbon particles additionally, occurrence of the spark discharges, accordingly the desorption of t:he adsorbed material can be accelerated. Further in a continuous regeneration apparatus of the present inven-tion, a number of baffle boards are provided on the suitable portion of swinging carrier passage of the active carbon particles so as to intercept the same tem-porarily and pass them selectively by overflowing from the lightened particles due to desorption in order, to make desorption process more perfectly. The present in-vention will be described in more details with reference to the accompanying drawings.
Accordingly, in accordance with the invention, there is provided an apparatus for regenerating active carbon. The apparatus includes a box type desorption tank for desorbing adsorbed material. The bottom of the tank is slanted lengthwise and has a channel forming a carrier passage of the active carbon formed on the bottom with an inlet port on the upper end and an outlet port on the lower end thereof. A swinging means swings the desorption tank to cause flow of the active carbon particles from the inlet port to the outlet port within the carrier passage. Electrodes means are provided within and along the carrier passage for applying a spark discharge voltage to the carbon particles to desorb adsorbed material therein. Intercepting means are pro-vided at suitable length intervals in the carrier passage for intercepting flow of active carbon in the carrier passage and overflowing the lightened particles caused by the desorption in turn. A generating apparatus gene-rates pulse voltage to be applied to the electrode means.
Fig. 1 is a front view illustrating an embo-diment of the apparatus for regenerating active carbon according to the present invention' 1 ~ 60988 Fig. 2 is a side elevational view of the appa-ratus shown in Fig. 1, Fig. 3 is an enlarged cross-sectional view, taken along line III-III of Fig. 1, Fig. 4 is a schematic view showing an example of waste water purification apparatus using the regener-ation apparatus according to the present invention.

-4a-.~

1 I B~988 Fig.5 is an example of wave forms of the applied voltage during the process of the present invention.

Best Mode for Carrying Out the Invention AS seen in Figures 1-3, the apparatus for regenerating active carbon includes a box type desorption tank 1, the bottom of which is slanted lengthwise at a suitable angle, and inside surface thereof is lined with refractory material
2, and a channel form carrier passage "a" is formed thereon for carrying active carbon powders. Refractory mo~tar such as LIGHT CASTER or PLYCAST~R sold by PLIBRICO CO. or the like refractory material of good insulation quality may by used for the lining material 2. Carbon electrodes 3,
3--- of plate form are provided within and along said carrier passage "a", each disposed opposedly. Carbon rods may be used also for the electrodes 3. A number of baffle boards
4, 4--- of suitable height and made'of the similar refractory material as lining material 2, are provided within the carrier passage "a". The same are disposed suitably spaced ~20 apart with each other. S is a dehydrator of the used active carbon, having screen 5' for filtering water. 6 is an - outlet port of the regenerated active carbon. 7 is an exhaust port of the desorbed gas. 8 is electrode terminal.
Thro~gh bearings 12, 12, the lower end of the slanted bottom of desorption tank 1 is mounted on an eccentric journal 11' 1 1 6~8 of a rotary shaft 11 which is supported on a base frame 9 through bearings 10, 10. The rotary shaft 11 is connected with a motor 16 through a pulley 13 mounted on the shaft, belt 14 and a small pulley 15 of the motor.
The upper end of the slanted bottom of tank 1 is supported on the base frame 9 through a spring 17. The apparatus will be operated as follows:
By starting the motor 16, desorption tank 1 may swing vertically and longitudinally, while each part thereof moving circularly. Then by charging used active carbon into the dehydrator 5, the wet carbon powders are dehydrated by the screen 5' and fed on upper end of the carrier passage "a" through opening 18. The powders advance downwards on the slanted passage "a" while being intercepted by the baffle boards 4, 4, -- temporarily, and discharged from the outlet port 6. During this operation, pulse voltage of the form as shown in Fig.5 is applied between the electrodes 3, 3---. By the application of pulse voltage, or by the combination of pulse voltage and swinging motion of the passage "a", a greater amount of spark discharges are gener-ated between active carbon particles, so that the desorption is accelerated and can be accomplished within a very short period of several to a dozen or so minutes. For generating pulse voltage, thylistor chopper or thyIistor Leonard system, as for example, may be used. (In this example, thylistor 1 1~û98~

chopper system was used.) Further, one of the eminent advantages of this method is to be able to control temperature during the desorbing process, by adjusting pulse width "t".
For example, with the pulse width of about 5-10 microsec. at an applied voltage of 200-500V, the temperature rise is minimlzed, so that the useful adsorbed material can be recovered as it is desorbed without decomposition.
Further, loss of the carbon electrodes may be reduced to about 1/100 of that in the prior art. On the contrary, with the pulse width of about 1-10 millisec., temperature rises up to 600-700C within several minutes, so that the harmful substance can be decomposed and burnt out immediately on desorption. Either A.C. wave form as shown in Fig.5, ~S or D.C. wave form without changing of polarity may be used for the pulse voltage. The used active carbon which has been fed on the carrier path-"a" ana intercepted by each baffle board 4, desorb the adsorbed material while repeating swinging motion. And lightened particles due to desorption move upwards and overflow the board 4, and then intercepted by the next board, thus the desorption goes on progressively, and, at the final stage, the active carbon of almost completely activated and regenerated are taken out from the outlet port 6. This desorption tank 1 with baffle boards 4, 4 can be used also for the regeneration apparatus of the above-1 1 6~988 mentioned prior art in which the usual-not pulsative-voltage application and vibration are used. Fig.4 shows one example of continuous purification apparatus of the waste water, in which the regenera~ion apparatus according S to the present invention is used. In the figure, 19 is an adsorption tank containing active carbon 20 as adsorbent.
21 is a dryer, 22 is a regeneration apparatus of the present invention, 23 is a storage tank of the regenerated active carbon, 24 is a feed pump. In this example, the dryer 21 is of the similar construction as regeneration apparatus 22, and provided with dehydrator 25 on the upper part thereof, but drying oven with an usual heating means such as hot blasting may be used also.
The apparatus will be operated as follows:
The waste water which flowed into the tank 19 through an inlet port 26, passes through filter screen 27 and removed of the harmful material by the adsorption while passing through layers of the adsorbent 20, and discharged from outlet port 28 as purified water. Used active carbon 20 is discharged through a discharge port 29 provided on the bottom of the tank 19, about constant amount at every predetermined time intervals by means of an automatic dis-charging apparatus 30. The powder 20 is dehydrated at the dehydrator 25, then dried at the dryer 21. If the powder 20 is accompanied with sludges, the same may be carbonized 1 ~ ~Q~88 or burnt out at this stage. The dried powder 20 is then activated and regenerated at the regeneration apparatus 22 in the similar manner as described above, and sent to the storage tank 23 as regenerated active carbon powder, and sent back to the adsorption tank 19 by means of feed pump 24.
Thus, by repeating these processes, purification of the water as well as regeneration of the used active carbon can be performed automatically and continuously without stopping the flow of water.
As mentioned above, in the present invention, by apply-ing pulse voltage a greater amount of spark discharge is generated so that the desorption of adsorbed material can be performed more easily and efficiently. Another advantage of the present invention is that by adjusting pulse width, it becomes possible to control temperature during the desorp-tion. Further, in the continuous regeneration apparatus, by providing baffIe boards within the swinging carrier path, it also becomes possible to pass the active carbon particles selectively according to the order of desorption degree.
As a result, according to the method and apparatus of the present invention the desorption is exceedingly accelerated and highly activated active carbon can be obtained within a relatively short time interval. In the above examples, ad~ustment of the pulse width was performed without changing cycles. Cycles of 50-400Hz were used in the examples.

Claims (2)

The embodiments of the invention in which an exclusive property or privilege is claimed are defined as follows:-
1. An apparatus for regenerating active carbon comprising: a box type desorption tank for desorbing adsorbed material, the bottom of which being slanted lengthwise and having a channel form a carrier passage of the active carbon formed on said bottom with an inlet port on the upper end and an outlet port on the lower end thereof, a swinging means to swing said desorption tank to cause flow of the active carbon particles from said inlet port to said outlet port within said carrier passage: electrode means provided within and along said carrier passage for applying a spark discharge voltage to said carbon particles to desorb adsorbed material therein, intercepting means provided at suitable length intervals in said carrier passage for intercepting flow of active carbon in said carrier passage and overflowing the lightened particles caused by said desorption in turn:
and a generating apparatus for generating pulse voltage to be applied to said electrode means.
2. The apparatus claimed in claim 1 wherein:
said generating apparatus is capable of adjusting pulse width.
CA000351085A 1979-05-11 1980-05-01 Apparatus for regenerating active carbon Expired CA1160988A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
PCT/JP1979/000119 WO1980002553A1 (en) 1979-05-11 1979-05-11 Method of regeneration of activated carbon and apparatus therefor
JP79/00119 1979-05-11

Publications (1)

Publication Number Publication Date
CA1160988A true CA1160988A (en) 1984-01-24

Family

ID=13677656

Family Applications (1)

Application Number Title Priority Date Filing Date
CA000351085A Expired CA1160988A (en) 1979-05-11 1980-05-01 Apparatus for regenerating active carbon

Country Status (11)

Country Link
AU (1) AU5820580A (en)
BE (1) BE883200A (en)
BR (1) BR7909006A (en)
CA (1) CA1160988A (en)
DE (1) DE2953672A1 (en)
DK (1) DK6881A (en)
FR (1) FR2455922A1 (en)
GB (1) GB2060595A (en)
IT (1) IT1209327B (en)
NL (1) NL8002677A (en)
WO (1) WO1980002553A1 (en)

Families Citing this family (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
AU7033681A (en) * 1981-04-10 1982-11-04 Sasaki, Y. Apparatus for regenerating activated carbon
DE3141906A1 (en) * 1981-10-08 1983-04-21 Degussa Ag, 6000 Frankfurt METHOD AND DEVICE FOR CARRYING OUT GAS / SOLID REACTIONS, IN PARTICULAR FOR ACTIVATING AND REACTIVATING ACTIVE CARBON
DE4104513C2 (en) * 1990-02-14 1996-11-28 Chmiel Horst Adsorber
CN110538647A (en) * 2019-10-14 2019-12-06 中国科学院过程工程研究所 An activated carbon desulfurization and denitrification regeneration system
CN111235403B (en) * 2020-03-01 2022-06-03 长春黄金研究院有限公司 Method for reducing high-grade powdered carbon in desorption electrolysis section

Family Cites Families (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS526393A (en) * 1975-07-05 1977-01-18 Mihara Kankyo Gijutsu Kk Regenerator of active carbon
JPS5342194A (en) * 1976-09-29 1978-04-17 Chubu Kk Apparatus for continuously regenerating active carbon
JPS546892A (en) * 1977-06-20 1979-01-19 Minoru Tanmachi Method and apparatus for regenerating active carbon

Also Published As

Publication number Publication date
BR7909006A (en) 1981-04-14
AU5820580A (en) 1980-11-13
NL8002677A (en) 1980-11-13
DE2953672A1 (en) 1982-01-28
IT1209327B (en) 1989-07-16
IT8021961A0 (en) 1980-05-09
WO1980002553A1 (en) 1980-11-27
BE883200A (en) 1980-09-01
FR2455922A1 (en) 1980-12-05
GB2060595A (en) 1981-05-07
DK6881A (en) 1981-01-08

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