MX166556B - Composiciones sulfuradas y concentrados de aditivos y aceites lubricantes que las contienen - Google Patents
Composiciones sulfuradas y concentrados de aditivos y aceites lubricantes que las contienenInfo
- Publication number
- MX166556B MX166556B MX014544A MX1454489A MX166556B MX 166556 B MX166556 B MX 166556B MX 014544 A MX014544 A MX 014544A MX 1454489 A MX1454489 A MX 1454489A MX 166556 B MX166556 B MX 166556B
- Authority
- MX
- Mexico
- Prior art keywords
- compositions
- fatty acid
- concentrates
- sulfurated
- additives
- Prior art date
Links
Classifications
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- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M135/00—Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing sulfur, selenium or tellurium
- C10M135/02—Sulfurised compounds
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- C—CHEMISTRY; METALLURGY
- C07—ORGANIC CHEMISTRY
- C07G—COMPOUNDS OF UNKNOWN CONSTITUTION
- C07G99/00—Subject matter not provided for in other groups of this subclass
- C07G99/002—Compounds of unknown constitution containing sulfur
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- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M135/00—Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing sulfur, selenium or tellurium
- C10M135/02—Sulfurised compounds
- C10M135/04—Hydrocarbons
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- C10M135/00—Lubricating compositions characterised by the additive being an organic non-macromolecular compound containing sulfur, selenium or tellurium
- C10M135/02—Sulfurised compounds
- C10M135/06—Esters, e.g. fats
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- C10M2201/00—Inorganic compounds or elements as ingredients in lubricant compositions
- C10M2201/087—Boron oxides, acids or salts
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- C10M2203/00—Organic non-macromolecular hydrocarbon compounds and hydrocarbon fractions as ingredients in lubricant compositions
- C10M2203/06—Well-defined aromatic compounds
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- C10M—LUBRICATING COMPOSITIONS; USE OF CHEMICAL SUBSTANCES EITHER ALONE OR AS LUBRICATING INGREDIENTS IN A LUBRICATING COMPOSITION
- C10M2205/00—Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
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- C10M2205/00—Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions
- C10M2205/02—Organic macromolecular hydrocarbon compounds or fractions, whether or not modified by oxidation as ingredients in lubricant compositions containing acyclic monomers
- C10M2205/026—Butene
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- C10M2207/00—Organic non-macromolecular hydrocarbon compounds containing hydrogen, carbon and oxygen as ingredients in lubricant compositions
- C10M2207/10—Carboxylix acids; Neutral salts thereof
- C10M2207/12—Carboxylix acids; Neutral salts thereof having carboxyl groups bound to acyclic or cycloaliphatic carbon atoms
- C10M2207/125—Carboxylix acids; Neutral salts thereof having carboxyl groups bound to acyclic or cycloaliphatic carbon atoms having hydrocarbon chains of eight up to twenty-nine carbon atoms, i.e. fatty acids
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- C10M2207/10—Carboxylix acids; Neutral salts thereof
- C10M2207/12—Carboxylix acids; Neutral salts thereof having carboxyl groups bound to acyclic or cycloaliphatic carbon atoms
- C10M2207/129—Carboxylix acids; Neutral salts thereof having carboxyl groups bound to acyclic or cycloaliphatic carbon atoms having hydrocarbon chains of thirty or more carbon atoms
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- C10M2209/00—Organic macromolecular compounds containing oxygen as ingredients in lubricant compositions
- C10M2209/02—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
- C10M2209/08—Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds containing monomers having an unsaturated radical bound to a carboxyl radical, e.g. acrylate type
- C10M2209/084—Acrylate; Methacrylate
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- C10M2215/02—Amines, e.g. polyalkylene polyamines; Quaternary amines
- C10M2215/04—Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to acyclic or cycloaliphatic carbon atoms
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- C10M2215/042—Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to acyclic or cycloaliphatic carbon atoms containing hydroxy groups; Alkoxylated derivatives thereof
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- C10M2215/02—Amines, e.g. polyalkylene polyamines; Quaternary amines
- C10M2215/06—Amines, e.g. polyalkylene polyamines; Quaternary amines having amino groups bound to carbon atoms of six-membered aromatic rings
- C10M2215/064—Di- and triaryl amines
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- C10M2215/00—Organic non-macromolecular compounds containing nitrogen as ingredients in lubricant Compositions
- C10M2215/24—Organic non-macromolecular compounds containing nitrogen as ingredients in lubricant Compositions having hydrocarbon substituents containing thirty or more carbon atoms, e.g. nitrogen derivatives of substituted succinic acid
- C10M2215/26—Amines
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- C10M2217/02—Macromolecular compounds obtained from nitrogen containing monomers by reactions only involving carbon-to-carbon unsaturated bonds
- C10M2217/024—Macromolecular compounds obtained from nitrogen containing monomers by reactions only involving carbon-to-carbon unsaturated bonds containing monomers having an unsaturated radical bound to an amido or imido group
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- C10M2217/04—Macromolecular compounds from nitrogen-containing monomers obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds
- C10M2217/046—Polyamines, i.e. macromoleculars obtained by condensation of more than eleven amine monomers
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- C10M2217/06—Macromolecular compounds obtained by functionalisation op polymers with a nitrogen containing compound
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- C10M2219/00—Organic non-macromolecular compounds containing sulfur, selenium or tellurium as ingredients in lubricant compositions
- C10M2219/02—Sulfur-containing compounds obtained by sulfurisation with sulfur or sulfur-containing compounds
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- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2040/00—Specified use or application for which the lubricating composition is intended
- C10N2040/25—Internal-combustion engines
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2040/00—Specified use or application for which the lubricating composition is intended
- C10N2040/25—Internal-combustion engines
- C10N2040/251—Alcohol-fuelled engines
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2040/00—Specified use or application for which the lubricating composition is intended
- C10N2040/25—Internal-combustion engines
- C10N2040/255—Gasoline engines
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2040/00—Specified use or application for which the lubricating composition is intended
- C10N2040/25—Internal-combustion engines
- C10N2040/255—Gasoline engines
- C10N2040/28—Rotary engines
-
- C—CHEMISTRY; METALLURGY
- C10—PETROLEUM, GAS OR COKE INDUSTRIES; TECHNICAL GASES CONTAINING CARBON MONOXIDE; FUELS; LUBRICANTS; PEAT
- C10N—INDEXING SCHEME ASSOCIATED WITH SUBCLASS C10M RELATING TO LUBRICATING COMPOSITIONS
- C10N2070/00—Specific manufacturing methods for lubricant compositions
- C10N2070/02—Concentrating of additives
Landscapes
- Chemical & Material Sciences (AREA)
- Organic Chemistry (AREA)
- Chemical Kinetics & Catalysis (AREA)
- General Chemical & Material Sciences (AREA)
- Oil, Petroleum & Natural Gas (AREA)
- Lubricants (AREA)
- Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
Abstract
La presente invención se refiere a una composición sulfurada, preparada por la reacción, a una temperatura delevada, de un agente sulfurador con una mezcla de reactivos que comprende: a) al menos un éster parcial de un ácido graso de un alcohol polihídrico y b) al menos un miembro del grupo que consta de i) cuando menos un éster de ácido graso de un alcohol polihídrico, este éster de ácido graso es diferente del éster parcial (a), ii) cuando menos un ácido graso, iii) cuando menos una olefina y iv) cuando menos un éster de ácido graso de un alcohol monohídrico.
Applications Claiming Priority (1)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| US07/144,369 US4959168A (en) | 1988-01-15 | 1988-01-15 | Sulfurized compositions, and additive concentrates and lubricating oils containing same |
Publications (1)
| Publication Number | Publication Date |
|---|---|
| MX166556B true MX166556B (es) | 1993-01-18 |
Family
ID=22508283
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| MX014544A MX166556B (es) | 1988-01-15 | 1989-01-13 | Composiciones sulfuradas y concentrados de aditivos y aceites lubricantes que las contienen |
Country Status (13)
| Country | Link |
|---|---|
| US (1) | US4959168A (es) |
| EP (1) | EP0357692B1 (es) |
| JP (1) | JP2807299B2 (es) |
| AT (1) | ATE83005T1 (es) |
| AU (1) | AU612762B2 (es) |
| BR (1) | BR8807416A (es) |
| CA (1) | CA1333173C (es) |
| DE (1) | DE3876438T2 (es) |
| IL (1) | IL88919A (es) |
| MX (1) | MX166556B (es) |
| SG (1) | SG25893G (es) |
| WO (1) | WO1989006682A1 (es) |
| ZA (1) | ZA89293B (es) |
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| US5124055A (en) * | 1988-03-31 | 1992-06-23 | Ethyl Petroleum Additives, Inc. | Lubricating oil composition |
| US5205948A (en) * | 1988-08-03 | 1993-04-27 | Mobil Oil Corp. | Sulfurized olefin-glycerol monooleate adducts and lubricant compositions containing same |
| WO1991009922A1 (en) * | 1990-01-05 | 1991-07-11 | The Lubrizol Corporation | Universal driveline fluide |
| EP0656414A3 (en) * | 1993-11-03 | 1995-11-08 | Lubrizol Corp | Sulfurized fatty acid or ester mixtures with lubricating olefins and methods of preparing them. |
| JPH08209171A (ja) * | 1994-11-15 | 1996-08-13 | Lubrizol Corp:The | チオカーバメートおよびリン含有エステルを含有する潤滑剤および流体 |
| FR2746409B1 (fr) * | 1996-03-19 | 1998-04-17 | Inst Francais Du Petrole | Procede de sulfuration de corps gras insatures par le soufre elementaire en presence de composes amines |
| US5958849A (en) * | 1997-01-03 | 1999-09-28 | Exxon Research And Engineering Co. | High performance metal working oil |
| US5703022A (en) * | 1997-01-06 | 1997-12-30 | The Lubrizol Corporation | Sulfurized vegetable oils containing anti-oxidants for use as base fluids |
| WO2007005423A2 (en) | 2005-06-29 | 2007-01-11 | The Lubrizol Corporation | Zinc-free farm tractor fluid |
| US9468600B2 (en) * | 2006-05-26 | 2016-10-18 | Dr. Holmquist Healthcare, LLC | Compositions for the transdermal delivery of physiologically active agents |
| US9023406B2 (en) * | 2011-02-17 | 2015-05-05 | Dr. Holmquist Healthcare, LLC | Amelioration of the appearance of bruises |
| US9771540B2 (en) | 2009-01-20 | 2017-09-26 | Exxonmobil Research And Engineering Company | Hydraulic oil compositions with improved hydraulic motor efficiency |
| US20110287989A1 (en) | 2009-01-20 | 2011-11-24 | The Lubrizol Corporation | Hydraulic Composition with Improved Wear Properties |
| JP5575815B2 (ja) | 2009-02-18 | 2014-08-20 | ザ ルブリゾル コーポレイション | 潤滑剤中の摩擦調整剤としてのアミン誘導体 |
| JP5748783B2 (ja) | 2010-02-19 | 2015-07-15 | トヨタ自動車株式会社 | ナトリウム清浄剤の使用により高い動的摩擦係数を与える湿式摩擦クラッチ−潤滑剤系 |
| SG183389A1 (en) | 2010-02-19 | 2012-09-27 | Infineum Int Ltd | Wet friction clutch-lubricant systems providing high dynamic coefficients of friction through the use of borated detergents |
| CN103534341B (zh) | 2011-05-12 | 2015-12-09 | 路博润公司 | 作为润滑剂添加剂的芳族酰亚胺和酯 |
| CA2842660C (en) | 2011-07-21 | 2019-05-28 | The Lubrizol Corporation | Carboxylic pyrrolidinones and methods of use thereof |
| RU2509144C1 (ru) * | 2012-10-25 | 2014-03-10 | Юрий Александрович Макунин | Смазка для механической обработки металлов |
| WO2015171364A1 (en) | 2014-05-06 | 2015-11-12 | The Lubrizol Corporation | Anti-corrosion additives |
| JP6525439B2 (ja) | 2014-06-27 | 2019-06-05 | ザ ルブリゾル コーポレイションThe Lubrizol Corporation | トランスミッション流体に良好な摩擦性能を提供する摩擦調整剤の混合物 |
| EP3177700B1 (en) * | 2014-08-06 | 2022-03-02 | The Lubrizol Corporation | Industrial gear lubricant with biodegradable sulfur component |
| WO2016144639A1 (en) | 2015-03-10 | 2016-09-15 | The Lubrizol Corporation | Lubricating compositions comprising an anti-wear/friction modifying agent |
| BR112017021697B1 (pt) | 2015-04-09 | 2020-11-24 | The Lubrizol Corporation | Lubrificantes que cont£m componentes quaternarios de am6nio |
| WO2017079123A1 (en) | 2015-11-02 | 2017-05-11 | Lubrizol Oilfield Solutions, Inc. | Lubricant for water based drilling fluid |
| US20190119594A1 (en) | 2016-04-20 | 2019-04-25 | The Lubrizol Corporation | Lubricant for two-stroke cycle engines |
| WO2017205271A1 (en) | 2016-05-24 | 2017-11-30 | The Lubrizol Corporation | Seal swell agents for lubricating compositions |
| US11193081B2 (en) | 2016-05-24 | 2021-12-07 | The Lubrizol Corporation | Seal swell agents for lubricating compositions |
| WO2017205274A1 (en) | 2016-05-24 | 2017-11-30 | The Lubrizol Corporation | Seal swell agents for lubricating compositions |
| US20200017794A1 (en) | 2016-09-21 | 2020-01-16 | The Lubrizol Corporation | Fluorinated polyacrylate antifoam components for lubricating compositions |
| BR112019005332A2 (pt) | 2016-09-21 | 2019-06-11 | Lubrizol Corp | componentes antiespumantes de poliacrilato para uso em combustíveis de diesel |
| CA3045129A1 (en) | 2016-12-16 | 2018-06-21 | The Lubrizol Corporation | Lubrication of an automatic transmission with reduced wear on a needle bearing |
| CN110312781A (zh) | 2016-12-22 | 2019-10-08 | 路博润公司 | 用于润滑组合物的氟化聚丙烯酸酯消泡组分 |
| WO2018125956A1 (en) | 2016-12-30 | 2018-07-05 | Exxonmobil Research And Engineering Company | Low viscosity lubricating oil compositions for turbomachines |
| US20190040335A1 (en) | 2017-08-04 | 2019-02-07 | Exxonmobil Research And Engineering Company | Novel formulation for lubrication of hyper compressors providing improved pumpability under high-pressure conditions |
| US20190085256A1 (en) | 2017-09-18 | 2019-03-21 | Exxonmobil Research And Engineering Company | Hydraulic oil compositions with improved hydrolytic and thermo-oxidative stability |
| US20190136147A1 (en) | 2017-11-03 | 2019-05-09 | Exxonmobil Research And Engineering Company | Lubricant compositions with improved performance and methods of preparing and using the same |
| US10774286B2 (en) | 2017-12-29 | 2020-09-15 | Exxonmobil Research And Engineering Company | Grease compositions with improved performance and methods of preparing and using the same |
| WO2019133191A1 (en) | 2017-12-29 | 2019-07-04 | Exxonmobil Research And Engineering Company | Lubrication of oxygenated diamond-like carbon surfaces |
| CA3094651A1 (en) | 2018-03-21 | 2019-09-26 | The Lubrizol Corporation | Novel fluorinated polyacrylates antifoams in ultra-low viscosity (<5 cst) finished fluids |
| US20190376000A1 (en) | 2018-06-11 | 2019-12-12 | Exxonmobil Research And Engineering Company | Non-zinc-based antiwear compositions, hydraulic oil compositions, and methods of using the same |
| US20190382680A1 (en) | 2018-06-18 | 2019-12-19 | Exxonmobil Research And Engineering Company | Formulation approach to extend the high temperature performance of lithium complex greases |
| GB201817589D0 (en) * | 2018-10-29 | 2018-12-12 | Castrol Ltd | Lubricant compositions |
| WO2020131603A1 (en) | 2018-12-18 | 2020-06-25 | Bp Corporation North America Inc. | Lubricating composition comprising a sulfur-containing carboxylic acid or ester additive |
| US20200199485A1 (en) | 2018-12-19 | 2020-06-25 | Exxonmobil Research And Engineering Company | Grease compositions having polyurea thickeners made with isocyanate terminated prepolymers |
| WO2020131441A1 (en) | 2018-12-19 | 2020-06-25 | Exxonmobil Research And Engineering Company | Grease compositions having improved performance |
| WO2020131440A1 (en) | 2018-12-19 | 2020-06-25 | Exxonmobil Research And Engineering Company | Grease compositions having calcium sulfonate and polyurea thickeners |
| US11760952B2 (en) | 2021-01-12 | 2023-09-19 | Ingevity South Carolina, Llc | Lubricant thickener systems from modified tall oil fatty acids, lubricating compositions, and associated methods |
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| US2113811A (en) * | 1936-12-28 | 1938-04-12 | Continental Oil Co | Sulphurized oils |
| US2542161A (en) * | 1946-03-09 | 1951-02-20 | Pure Oil Co | Mineral oil lubricant containing phosphorized and sulfurized glyceryl trioleate |
| US2541789A (en) * | 1947-04-10 | 1951-02-13 | Pure Oil Co | Mineral oil lubricant containing sulfurized and phosphorized propylene and butylene glycol esters of oleic acid |
| US2672444A (en) * | 1948-06-05 | 1954-03-16 | Standard Oil Dev Co | Rust preventive compositions |
| NL75274C (es) * | 1950-07-13 | |||
| US2845438A (en) * | 1955-10-13 | 1958-07-29 | Frederick E Dearborn | Esters of glycols and sulfurized fatty acids |
| US3455896A (en) * | 1966-09-06 | 1969-07-15 | Standard Oil Co | Reaction products of sulfurized polybutenes and triglycerides |
| US3455830A (en) * | 1966-12-19 | 1969-07-15 | Kendall Refining Co | Co-sulfur condensed petroleum fraction and a reactive monomer composition |
| US3825495A (en) * | 1971-02-19 | 1974-07-23 | Sun Research Development | Lubricant for controlled-slip differential |
| US4487705A (en) * | 1971-02-19 | 1984-12-11 | Sun Ventures, Inc. | Oil containing a cosulfurized olefin-triglyceride blend |
| US4180466A (en) * | 1971-02-19 | 1979-12-25 | Sun Ventures, Inc. | Method of lubrication of a controlled-slip differential |
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| US4166797A (en) * | 1971-04-19 | 1979-09-04 | Suntech, Inc. | Oil containing a consulfurized olefin-triglyceride blend |
| US4166796A (en) * | 1971-04-19 | 1979-09-04 | Suntech, Inc. | Composition comprising a cosulfurized blend of lard oil and an olefin |
| US4321153A (en) * | 1971-04-19 | 1982-03-23 | Suntech, Inc. | Process of sulfurizing triglyceride and an olefin |
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| US4176072A (en) * | 1978-03-22 | 1979-11-27 | Ethyl Corporation | Diesel engine crankcase lubricating oil composition |
| DE2842138A1 (de) * | 1978-09-28 | 1980-04-10 | Rhein Chemie Rheinau Gmbh | Schwefelhaltige umsetzungsprodukte, verfahren zu ihrer herstellung und verwendung als zusatz zu schmiermitteln |
| US4456540A (en) * | 1979-06-18 | 1984-06-26 | Sun Tech, Inc. | Process of sulfurizing triglyceride and an olefin |
| US4594171A (en) * | 1981-05-20 | 1986-06-10 | Mobil Oil Corporation | Friction reducing additives and compositions thereof |
| CA1294611C (en) * | 1985-04-25 | 1992-01-21 | Frederick William Koch | Sulfur-containing compositions, and additive concentrates, lubricating oils and metal working lubricants containing same |
| US4708753A (en) * | 1985-12-06 | 1987-11-24 | The Lubrizol Corporation | Water-in-oil emulsions |
-
1988
- 1988-01-15 US US07/144,369 patent/US4959168A/en not_active Expired - Lifetime
- 1988-12-22 AU AU28297/89A patent/AU612762B2/en not_active Ceased
- 1988-12-22 DE DE8989901044T patent/DE3876438T2/de not_active Expired - Fee Related
- 1988-12-22 BR BR888807416A patent/BR8807416A/pt not_active Application Discontinuation
- 1988-12-22 JP JP1500926A patent/JP2807299B2/ja not_active Expired - Lifetime
- 1988-12-22 EP EP89901044A patent/EP0357692B1/en not_active Expired - Lifetime
- 1988-12-22 AT AT89901044T patent/ATE83005T1/de not_active IP Right Cessation
- 1988-12-22 WO PCT/US1988/004634 patent/WO1989006682A1/en not_active Ceased
-
1989
- 1989-01-06 CA CA000587674A patent/CA1333173C/en not_active Expired - Fee Related
- 1989-01-10 IL IL88919A patent/IL88919A/xx not_active IP Right Cessation
- 1989-01-13 ZA ZA89293A patent/ZA89293B/xx unknown
- 1989-01-13 MX MX014544A patent/MX166556B/es unknown
-
1993
- 1993-03-09 SG SG258/93A patent/SG25893G/en unknown
Also Published As
| Publication number | Publication date |
|---|---|
| DE3876438D1 (de) | 1993-01-14 |
| ZA89293B (en) | 1989-10-25 |
| EP0357692B1 (en) | 1992-12-02 |
| AU612762B2 (en) | 1991-07-18 |
| WO1989006682A1 (en) | 1989-07-27 |
| JP2807299B2 (ja) | 1998-10-08 |
| US4959168A (en) | 1990-09-25 |
| EP0357692A1 (en) | 1990-03-14 |
| BR8807416A (pt) | 1990-03-27 |
| IL88919A0 (en) | 1989-08-15 |
| AU2829789A (en) | 1989-08-11 |
| SG25893G (en) | 1993-05-21 |
| DE3876438T2 (de) | 1993-06-09 |
| JPH02502922A (ja) | 1990-09-13 |
| IL88919A (en) | 1993-01-31 |
| CA1333173C (en) | 1994-11-22 |
| ATE83005T1 (de) | 1992-12-15 |
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